Evidence for Topological Magnon–Phonon Hybridization in a 2D Antiferromagnet down to the Monolayer Limit

• Published in: Nano letters Vol. 23; no. 5; pp. 2023 - 2030
• Main Authors: Luo, Jiaming, Li, Shuyi, Ye, Zhipeng, Xu, Rui, Yan, Han, Zhang, Junjie, Ye, Gaihua, Chen, Lebing, Hu, Ding, Teng, Xiaokun, Smith, William A., Yakobson, Boris I., Dai, Pengcheng, Nevidomskyy, Andriy H., He, Rui, Zhu, Hanyu
• Format: Journal Article
• Language: English
• Published: United States American Chemical Society 08.03.2023
• Subjects: two-dimensional antiferromagnets; terahertz magnons in monolayers; magnon−phonon hybridization; chiral topological phonons
• ISSN: 1530-6984; 1530-6992
• DOI: 10.1021/acs.nanolett.3c00351

Topological phonons and magnons potentially enable low-loss, quantum coherent, and chiral transport of information and energy at the atomic scale. Van der Waals magnetic materials are promising to realize such states due to their recently discovered strong interactions among the electronic, spin, and lattice degrees of freedom. Here, we report the first observation of coherent hybridization of magnons and phonons in monolayer antiferromagnet FePSe3 by cavity-enhanced magneto-Raman spectroscopy. The robust magnon–phonon cooperativity in the 2D limit occurs even in zero magnetic field, which enables nontrivial band inversion between longitudinal and transverse optical phonons caused by the strong coupling with magnons. The spin and lattice symmetry theoretically guarantee magnetic-field-controlled topological phase transition, verified by nonzero Chern numbers calculated from the coupled spin–lattice model. The 2D topological magnon–phonon hybridization potentially offers a new route toward quantum phononics and magnonics with an ultrasmall footprint.