Parallel Carbon Nanotube Stripes in Polymer Thin Film with Remarkable Conductive Anisotropy
In our previous study (Mao et al. J. Phys. Chem. Lett. 2013, 4, 43−47 ), we proposed a novel method, that is, the shear-flow-induced hierarchical self-assembly of two-dimensional fillers (octadecylamine-functionalized graphene) into the well-ordered parallel stripes in a polymer matrix, to fabricate...
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| Published in | ACS applied materials & interfaces Vol. 6; no. 3; pp. 1754 - 1758 |
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| Main Authors | , , , , , |
| Format | Journal Article |
| Language | English |
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American Chemical Society
12.02.2014
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| Abstract | In our previous study (Mao et al. J. Phys. Chem. Lett. 2013, 4, 43−47 ), we proposed a novel method, that is, the shear-flow-induced hierarchical self-assembly of two-dimensional fillers (octadecylamine-functionalized graphene) into the well-ordered parallel stripes in a polymer matrix, to fabricate the anisotropic conductive materials. In this study, we extend this method to one-dimensional multiwalled carbon nanotubes (MWCNTs). Under the induction of shear flow, the dispersed poly(styrene ethylene/butadiene-styrene) (SEBS) phase and MWCNTs can spontaneously assemble into well-ordered parallel stripes in the polypropylene (PP) thin film. The electrical measurements indicate that the electrical resistivity in the direction parallel to the stripes is almost 6 orders of magnitude lower than that in the perpendicular direction, which is by far the most striking conductive anisotropy for the plastic anisotropic conductive materials. In addition, it is found that the size of the MWCNT stripe as well as the electrical property of the resulting anisotropic conductive thin film can be well-controlled by the gap of the shear cell. |
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| AbstractList | In our previous study (Mao et al. J. Phys. Chem. Lett. 2013, 4, 43−47 ), we proposed a novel method, that is, the shear-flow-induced hierarchical self-assembly of two-dimensional fillers (octadecylamine-functionalized graphene) into the well-ordered parallel stripes in a polymer matrix, to fabricate the anisotropic conductive materials. In this study, we extend this method to one-dimensional multiwalled carbon nanotubes (MWCNTs). Under the induction of shear flow, the dispersed poly(styrene ethylene/butadiene-styrene) (SEBS) phase and MWCNTs can spontaneously assemble into well-ordered parallel stripes in the polypropylene (PP) thin film. The electrical measurements indicate that the electrical resistivity in the direction parallel to the stripes is almost 6 orders of magnitude lower than that in the perpendicular direction, which is by far the most striking conductive anisotropy for the plastic anisotropic conductive materials. In addition, it is found that the size of the MWCNT stripe as well as the electrical property of the resulting anisotropic conductive thin film can be well-controlled by the gap of the shear cell. In our previous study ( Mao et al. J. Phys. Chem. Lett. 2013 , 4 , 43 - 47 ), we proposed a novel method, that is, the shear-flow-induced hierarchical self-assembly of two-dimensional fillers (octadecylamine-functionalized graphene) into the well-ordered parallel stripes in a polymer matrix, to fabricate the anisotropic conductive materials. In this study, we extend this method to one-dimensional multiwalled carbon nanotubes (MWCNTs). Under the induction of shear flow, the dispersed poly(styrene ethylene/butadiene-styrene) (SEBS) phase and MWCNTs can spontaneously assemble into well-ordered parallel stripes in the polypropylene (PP) thin film. The electrical measurements indicate that the electrical resistivity in the direction parallel to the stripes is almost 6 orders of magnitude lower than that in the perpendicular direction, which is by far the most striking conductive anisotropy for the plastic anisotropic conductive materials. In addition, it is found that the size of the MWCNT stripe as well as the electrical property of the resulting anisotropic conductive thin film can be well-controlled by the gap of the shear cell. |
| Author | Zhu, Yutian Yin, Jinghua Yang, Xiaodong Jiang, Wei Huang, Jinrui Tang, Qingxin |
| AuthorAffiliation | Chinese Academy of Sciences Changchun Institute of Technology Key Laboratory of UV Light Emitting Materials and Technology under Ministry of Education Northeast Normal University State Key Laboratory of Polymer Physics and Chemistry, Changchun Institute of Applied Chemistry University of Chinese Academy of Sciences |
| AuthorAffiliation_xml | – name: Key Laboratory of UV Light Emitting Materials and Technology under Ministry of Education – name: University of Chinese Academy of Sciences – name: Northeast Normal University – name: Chinese Academy of Sciences – name: Changchun Institute of Technology – name: State Key Laboratory of Polymer Physics and Chemistry, Changchun Institute of Applied Chemistry |
| Author_xml | – sequence: 1 givenname: Jinrui surname: Huang fullname: Huang, Jinrui – sequence: 2 givenname: Yutian surname: Zhu fullname: Zhu, Yutian email: ytzhu@ciac.ac.cn – sequence: 3 givenname: Wei surname: Jiang fullname: Jiang, Wei email: wjiang@ciac.ac.cn – sequence: 4 givenname: Jinghua surname: Yin fullname: Yin, Jinghua – sequence: 5 givenname: Qingxin surname: Tang fullname: Tang, Qingxin – sequence: 6 givenname: Xiaodong surname: Yang fullname: Yang, Xiaodong |
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