All-Optical Tunability of Metalenses Permeated with Liquid Crystals

• Published in: ACS nano Vol. 16; no. 10; pp. 16539 - 16548
• Main Authors: Palermo, Giovanna, Lininger, Andrew, Guglielmelli, Alexa, Ricciardi, Loredana, Nicoletta, Giuseppe, De Luca, Antonio, Park, Joon-Suh, Lim, Soon Wei Daniel, Meretska, Maryna L., Capasso, Federico, Strangi, Giuseppe
• Format: Journal Article
• Language: English
• Published: American Chemical Society 25.10.2022
• Subjects: reconfigurable; metalens; tunable; liquid crystal; metasurface; thermoplasmonics
• ISSN: 1936-0851; 1936-086X
• DOI: 10.1021/acsnano.2c05887

Metasurfaces have been extensively engineered to produce a wide range of optical phenomena, allowing exceptional control over the propagation of light. However, they are generally designed as single-purpose devices without a modifiable postfabrication optical response, which can be a limitation to real-world applications. In this work, we report a nanostructured planar-fused silica metalens permeated with a nematic liquid crystal (NLC) and gold nanoparticle solution. The physical properties of embedded NLCs can be manipulated with the application of external stimuli, enabling reconfigurable optical metasurfaces. We report the all-optical, dynamic control of the metalens optical response resulting from thermoplasmonic-induced changes of the NLC solution associated with the nematic–isotropic phase transition. A continuous and reversible tuning of the metalens focal length is experimentally demonstrated, with a variation of 80 μm (0.16% of the 5 cm nominal focal length) along the optical axis. This is achieved without direct mechanical or electrical manipulation of the device. The reconfigurable properties are compared with corroborating numerical simulations of the focal length shift and exhibit close correspondence.