Shape-Memory Three-Dimensional Evaporators with High Portability for Efficient Solar-Driven Freshwater Production

• Published in: ACS applied materials & interfaces Vol. 15; no. 44; pp. 51289 - 51299
• Main Authors: Zhang, Xintao, Liu, Ji, Han, Shuang, Li, Wei, Li, Changjun, Gao, Fu-Lin, Shu, Chao, Yu, Zhong-Zhen, Li, Xiaofeng
• Format: Journal Article
• Language: English
• Published: American Chemical Society 08.11.2023
• Subjects: Energy, Environmental, and Catalysis Applications; solar vapor generation; portability; shape-memory effect; 3D evaporator; seawater desalination
• ISSN: 1944-8244; 1944-8252
• DOI: 10.1021/acsami.3c13297

Solar-driven water evaporation can alleviate the severe water scarcity situation in a nonpolluting and sustainable manner. Although the design of integrated three-dimensional (3D) solar evaporators has been proven to be effective in achieving ultrahigh evaporation rates and energy efficiency, their scalable application is still hindered by complex manufacturing processes and poor portability. Herein, we report a highly portable shape-memory 3D solar evaporator by depositing MXene on low-cost lignin-cellulosic sponges for freshwater production. When not in use, the 3D evaporator can be compressed into a thin film with up to 89.3% volume reduction, ensuring minimal space occupation and high portability. When needed, due to the shape-memory effect, the 3D structure can be rapidly restored by swelling the compressed film in water, resulting in an efficient 3D solar evaporator. This 3D evaporator exhibits not only a high evaporation rate of 2.48 kg m–2 h–1 under 1 sun illumination but also excellent long-term stability and recyclability. In addition, the 3D evaporator itself can serve as a water reservoir without requiring a continuous water supply during evaporation, showing remarkable application flexibility. This work opens a new perspective for manufacturing highly portable and efficient 3D solar evaporators and may facilitate their progress from the laboratory to commercial applications.