Correlating Molecular Structure to Field-Effect Mobility: The Investigation of Side-Chain Functionality in Phenylene−Thiophene Oligomers and Their Application in Field Effect Transistors
Short conjugated phenylene (P)−thiophene (T) oligomers with varying α and ω alkyl and alkoxy substitutions were synthesized using Stille and Suzuki coupling reactions to investigate the correlation between end-group structure and electronic properties on P2TP and P3TP conjugated cores. Several solub...
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Published in | Chemistry of materials Vol. 19; no. 9; pp. 2342 - 2351 |
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Main Authors | , , , , |
Format | Journal Article |
Language | English |
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American Chemical Society
01.05.2007
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Abstract | Short conjugated phenylene (P)−thiophene (T) oligomers with varying α and ω alkyl and alkoxy substitutions were synthesized using Stille and Suzuki coupling reactions to investigate the correlation between end-group structure and electronic properties on P2TP and P3TP conjugated cores. Several soluble oligomers were synthesized with 5,5‘-bis(4-n-octylphenyl)-2,2‘-bithiophene (do-PTTP) showing the highest mobility (μ = 0.18 cm2 V-1 s-1) and on/off ratio of 107 at a substrate temperature of 50 °C. Thin film morphologies analyzed using atomic force microscopy revealed higher nucleation densities for branched alkoxy side-chain molecules compared to those of their straight alkyl side-chain counterparts. Field-effect mobility showed an inverse correlation to side-group bulkiness, indicating a strong morphological component to charge transport in the P2TP and P3TP series. |
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AbstractList | Short conjugated phenylene (P)−thiophene (T) oligomers with varying α and ω alkyl and alkoxy substitutions were synthesized using Stille and Suzuki coupling reactions to investigate the correlation between end-group structure and electronic properties on P2TP and P3TP conjugated cores. Several soluble oligomers were synthesized with 5,5‘-bis(4-n-octylphenyl)-2,2‘-bithiophene (do-PTTP) showing the highest mobility (μ = 0.18 cm2 V-1 s-1) and on/off ratio of 107 at a substrate temperature of 50 °C. Thin film morphologies analyzed using atomic force microscopy revealed higher nucleation densities for branched alkoxy side-chain molecules compared to those of their straight alkyl side-chain counterparts. Field-effect mobility showed an inverse correlation to side-group bulkiness, indicating a strong morphological component to charge transport in the P2TP and P3TP series. |
Author | Tang, Ming Lee Ling, Mang Mang Sung, Andrew Locklin, Jason Bao, Zhenan |
Author_xml | – sequence: 1 givenname: Andrew surname: Sung fullname: Sung, Andrew – sequence: 2 givenname: Mang Mang surname: Ling fullname: Ling, Mang Mang – sequence: 3 givenname: Ming Lee surname: Tang fullname: Tang, Ming Lee – sequence: 4 givenname: Zhenan surname: Bao fullname: Bao, Zhenan – sequence: 5 givenname: Jason surname: Locklin fullname: Locklin, Jason |
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Title | Correlating Molecular Structure to Field-Effect Mobility: The Investigation of Side-Chain Functionality in Phenylene−Thiophene Oligomers and Their Application in Field Effect Transistors |
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