Nanovortex-driven all-dielectric optical diffusion boosting and sorting concept for lab-on-a-chip platforms

• Published in: arXiv.org
• Main Authors: Valero, Adrià Canós, Kislov, Denis, Gurvitz, Egor A, Shamkhi, Hadi K, Redka, Dmitrii, Yankin, Sergey, Zemánek, Pavel, Shalin, Alexander S
• Format: Paper
• Language: English
• Published: Ithaca Cornell University Library, arXiv.org 24.10.2019
• Subjects: Angular momentum; Biomolecules; Chemical synthesis; Dependence; Dielectric strength; Emulsions; Fluid dynamics; Fluid flow; Laser beams; Microfluidics; Microreactors; Miniaturization; Momentum transfer; Nanoparticles; Organic chemistry; Particle diffusion; Radiation pressure; Stability

The ever-growing field of microfluidics requires precise and flexible control over fluid flow at the micro- and nanoscales. Current constraints demand a variety of controllable components for performing different operations inside closed microchambers and microreactors. In this context, novel nanophotonic approaches can significantly enhance existing capabilities and provide new functionalities via finely tuned light-matter interaction mechanisms. Here we propose a novel design, featuring a dual functionality on-chip: boosted optically-driven particle diffusion and nanoparticle sorting. Our methodology is based on a specially designed high-index dielectric nanoantenna, which strongly enhances spin-orbit angular momentum transfer from an incident laser beam to the scattered field. As a result, exceptionally compact, subwavelength optical nanovortices are formed and drive spiral motion of peculiar plasmonic nanoparticles via the efficient interplay between curled spin optical forces and radiation pressure. The nanovortex size is an order of magnitude smaller than that provided by conventional beam-based approaches. The nanoparticles mediate nano-confined fluid motion enabling nanomixing without a need of moving bulk elements inside a microchamber. Moreover, precise sorting of gold nanoparticles, demanded for on-chip separation and filtering, can be achieved by exploiting the non-trivial dependence of the curled optical forces on the nanoobject size. Altogether, this study introduces a versatile platform for further miniaturization of moving-part-free, optically driven microfluidic chips for fast chemical synthesis and analysis, preparation of emulsions, or generation of chemical gradients with light-controlled navigation of nanoparticles, viruses or biomolecules.