CONJUGATE, CATALYST AND METHOD FOR PRODUCING AMMONIA
The present invention relates to a complex including a mayenite type compound and an active metal supported on the mayenite type compound, wherein after heating the complex from a temperature of 20°C to a temperature of 450°C at a temperature rise rate of 10°C/min and then holding in an environment...
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Format | Patent |
Language | English French German |
Published |
16.12.2020
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Abstract | The present invention relates to a complex including a mayenite type compound and an active metal supported on the mayenite type compound, wherein after heating the complex from a temperature of 20°C to a temperature of 450°C at a temperature rise rate of 10°C/min and then holding in an environment at a temperature of 450°C and a pressure of 3 MPa for 10 hours while bringing a mixed gas containing a nitrogen gas and a hydrogen gas at a volume ratio of the nitrogen gas to the hydrogen gas of 1/3 into contact with the complex, an average particle diameter of the active metal is less than 5.5 nm, and in the active metal, a proportion of an active metal having a particle diameter of 1 nm or more and less than 3 nm is 60% or more. A catalyst of the present invention contains the complex of the present invention. A method for producing ammonia of the present invention includes a step of producing ammonia by bringing a gas containing nitrogen and hydrogen into contact with the catalyst of the present invention. In accordance with the present invention, a complex from which a catalyst having high catalytic activity can be obtained, a catalyst containing the complex, and a method for producing ammonia using the catalyst can be provided. |
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AbstractList | The present invention relates to a complex including a mayenite type compound and an active metal supported on the mayenite type compound, wherein after heating the complex from a temperature of 20°C to a temperature of 450°C at a temperature rise rate of 10°C/min and then holding in an environment at a temperature of 450°C and a pressure of 3 MPa for 10 hours while bringing a mixed gas containing a nitrogen gas and a hydrogen gas at a volume ratio of the nitrogen gas to the hydrogen gas of 1/3 into contact with the complex, an average particle diameter of the active metal is less than 5.5 nm, and in the active metal, a proportion of an active metal having a particle diameter of 1 nm or more and less than 3 nm is 60% or more. A catalyst of the present invention contains the complex of the present invention. A method for producing ammonia of the present invention includes a step of producing ammonia by bringing a gas containing nitrogen and hydrogen into contact with the catalyst of the present invention. In accordance with the present invention, a complex from which a catalyst having high catalytic activity can be obtained, a catalyst containing the complex, and a method for producing ammonia using the catalyst can be provided. |
Author | HOSONO, Hideo KITANO, Masaaki KISHIDA, Kazuhisa INOUE, Yasunori ITO, Munenobu KAWAMURA, Shigeki YOKOYAMA, Toshiharu |
Author_xml | – fullname: YOKOYAMA, Toshiharu – fullname: KAWAMURA, Shigeki – fullname: KISHIDA, Kazuhisa – fullname: ITO, Munenobu – fullname: HOSONO, Hideo – fullname: INOUE, Yasunori – fullname: KITANO, Masaaki |
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DocumentTitleAlternate | KONJUGAT, KATALYSATOR UND VERFAHREN ZUR HERSTELLUNG VON AMMONIAK CONJUGUÉ, CATALYSEUR ET PROCÉDÉ DE PRODUCTION D'AMMONIAC |
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RelatedCompanies | Tokyo Institute of Technology Tsubame BHB Co., Ltd |
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Snippet | The present invention relates to a complex including a mayenite type compound and an active metal supported on the mayenite type compound, wherein after... |
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SubjectTerms | AMMONIA CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOIDCHEMISTRY CHEMISTRY COMPOUNDS OF THE METALS BERYLLIUM, MAGNESIUM, ALUMINIUM,CALCIUM, STRONTIUM, BARIUM, RADIUM, THORIUM, OR OF THERARE-EARTH METALS COMPOUNDS THEREOF CYANOGEN INORGANIC CHEMISTRY METALLURGY PERFORMING OPERATIONS PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL THEIR RELEVANT APPARATUS TRANSPORTING |
Title | CONJUGATE, CATALYST AND METHOD FOR PRODUCING AMMONIA |
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