Study on expansion characteristics of Al–Al 2 O 3 composite seals for intermediate‐temperature solid oxide fuel cell

Abstract Al 2 O 3 ‐based composite seal with 10 wt% Al powder addition (A10) possesses excellent plastic and mechanical performance under wide temperature range of solid oxide fuel cell. The thickening phenomenon of A10 seal between 250°C–400°C and 600°C–750°C is caused by the thermal expansion of o...

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Published inInternational journal of applied ceramic technology Vol. 21; no. 6; pp. 4091 - 4099
Main Authors Xu, Shanping, Wang, Xiaochun, Kang, Jie, Wang, Wei, Ding, Yun, Zhao, Xuepeng, Wang, Yaocheng, Li, Li
Format Journal Article
LanguageEnglish
Published 01.11.2024
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Abstract Abstract Al 2 O 3 ‐based composite seal with 10 wt% Al powder addition (A10) possesses excellent plastic and mechanical performance under wide temperature range of solid oxide fuel cell. The thickening phenomenon of A10 seal between 250°C–400°C and 600°C–750°C is caused by the thermal expansion of organic additives and the volume expansion when solid–liquid Al react with oxygen to form Al 2 O 3 . The thickness change rate reaches the maximum which is about 5% at 300°C and is about 4.46% at 650°C. The Gibbs free energy for reaction between Al and Al 2 O 3 in the temperature range of 523–1 023 K is all less than 0, which is proved by the fact that A10 exhibits excellent self‐expansion and thermodynamic properties in the solid oxide fuel cell operating temperature.
AbstractList Abstract Al 2 O 3 ‐based composite seal with 10 wt% Al powder addition (A10) possesses excellent plastic and mechanical performance under wide temperature range of solid oxide fuel cell. The thickening phenomenon of A10 seal between 250°C–400°C and 600°C–750°C is caused by the thermal expansion of organic additives and the volume expansion when solid–liquid Al react with oxygen to form Al 2 O 3 . The thickness change rate reaches the maximum which is about 5% at 300°C and is about 4.46% at 650°C. The Gibbs free energy for reaction between Al and Al 2 O 3 in the temperature range of 523–1 023 K is all less than 0, which is proved by the fact that A10 exhibits excellent self‐expansion and thermodynamic properties in the solid oxide fuel cell operating temperature.
Author Li, Li
Xu, Shanping
Wang, Wei
Wang, Xiaochun
Ding, Yun
Zhao, Xuepeng
Wang, Yaocheng
Kang, Jie
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