Modulation of photophysical properties in o -carborane derivatives and their application in white organic light-emitting diode devices
Two derivatives of o -carborane ( o -Cb) were synthesized, enabling effective modulation of their photophysical properties by varying the substituents on the carbon atom within the o -Cb cage. CAPCb incorporates phenyl groups into the carbazole–anthracene motif, demonstrating weak dual emissions in...
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Published in | Journal of materials chemistry. C, Materials for optical and electronic devices |
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Main Authors | , , , , , , |
Format | Journal Article |
Language | English |
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2024
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Abstract | Two derivatives of o -carborane ( o -Cb) were synthesized, enabling effective modulation of their photophysical properties by varying the substituents on the carbon atom within the o -Cb cage. CAPCb incorporates phenyl groups into the carbazole–anthracene motif, demonstrating weak dual emissions in solution due to efficient charge transfer (CT) from the carbazole to the o -Cb groups. In contrast, its methyl analog (CAMCb) primarily emits from a locally excited (LE) state in solution. The most notable characteristics were revealed in their solid-state photochemistry. CAMCb displayed multiple photoemissions in the film state, featuring strong LE emission at 450 nm and slightly weaker CT emission at 640 nm. In comparison, CAPCb exhibited weaker LE emission at 430 nm and stronger CT emission at 620 nm. This indicates that the CT states can be selectively activated or deactivated based on the substituents on the o -Cb and the phase. Minor modifications in molecular geometries through changes in the substituents at the o -Cb cage significantly influence their excited-state properties and emission characteristics. The distinct properties of CAPCb and CAMCb were utilized in the fabrication of white OLED devices, which demonstrated cool white emission with Commission Internationale de L’Eclairage (CIE) coordinates of (0.37, 0.30) and a correlated color temperature (CCT) of 3556 K measured at 500 cd m −2 . |
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AbstractList | Two derivatives of o -carborane ( o -Cb) were synthesized, enabling effective modulation of their photophysical properties by varying the substituents on the carbon atom within the o -Cb cage. CAPCb incorporates phenyl groups into the carbazole–anthracene motif, demonstrating weak dual emissions in solution due to efficient charge transfer (CT) from the carbazole to the o -Cb groups. In contrast, its methyl analog (CAMCb) primarily emits from a locally excited (LE) state in solution. The most notable characteristics were revealed in their solid-state photochemistry. CAMCb displayed multiple photoemissions in the film state, featuring strong LE emission at 450 nm and slightly weaker CT emission at 640 nm. In comparison, CAPCb exhibited weaker LE emission at 430 nm and stronger CT emission at 620 nm. This indicates that the CT states can be selectively activated or deactivated based on the substituents on the o -Cb and the phase. Minor modifications in molecular geometries through changes in the substituents at the o -Cb cage significantly influence their excited-state properties and emission characteristics. The distinct properties of CAPCb and CAMCb were utilized in the fabrication of white OLED devices, which demonstrated cool white emission with Commission Internationale de L’Eclairage (CIE) coordinates of (0.37, 0.30) and a correlated color temperature (CCT) of 3556 K measured at 500 cd m −2 . |
Author | Jeong, Yeonju Han, Won-Sik Kim, Taekyung Lee, Jina Lee, Sunhee Lee, Yi Sak Park, Bubae |
Author_xml | – sequence: 1 givenname: Jina surname: Lee fullname: Lee, Jina organization: Department of Chemistry, Seoul Women's University, Seoul 01797, South Korea – sequence: 2 givenname: Yeonju surname: Jeong fullname: Jeong, Yeonju organization: Department of Information Display, Hongik University, Seoul 04066, South Korea – sequence: 3 givenname: Sunhee surname: Lee fullname: Lee, Sunhee organization: Department of Chemistry, Seoul Women's University, Seoul 01797, South Korea – sequence: 4 givenname: Yi Sak surname: Lee fullname: Lee, Yi Sak organization: Department of Information Display, Hongik University, Seoul 04066, South Korea – sequence: 5 givenname: Bubae surname: Park fullname: Park, Bubae organization: Department of Information Display, Hongik University, Seoul 04066, South Korea – sequence: 6 givenname: Taekyung orcidid: 0000-0001-7632-8756 surname: Kim fullname: Kim, Taekyung organization: Department of Information Display, Hongik University, Seoul 04066, South Korea, Department of Materials Science and Engineering, Hongik University, Sejong 30016, South Korea – sequence: 7 givenname: Won-Sik orcidid: 0000-0003-2900-1093 surname: Han fullname: Han, Won-Sik organization: Department of Chemistry, Seoul Women's University, Seoul 01797, South Korea |
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