天然低共熔溶剂降低卷烟烟气苯酚释放量的性能评价

TS411.2; 为开发可降低卷烟烟气中苯酚释放量的功能材料,针对苯酚酚羟基易形成氢键的特性,设计制备了36种天然低共熔溶剂(NADESs).采用傅里叶变换红外光谱(FT-IR)、元素分析(EA)和热重分析(TG)技术表征合成产物的结构和热稳定性,采用滤嘴添加剂减害性能模拟评价装置评价合成产物降低烟气苯酚释放量的性能.结果表明:①FT-IR和EA结果表明合成产物为NADESs,TG分析表明NADESs在150℃下具有良好的热稳定性.②13种NADESs对卷烟烟气中苯酚释放量的降低率高于30％,其中氯化胆碱-乙酰丙酸(ChCl-LA)、甜菜碱-乙酰丙酸(Bet-LA)、氯化胆碱-DL-乳酸(Ch...

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Published in烟草科技 Vol. 54; no. 10; pp. 37 - 44
Main Authors 王嘉琪, 孙学辉, 杨松, 胡少东, 孙培健, 余晶晶, 王宜鹏, 贾云祯, 田海英, 聂聪
Format Journal Article
LanguageChinese
Published 中国烟草总公司郑州烟草研究院,郑州高新技术产业开发区枫杨街2号 450001%河南中烟工业有限责任公司技术中心,郑州经济技术开发区第三大街8号 450000 01.10.2021
Subjects
天然低共熔溶剂;卷烟;主流烟气;苯酚;氢键;氯化胆碱
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ISSN1002-0861
DOI10.16135/j.issn1002-0861.2021.0083

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Abstract TS411.2; 为开发可降低卷烟烟气中苯酚释放量的功能材料,针对苯酚酚羟基易形成氢键的特性,设计制备了36种天然低共熔溶剂(NADESs).采用傅里叶变换红外光谱(FT-IR)、元素分析(EA)和热重分析(TG)技术表征合成产物的结构和热稳定性,采用滤嘴添加剂减害性能模拟评价装置评价合成产物降低烟气苯酚释放量的性能.结果表明:①FT-IR和EA结果表明合成产物为NADESs,TG分析表明NADESs在150℃下具有良好的热稳定性.②13种NADESs对卷烟烟气中苯酚释放量的降低率高于30％,其中氯化胆碱-乙酰丙酸(ChCl-LA)、甜菜碱-乙酰丙酸(Bet-LA)、氯化胆碱-DL-乳酸(ChCl-Lac)、L-脯氨酸-DL-乳酸(Pro-Lac)和氯化胆碱-果糖(ChCl-Fru)对苯酚的降低率高于40％.③NADESs的制备过程简单、绿色,制备成本低廉,能有效降低卷烟主流烟气苯酚的释放量.
AbstractList TS411.2; 为开发可降低卷烟烟气中苯酚释放量的功能材料,针对苯酚酚羟基易形成氢键的特性,设计制备了36种天然低共熔溶剂(NADESs).采用傅里叶变换红外光谱(FT-IR)、元素分析(EA)和热重分析(TG)技术表征合成产物的结构和热稳定性,采用滤嘴添加剂减害性能模拟评价装置评价合成产物降低烟气苯酚释放量的性能.结果表明:①FT-IR和EA结果表明合成产物为NADESs,TG分析表明NADESs在150℃下具有良好的热稳定性.②13种NADESs对卷烟烟气中苯酚释放量的降低率高于30％,其中氯化胆碱-乙酰丙酸(ChCl-LA)、甜菜碱-乙酰丙酸(Bet-LA)、氯化胆碱-DL-乳酸(ChCl-Lac)、L-脯氨酸-DL-乳酸(Pro-Lac)和氯化胆碱-果糖(ChCl-Fru)对苯酚的降低率高于40％.③NADESs的制备过程简单、绿色,制备成本低廉,能有效降低卷烟主流烟气苯酚的释放量.
Author 王嘉琪
贾云祯
胡少东
王宜鹏
孙培健
聂聪
杨松
孙学辉
余晶晶
田海英
AuthorAffiliation 中国烟草总公司郑州烟草研究院,郑州高新技术产业开发区枫杨街2号 450001%河南中烟工业有限责任公司技术中心,郑州经济技术开发区第三大街8号 450000
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Author_FL JIA Yunzhen
SUN Peijian
WANG Yipeng
TIAN Haiying
WANG Jiaqi
HU Shaodong
YANG Song
SUN Xuehui
YU Jingjing
NIE Cong
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Title 天然低共熔溶剂降低卷烟烟气苯酚释放量的性能评价
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