The Controllable Reconstruction of Bi‐MOFs for Electrochemical CO2 Reduction through Electrolyte and Potential Mediation

• Published in: Angewandte Chemie International Edition Vol. 60; no. 33; pp. 18178 - 18184
• Main Authors: Yao, Dazhi, Tang, Cheng, Vasileff, Anthony, Zhi, Xing, Jiao, Yan, Qiao, Shi‐Zhang
• Format: Journal Article
• Language: English
• Published: Weinheim Wiley Subscription Services, Inc 09.08.2021
• Edition: International ed. in English
• Subjects: Carbon dioxide; Case studies; catalyst design; Catalysts; CO2 reduction; controllable surface reconstruction; electrocatalysis; Electrocatalysts; Electrochemistry; Electrolytes; Electron microscopy; in situ characterization; Metal-organic frameworks; Raman spectra; Raman spectroscopy; Reaction mechanisms; Reconstruction; Selectivity; Stability; Working conditions

Monitoring and controlling the reconstruction of materials under working conditions is crucial for the precise identification of active sites, elucidation of reaction mechanisms, and rational design of advanced catalysts. Herein, a Bi‐based metal–organic framework (Bi‐MOF) for electrochemical CO2 re...