Modulating the Electronic Structures of Dual‐Atom Catalysts via Coordination Environment Engineering for Boosting CO2 Electroreduction

• Published in: Angewandte Chemie International Edition Vol. 61; no. 51; pp. e202215187 - n/a
• Main Authors: Gong, Yun‐Nan, Cao, Chang‐Yu, Shi, Wen‐Jie, Zhang, Ji‐Hong, Deng, Ji‐Hua, Lu, Tong‐Bu, Zhong, Di‐Chang
• Format: Journal Article
• Language: English
• Published: Weinheim Wiley Subscription Services, Inc 19.12.2022
• Edition: International ed. in English
• Subjects: Carbon dioxide; Catalysts; CO2 Electroreduction; Coordination; Coordination Environment; Density functional theory; Dual-Atom Catalyst; Electrocatalysts; Electronic Structure; Intermediates; Modulation; Synergistic Effect

Dual‐atom catalysts (DACs) have emerged as efficient electrocatalysts for CO2 reduction owing to the synergistic effect between the binary metal sites. However, rationally modulating the electronic structure of DACs to optimize the catalytic performance remains a great challenge. Herein, we report t...