Evidence of near-ambient superconductivity in a N-doped lutetium hydride
The absence of electrical resistance exhibited by superconducting materials would have enormous potential for applications if it existed at ambient temperature and pressure conditions. Despite decades of intense research efforts, such a state has yet to be realized . At ambient pressures, cuprates a...
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Published in | Nature (London) Vol. 615; no. 7951; pp. 244 - 250T |
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Main Authors | , , , , , , , , , , |
Format | Journal Article |
Language | English |
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Nature Publishing Group
09.03.2023
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Abstract | The absence of electrical resistance exhibited by superconducting materials would have enormous potential for applications if it existed at ambient temperature and pressure conditions. Despite decades of intense research efforts, such a state has yet to be realized
. At ambient pressures, cuprates are the material class exhibiting superconductivity to the highest critical superconducting transition temperatures (T
), up to about 133 K (refs.
). Over the past decade, high-pressure 'chemical precompression'
of hydrogen-dominant alloys has led the search for high-temperature superconductivity, with demonstrated T
approaching the freezing point of water in binary hydrides at megabar pressures
. Ternary hydrogen-rich compounds, such as carbonaceous sulfur hydride, offer an even larger chemical space to potentially improve the properties of superconducting hydrides
. Here we report evidence of superconductivity on a nitrogen-doped lutetium hydride with a maximum T
of 294 K at 10 kbar, that is, superconductivity at room temperature and near-ambient pressures. The compound was synthesized under high-pressure high-temperature conditions and then-after full recoverability-its material and superconducting properties were examined along compression pathways. These include temperature-dependent resistance with and without an applied magnetic field, the magnetization (M) versus magnetic field (H) curve, a.c. and d.c. magnetic susceptibility, as well as heat-capacity measurements. X-ray diffraction (XRD), energy-dispersive X-ray (EDX) and theoretical simulations provide some insight into the stoichiometry of the synthesized material. Nevertheless, further experiments and simulations are needed to determine the exact stoichiometry of hydrogen and nitrogen, and their respective atomistic positions, in a greater effort to further understand the superconducting state of the material. |
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AbstractList | The absence of electrical resistance exhibited by superconducting materials would have enormous potential for applications if it existed at ambient temperature and pressure conditions. Despite decades of intense research efforts, such a state has yet to be realized1,2. At ambient pressures, cuprates are the material class exhibiting superconductivity to the highest critical superconducting transition temperatures (Tc), up to about 133 K (refs. 3-5). Over the past decade, high-pressure 'chemical precompression'6,7 of hydrogen-dominant alloys has led the search for high-temperature superconductivity, with demonstrated Tc approaching the freezing point of water in binary hydrides at megabar pressures8-13. Ternary hydrogen-rich compounds, such as carbonaceous sulfur hydride, offer an even larger chemical space to potentially improve the properties of superconducting hydrides14-21. Here we report evidence of superconductivity on a nitrogen-doped lutetium hydride with a maximum Tc of 294 K at 10 kbar, that is, superconductivity at room temperature and near-ambient pressures. The compound was synthesized under high-pressure high-temperature conditions and then-after full recoverability-its material and superconducting properties were examined along compression pathways. These include temperature-dependent resistance with and without an applied magnetic field, the magnetization (M) versus magnetic field (H) curve, a.c. and d.c. magnetic susceptibility, as well as heat-capacity measurements. X-ray diffraction (XRD), energy-dispersive X-ray (EDX) and theoretical simulations provide some insight into the stoichiometry of the synthesized material. Nevertheless, further experiments and simulations are needed to determine the exact stoichiometry of hydrogen and nitrogen, and their respective atomistic positions, in a greater effort to further understand the superconducting state of the material. The absence of electrical resistance exhibited by superconducting materials would have enormous potential for applications if it existed at ambient temperature and pressure conditions. Despite decades of intense research efforts, such a state has yet to be realized1,2. At ambient pressures, cuprates are the material class exhibiting superconductivity to the highest critical superconducting transition temperatures (Tc), up to about 133 K (refs.3-5). Over the past decade, high-pressure 'chemical precompression'6,7 of hydrogen-dominant alloys has led the search for high-temperature superconductivity, with demonstrated Tc approaching the freezing point of water in binary hydrides at megabar pressures8-13. Ternary hydrogen-rich compounds, such as carbonaceous sulfur hydride, offer an even larger chemical space to potentially improve the properties of superconducting hydrides14-21. Here we report evidence of superconductivity on a nitrogen-doped lutetium hydride with a maximum Tc of294 K at 10 kbar, that is, superconductivity at room temperature and near-ambient pressures. The compound was synthesized under high-pressure high-temperature conditions and then-after full recoverability-its material and superconducting properties were examined along compression pathways. These include temperature-dependent resistance with and without an applied magnetic field, the magnetization (M) versus magnetic field (H) curve, a.c. and d.c. magnetic susceptibility, as well as heat-capacity measurements. X-ray diffraction (XRD), energy-dispersive X-ray (EDX) and theoretical simulations provide some insight into the stoichiometry ofthe synthesized material. Nevertheless, further experiments and simulations are needed to determine the exact stoichiometry of hydrogen and nitrogen, and their respective atomistic positions, in a greater effort to further understand the superconducting state of the material. The absence of electrical resistance exhibited by superconducting materials would have enormous potential for applications if it existed at ambient temperature and pressure conditions. Despite decades of intense research efforts, such a state has yet to be realized . At ambient pressures, cuprates are the material class exhibiting superconductivity to the highest critical superconducting transition temperatures (T ), up to about 133 K (refs. ). Over the past decade, high-pressure 'chemical precompression' of hydrogen-dominant alloys has led the search for high-temperature superconductivity, with demonstrated T approaching the freezing point of water in binary hydrides at megabar pressures . Ternary hydrogen-rich compounds, such as carbonaceous sulfur hydride, offer an even larger chemical space to potentially improve the properties of superconducting hydrides . Here we report evidence of superconductivity on a nitrogen-doped lutetium hydride with a maximum T of 294 K at 10 kbar, that is, superconductivity at room temperature and near-ambient pressures. The compound was synthesized under high-pressure high-temperature conditions and then-after full recoverability-its material and superconducting properties were examined along compression pathways. These include temperature-dependent resistance with and without an applied magnetic field, the magnetization (M) versus magnetic field (H) curve, a.c. and d.c. magnetic susceptibility, as well as heat-capacity measurements. X-ray diffraction (XRD), energy-dispersive X-ray (EDX) and theoretical simulations provide some insight into the stoichiometry of the synthesized material. Nevertheless, further experiments and simulations are needed to determine the exact stoichiometry of hydrogen and nitrogen, and their respective atomistic positions, in a greater effort to further understand the superconducting state of the material. |
Author | Pasan, Hiranya Dias, Ranga P Durkee, Dylan Dissanayake, Sachith E Salamat, Ashkan Lawler, Keith V Snider, Elliot Khalvashi-Sutter, Nugzari Munasinghe, Sasanka Dasenbrock-Gammon, Nathan McBride, Raymond |
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SubjectTerms | Ambient temperature Compression Cuprates Electrical resistivity Freezing Freezing point Heat High pressure High temperature Hydrides Hydrogen Lutetium Magnetic fields Magnetic permeability Magnetic susceptibility Melting points Nitrogen Phase transitions Pressure Recoverability Room temperature Simulation Stoichiometry Sulfur Superconductivity Synthesis Temperature Temperature dependence Transition temperatures X-ray diffraction |
Title | Evidence of near-ambient superconductivity in a N-doped lutetium hydride |
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