A Nanocomposite of Bismuth Clusters and Bi2O2CO3 Sheets for Highly Efficient Electrocatalytic Reduction of CO2 to Formate

• Published in: Angewandte Chemie International Edition Vol. 62; no. 3
• Main Authors: Lin, Li, He, Xiaoyang, Zhang, Xia‐Guang, Ma, Wenchao, Zhang, Biao, Wei, Diye, Xie, Shunji, Zhang, Qinghong, Yi, Xiaodong, Wang, Ye
• Format: Journal Article
• Language: English
• Published: Weinheim Wiley Subscription Services, Inc 16.01.2023
• Edition: International ed. in English
• Subjects: Bismuth; Carbon dioxide; Carbon Dioxide Reduction; Catalysts; Chemical reduction; Clusters; Current density; Electrochemistry; Energy conversion; Energy conversion efficiency; Formic Acid; Heterogeneous Catalysis; Nanocomposites; Selectivity

The renewable‐electricity‐driven CO2 reduction to formic acid would contribute to establishing a carbon‐neutral society. The current catalyst suffers from limited activity and stability under high selectivity and the ambiguous nature of active sites. Herein, we report a powerful Bi2S3‐derived cataly...