Bridging Thermal Catalysis and Electrocatalysis: Catalyzing CO2 Conversion with Carbon‐Based Materials

• Published in: Angewandte Chemie (International ed.) Vol. 60; no. 32; pp. 17472 - 17480
• Main Authors: Koshy, David M., Nathan, Sindhu S., Asundi, Arun S., Abdellah, Ahmed M., Dull, Samuel M., Cullen, David A., Higgins, Drew, Bao, Zhenan, Bent, Stacey F., Jaramillo, Thomas F.
• Format: Journal Article
• Language: English
• Published: Germany Wiley Subscription Services, Inc 02.08.2021; Wiley
• Edition: International ed. in English
• Subjects: Carbon dioxide; Carbon monoxide; Catalysis; Chemical reduction; Electric potential; Electrocatalysts; electrochemistry; High temperature; INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CHEMISTRY; nitrogen-doped carbon; reverse water-gas shift; Water gas; Electrochemistry; carbon dioxide; catalysis; metal, nitrogen-doped carbon; reverse water-gas shift

Understanding the differences between reactions driven by elevated temperature or electric potential remains challenging, largely due to materials incompatibilities between thermal catalytic and electrocatalytic environments. We show that Ni, N‐doped carbon (NiPACN), an electrocatalyst for the reduc...