Anomalous normal-state gap in an electron-doped cuprate

In the underdoped n-type cuprate Nd Ce CuO , long-range antiferromagnetic order reconstructs the Fermi surface, resulting in a putative antiferromagnetic metal with small Fermi pockets. Using angle-resolved photoemission spectroscopy, we observe an anomalous energy gap, an order of magnitude smaller...

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Published inScience (American Association for the Advancement of Science) Vol. 385; no. 6710; pp. 796 - 800
Main Authors Xu, Ke-Jun, He, Junfeng, Chen, Su-Di, He, Yu, Abadi, Sebastien N, Rotundu, Costel R, Lee, Young S, Lu, Dong-Hui, Guo, Qinda, Tjernberg, Oscar, Devereaux, Thomas P, Lee, Dung-Hai, Hashimoto, Makoto, Shen, Zhi-Xun
Format Journal Article
LanguageEnglish
Published United States The American Association for the Advancement of Science 16.08.2024
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Abstract In the underdoped n-type cuprate Nd Ce CuO , long-range antiferromagnetic order reconstructs the Fermi surface, resulting in a putative antiferromagnetic metal with small Fermi pockets. Using angle-resolved photoemission spectroscopy, we observe an anomalous energy gap, an order of magnitude smaller than the antiferromagnetic gap, in a wide portion of the underdoped regime and smoothly connecting to the superconducting gap at optimal doping. After considering all the known ordering tendencies in tandem with the phase diagram, we hypothesize that the normal-state gap in the underdoped n-type cuprates originates from Cooper pairing. The high temperature scale of the normal-state gap raises the prospect of engineering higher transition temperatures in the n-type cuprates comparable to those of the p-type cuprates.
AbstractList Editor’s summaryCopper oxide materials can be made superconducting by doping the parent compound with either electrons or holes. Hole-doped cuprates typically have higher transition temperatures and have been studied more extensively. Xu et al. used photoemission measurements to investigate the phase diagram of the electron-doped cuprate Nd2-xCexCuO4. An unusual energy gap was observed to develop high above the temperature of the superconducting transition. The researchers ascribed the gap to superconducting pairing lacking global coherence. —Jelena Stajic
In the underdoped n-type cuprate Nd2-xCexCuO4, long-range antiferromagnetic order reconstructs the Fermi surface, resulting in a putative antiferromagnetic metal with small Fermi pockets. Using angle-resolved photoemission spectroscopy, we observe an anomalous energy gap, an order of magnitude smaller than the antiferromagnetic gap, in a wide portion of the underdoped regime and smoothly connecting to the superconducting gap at optimal doping. After considering all the known ordering tendencies in tandem with the phase diagram, we hypothesize that the normal-state gap in the underdoped n-type cuprates originates from Cooper pairing. The high temperature scale of the normal-state gap raises the prospect of engineering higher transition temperatures in the n-type cuprates comparable to those of the p-type cuprates.In the underdoped n-type cuprate Nd2-xCexCuO4, long-range antiferromagnetic order reconstructs the Fermi surface, resulting in a putative antiferromagnetic metal with small Fermi pockets. Using angle-resolved photoemission spectroscopy, we observe an anomalous energy gap, an order of magnitude smaller than the antiferromagnetic gap, in a wide portion of the underdoped regime and smoothly connecting to the superconducting gap at optimal doping. After considering all the known ordering tendencies in tandem with the phase diagram, we hypothesize that the normal-state gap in the underdoped n-type cuprates originates from Cooper pairing. The high temperature scale of the normal-state gap raises the prospect of engineering higher transition temperatures in the n-type cuprates comparable to those of the p-type cuprates.
In the underdoped n-type cuprate Nd Ce CuO , long-range antiferromagnetic order reconstructs the Fermi surface, resulting in a putative antiferromagnetic metal with small Fermi pockets. Using angle-resolved photoemission spectroscopy, we observe an anomalous energy gap, an order of magnitude smaller than the antiferromagnetic gap, in a wide portion of the underdoped regime and smoothly connecting to the superconducting gap at optimal doping. After considering all the known ordering tendencies in tandem with the phase diagram, we hypothesize that the normal-state gap in the underdoped n-type cuprates originates from Cooper pairing. The high temperature scale of the normal-state gap raises the prospect of engineering higher transition temperatures in the n-type cuprates comparable to those of the p-type cuprates.
In the underdoped n-type cuprate Nd 2- x Ce x CuO 4 , long-range antiferromagnetic order reconstructs the Fermi surface, resulting in a putative antiferromagnetic metal with small Fermi pockets. Using angle-resolved photoemission spectroscopy, we observe an anomalous energy gap, an order of magnitude smaller than the antiferromagnetic gap, in a wide portion of the underdoped regime and smoothly connecting to the superconducting gap at optimal doping. After considering all the known ordering tendencies in tandem with the phase diagram, we hypothesize that the normal-state gap in the underdoped n-type cuprates originates from Cooper pairing. The high temperature scale of the normal-state gap raises the prospect of engineering higher transition temperatures in the n-type cuprates comparable to those of the p-type cuprates.
In the underdoped n-type cuprate Nd 2-x Ce x CuO 4 , long-range antiferromagnetic order reconstructs the Fermi surface, resulting in a putative antiferromagnetic metal with small Fermi pockets. Using angle-resolved photoemission spectroscopy, we observe an anomalous energy gap, an order of magnitude smaller than the antiferromagnetic gap, in a wide portion of the underdoped regime and smoothly connecting to the superconducting gap at optimal doping. After considering all the known ordering tendencies in tandem with the phase diagram, we hypothesize that the normal-state gap in the underdoped n-type cuprates originates from Cooper pairing. The high temperature scale of the normal-state gap raises the prospect of engineering higher transition temperatures in the n-type cuprates comparable to those of the p-type cuprates.
Author Xu, Ke-Jun
Abadi, Sebastien N
Hashimoto, Makoto
Tjernberg, Oscar
Guo, Qinda
Chen, Su-Di
He, Junfeng
He, Yu
Lee, Dung-Hai
Devereaux, Thomas P
Shen, Zhi-Xun
Lee, Young S
Lu, Dong-Hui
Rotundu, Costel R
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  organization: Department of Physics and CAS Key Laboratory of Strongly-coupled Quantum Matter Physics, University of Science and Technology of China, Hefei, Anhui 230026, China
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  givenname: Su-Di
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  givenname: Dong-Hui
  orcidid: 0000-0002-9708-0443
  surname: Lu
  fullname: Lu, Dong-Hui
  organization: Stanford Synchrotron Radiation Lightsource, SLAC National Accelerator Laboratory, 2575 Sand Hill Road, Menlo Park, CA 94025, USA
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  orcidid: 0000-0003-0585-4331
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  organization: Department of Applied Physics, KTH Royal Institute of Technology, Hannes Alfvéns väg 12, 114 19 Stockholm, Sweden
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  surname: Tjernberg
  fullname: Tjernberg, Oscar
  organization: Department of Applied Physics, KTH Royal Institute of Technology, Hannes Alfvéns väg 12, 114 19 Stockholm, Sweden
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  givenname: Thomas P
  orcidid: 0000-0001-8072-9237
  surname: Devereaux
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  orcidid: 0000-0002-1454-0281
  surname: Shen
  fullname: Shen, Zhi-Xun
  organization: Department of Physics, Stanford University, Stanford, CA 94305, USA
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Snippet In the underdoped n-type cuprate Nd Ce CuO , long-range antiferromagnetic order reconstructs the Fermi surface, resulting in a putative antiferromagnetic metal...
Editor’s summaryCopper oxide materials can be made superconducting by doping the parent compound with either electrons or holes. Hole-doped cuprates typically...
In the underdoped n-type cuprate Nd2-xCexCuO4, long-range antiferromagnetic order reconstructs the Fermi surface, resulting in a putative antiferromagnetic...
In the underdoped n-type cuprate Nd 2- x Ce x CuO 4 , long-range antiferromagnetic order reconstructs the Fermi surface, resulting in a putative...
In the underdoped n-type cuprate Nd 2-x Ce x CuO 4 , long-range antiferromagnetic order reconstructs the Fermi surface, resulting in a putative...
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SubjectTerms CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY
Copper oxides
Cuprates
Electrons
Energy gap
Phase diagrams
Photoelectric emission
Superconductivity
Transition temperatures
Title Anomalous normal-state gap in an electron-doped cuprate
URI https://www.ncbi.nlm.nih.gov/pubmed/39146411
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