Implanting Numerous Hydrogen‐Bonding Networks in a Cu‐Porphyrin‐Based Nanosheet to Boost CH4 Selectivity in Neutral‐Media CO2 Electroreduction

• Published in: Angewandte Chemie International Edition Vol. 60; no. 40; pp. 21952 - 21958
• Main Authors: Wang, Yi‐Rong, Liu, Ming, Gao, Guang‐Kuo, Yang, Yi‐Lu, Yang, Ru‐Xin, Ding, Hui‐Min, Chen, Yifa, Li, Shun‐Li, Lan, Ya‐Qian
• Format: Journal Article
• Language: English
• Published: Weinheim Wiley Subscription Services, Inc 27.09.2021
• Edition: International ed. in English
• Subjects: Bonding; Carbon dioxide; Catalysts; Chemical reduction; Electrocatalysts; Electrochemistry; electroreduction; Hydrogen; Hydrogen bonding; hydrogen bonds; Methane; Nanosheets; Porphyrins; Protons; Selectivity

The exploration of novel systems for the electrochemical CO2 reduction reaction (CO2RR) for the production of hydrocarbons like CH4 remains a giant challenge. Well‐designed electrocatalysts with advantages like proton generation/transferring and intermediate‐fixating for efficient CO2RR are much pre...