Visualizing the formation of the Kondo lattice and the hidden order in URu2Si2

Heavy electronic states originating from the f atomic orbitals underlie a rich variety of quantum phases of matter. We use atomic scale imaging and spectroscopy with the scanning tunneling microscope to examine the novel electronic states that emerge from the uranium f states in URu 2 Si 2 . We find...

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Published inProceedings of the National Academy of Sciences - PNAS Vol. 107; no. 23; pp. 10383 - 10388
Main Authors Aynajian, Pegor, da Silva Neto, Eduardo H., Parker, Colin V., Huang, Yingkai, Pasupathy, Abhay, Mydosh, John, Yazdani, Ali
Format Journal Article
LanguageEnglish
Published National Acad Sciences 08.06.2010
National Academy of Sciences
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Abstract Heavy electronic states originating from the f atomic orbitals underlie a rich variety of quantum phases of matter. We use atomic scale imaging and spectroscopy with the scanning tunneling microscope to examine the novel electronic states that emerge from the uranium f states in URu 2 Si 2 . We find that, as the temperature is lowered, partial screening of the f electrons’ spins gives rise to a spatially modulated Kondo–Fano resonance that is maximal between the surface U atoms. At T  = 17.5 K, URu 2 Si 2 is known to undergo a second-order phase transition from the Kondo lattice state into a phase with a hidden order parameter. From tunneling spectroscopy, we identify a spatially modulated, bias-asymmetric energy gap with a mean-field temperature dependence that develops in the hidden order state. Spectroscopic imaging further reveals a spatial correlation between the hidden order gap and the Kondo resonance, suggesting that the two phenomena involve the same electronic states.
AbstractList Heavy electronic states originating from the f atomic orbitals underlie a rich variety of quantum phases of matter. We use atomic scale imaging and spectroscopy with the scanning tunneling microscope to examine the novel electronic states that emerge from the uranium f states in URu 2 Si 2 . We find that, as the temperature is lowered, partial screening of the f electrons’ spins gives rise to a spatially modulated Kondo–Fano resonance that is maximal between the surface U atoms. At T  = 17.5 K, URu 2 Si 2 is known to undergo a second-order phase transition from the Kondo lattice state into a phase with a hidden order parameter. From tunneling spectroscopy, we identify a spatially modulated, bias-asymmetric energy gap with a mean-field temperature dependence that develops in the hidden order state. Spectroscopic imaging further reveals a spatial correlation between the hidden order gap and the Kondo resonance, suggesting that the two phenomena involve the same electronic states.
Heavy electronic states originating from the f atomic orbitals underlie a rich variety of quantum phases of matter. We use atomic scale imaging and spectroscopy with the scanning tunneling microscope to examine the novel electronic states that emerge from the uranium f states in URu 2 Si 2 . We find that, as the temperature is lowered, partial screening of the f electrons’ spins gives rise to a spatially modulated Kondo–Fano resonance that is maximal between the surface U atoms. At T  = 17.5 K, URu 2 Si 2 is known to undergo a second-order phase transition from the Kondo lattice state into a phase with a hidden order parameter. From tunneling spectroscopy, we identify a spatially modulated, bias-asymmetric energy gap with a mean-field temperature dependence that develops in the hidden order state. Spectroscopic imaging further reveals a spatial correlation between the hidden order gap and the Kondo resonance, suggesting that the two phenomena involve the same electronic states.
Author Pegor Aynajian
Eduardo H. da Silva Neto
Ali Yazdani
John Mydosh
Yingkai Huang
Colin V. Parker
Abhay Pasupathy
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  email: yazdani@princeton.edu
  organization: Joseph Henry Laboratories and Department of Physics, Princeton University, Princeton, NJ 08544
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Notes Communicated by Philip W. Anderson, Princeton University, Princeton, NJ, April 28, 2010 (received for review March 26, 2010)
1P.A., E.H.d.S.N., and C.V.P. contributed equally to this work.
Author contributions: A.P. and A.Y. designed research; P.A., E.H.d.S.N., C.V.P., Y.H., and J.M. performed research; Y.H. and J.M. contributed new reagents/analytic tools; P.A., E.H.d.S.N., and C.V.P. analyzed data; and P.A., E.H.d.S.N., C.V.P., A.P., J.M., and A.Y. wrote the paper.
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Snippet Heavy electronic states originating from the f atomic orbitals underlie a rich variety of quantum phases of matter. We use atomic scale imaging and...
Heavy electronic states originating from the f atomic orbitals underlie a rich variety of quantum phases of matter. We use atomic scale imaging and...
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SubjectTerms Physical Sciences
Title Visualizing the formation of the Kondo lattice and the hidden order in URu2Si2
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