横浜市磯子区における殺虫剤の大気から水への移動量に係る検討について
Dichlorvos and fenitrothion were detected frequently in rainwater collected at Yokohama Environmental Science Research Institute located in the Isogo ward of Yokohama in 2001 and 2002. Further, some rainwater samples in 2003 had a lethal effect on Daphnia magna after adding minerals. Thus, toxic pot...
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Published in | Journal of environmental chemistry Vol. 27; no. 3; pp. 63 - 67 |
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Main Authors | , , |
Format | Journal Article |
Language | Japanese |
Published |
Tsukuba
一般社団法人 日本環境化学会
01.01.2017
Japan Science and Technology Agency |
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Abstract | Dichlorvos and fenitrothion were detected frequently in rainwater collected at Yokohama Environmental Science Research Institute located in the Isogo ward of Yokohama in 2001 and 2002. Further, some rainwater samples in 2003 had a lethal effect on Daphnia magna after adding minerals. Thus, toxic potency of insecticide in rainwater (wet deposition) was considered to be an important problem for environmental protection. However, there were few studies on the atmospheric dry deposition of organophosphorous insecticides in Japan. Therefore, atmospheric deposition of dichlorvos and fenitrothion were determined by gas chromatograph mass spectrometer (GC/MS). Average atmospheric deposition amount of dichlorvos was 7.0 ng/m2/hr and that of fenitrothion was 6.3 ng/m2/hr. The highest concentration of insecticides in the aqueous solution exposed to air overnight was less than 0.05 μg/L, although the concentraions of dichlorvos and fenitrothion in rainwater sampled on October 1st, 2014 were more than 0.10. μg/L. The toxic potency of insecticides in aqueous solution exposed to air overnight might be less than that in rainwater sampled on October 1st, 2014. However, the concentrations of dichlorvos and fenitrothion in the solution exposed to air overnight were not less than PNEC (predicted no-effect of concentration). Therefore the atmospheric deposition of insecticides was considered to be one of important ecological problems for environmental protection as well as wet deposition of them. |
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AbstractList | Dichlorvos and fenitrothion were detected frequently in rainwater collected at Yokohama Environmental Science Research Institute located in the Isogo ward of Yokohama in 2001 and 2002. Further, some rainwater samples in 2003 had a lethal effect on Daphnia magna after adding minerals. Thus, toxic potency of insecticide in rainwater (wet deposition) was considered to be an important problem for environmental protection. However, there were few studies on the atmospheric dry deposition of organophosphorous insecticides in Japan. Therefore, atmospheric deposition of dichlorvos and fenitrothion were determined by gas chromatograph mass spectrometer (GC/MS). Average atmospheric deposition amount of dichlorvos was 7.0 ng/m2/hr and that of fenitrothion was 6.3 ng/m2/hr. The highest concentration of insecticides in the aqueous solution exposed to air overnight was less than 0.05 μg/L, although the concentraions of dichlorvos and fenitrothion in rainwater sampled on October 1st, 2014 were more than 0.10. μg/L. The toxic potency of insecticides in aqueous solution exposed to air overnight might be less than that in rainwater sampled on October 1st, 2014. However, the concentrations of dichlorvos and fenitrothion in the solution exposed to air overnight were not less than PNEC (predicted no-effect of concentration). Therefore the atmospheric deposition of insecticides was considered to be one of important ecological problems for environmental protection as well as wet deposition of them. |
Author | 小神野, 豊 酒井, 学 多田, 満 |
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References | 16) Kikuchi, M., Sasaki, Y., and Wakabayashi, M.: Screening of Organophosphorous insecticide pollution in water by using Daphnia magna. Ecotoxicology Environmental Safety, 47, 239-245 (2000 6) 酒井, 学:横浜市(磯子区)における大気中の有機リン系農薬調査,横浜市環境科学研究所報,28,70-71(2004) 4) Suzuki, S., Otani, T., Iwasaki, S., Ito, K., Omura, H. and Tanaka, Y.: Monitoring of 15 pesticides in rainwater in Utunomiya, eastern Japan, 1999-2000. J. Pesticide Sci., 28, 1-7 (2003 19) 経済産業省・環境省:PRTR排出量算出マニュアル第4.1版(2011) 18) Majewski, M.S., Zamora,C., Foreman, W.T. and Kratzer, C.R.: Contribution of atmospheric deposition to pesticide loads in surface water runoff. Open file report( https://pubs.usgs.gov/of/2005/1307/ofr2005_1307.pdf)(アクセス2017/04/12) 7) 鈴木 茂,張山嘉道,緒方行治:川崎市内の大気中農薬の一斉分析調査,川崎市公害研年報,20,7-14(1994) 1) Sakai, M.: Investigation of pesticides in rainwater at Isogo Ward of Yokohama. J. Health Sci., 49, 221-225 (2003 11) Waite, D.T., Sproull, J.F., Quiring, D.V. and Cessna, A.J.: Dry atmospheric deposition and deposition velocities of dicamba, 2,4-dichlorophenoxyacetic acid and γ-1,2,3,4,5,6- hexachlorocyclohexane. Anal Chim Acta, 467, 245-252 (2002 2) Sakai, M.: Acute toxic tests of rainwater samples using Daphnia magna. Ecotoxicology Environmental Safety, 64, 215-220 (2006 3) Kawata, K., Muraki, H., Tanabe, H. and Yasuhara, A.: Annual variation of insecticides in precipitation in rural Japan. Bull. Environ. Contam. Toxicol., 57, 853-858 (1996 12) 気象庁:過去の気象データ 神奈川県横浜(http://www.data. jma.go.jp/obd/stats/etrn/index.php?prec_no=46&block_no=476 70&year=&month=&day=&view=)(アクセス2017/04/12) 17) 環境省環境保健部環境安全課:化学物質ファクトシート2012年版(2012) 14) 環境省環境保健部環境リスク評価室:化学物質の環境リスク評価第2巻(2003) 5) 酒井, 学:横浜市(磯子区)における殺虫剤,殺菌剤,除草剤 の湿性沈着について, 横浜市環境化学研究所報,29,137-139 (2005) 8) 斎藤育江,大貫 文,瀬戸 博,上原真一:有機リン系殺虫剤の室内および外気濃度測定,大気環境学会誌,38,78-88(2003) 9) 環境省環境保健部環境安全課:平成27年度版化学物質と環境 (2016) 13) 神奈川県環境科学センター:かながわのPRTR(http://www. k-erc.pref.kanagawa.jp/prtr/H27data/hyouji6.asp)(アクセス 2017/04/12) 10) 環境省環境保健部環境安全課:化学物質環境実態調査の手引き(平成27年度版)(2016) 15) 環境省環境保健部環境安全課:化学物質と環境 平成22年度化学物質分析法開発調査報告書,371-388(2011) |
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SubjectTerms | Aqueous solutions Atmospheric pollution deposition Deposition Dichlorvos Dry deposition Environmental protection Environmental science Exposure Fenitrothion Gas chromatography Insecticides Minerals Pesticides Rain water Surface water Wet deposition |
Title | 横浜市磯子区における殺虫剤の大気から水への移動量に係る検討について |
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