Rapid Charge Transport in Dye-Sensitized Solar Cells Made from Vertically Aligned Single-Crystal Rutile TiO2 Nanowires
A rapid solvothermal approach was used to synthesize aligned 1D single‐crystal rutile TiO2 nanowire (NW) arrays on transparent conducting substrates as electrodes for dye‐sensitized solar cells. The NW arrays showed a more than 200 times faster charge transport (see picture) and a factor four lower...
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| Published in | Angewandte Chemie (International ed.) Vol. 51; no. 11; pp. 2727 - 2730 |
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| Main Authors | , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Weinheim
WILEY-VCH Verlag
12.03.2012
WILEY‐VCH Verlag Wiley Subscription Services, Inc |
| Edition | International ed. in English |
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| Abstract | A rapid solvothermal approach was used to synthesize aligned 1D single‐crystal rutile TiO2 nanowire (NW) arrays on transparent conducting substrates as electrodes for dye‐sensitized solar cells. The NW arrays showed a more than 200 times faster charge transport (see picture) and a factor four lower defect state density than conventional rutile nanoparticle films. |
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| AbstractList | A rapid solvothermal approach was used to synthesize aligned 1D single‐crystal rutile TiO2 nanowire (NW) arrays on transparent conducting substrates as electrodes for dye‐sensitized solar cells. The NW arrays showed a more than 200 times faster charge transport (see picture) and a factor four lower defect state density than conventional rutile nanoparticle films. A rapid solvothermal approach was used to synthesize aligned 1D single-crystal rutile TiO(2) nanowire (NW) arrays on transparent conducting substrates as electrodes for dye-sensitized solar cells. The NW arrays showed a more than 200 times faster charge transport and a factor four lower defect state density than conventional rutile nanoparticle films. |
| Author | Mallouk, Thomas E. Feng, Xinjian Grimes, Craig A. Zhu, Kai Frank, Arthur J. |
| Author_xml | – sequence: 1 givenname: Xinjian surname: Feng fullname: Feng, Xinjian organization: Department of Chemistry, Materials Research Institute, The Pennsylvania State University, University Park, PA 16802 (USA) – sequence: 2 givenname: Kai surname: Zhu fullname: Zhu, Kai organization: National Renewable Energy Laboratory, 1617 Cole Boulevard, Golden, CO 80401 (USA) – sequence: 3 givenname: Arthur J. surname: Frank fullname: Frank, Arthur J. organization: National Renewable Energy Laboratory, 1617 Cole Boulevard, Golden, CO 80401 (USA) – sequence: 4 givenname: Craig A. surname: Grimes fullname: Grimes, Craig A. organization: Department of Chemistry, Materials Research Institute, The Pennsylvania State University, University Park, PA 16802 (USA) – sequence: 5 givenname: Thomas E. surname: Mallouk fullname: Mallouk, Thomas E. email: tem5@psu.edu organization: Department of Chemistry, Materials Research Institute, The Pennsylvania State University, University Park, PA 16802 (USA) |
| BackLink | https://www.osti.gov/biblio/1044466$$D View this record in Osti.gov |
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| Copyright | Copyright © 2012 WILEY‐VCH Verlag GmbH & Co. KGaA, Weinheim Copyright © 2012 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim |
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| Notes | ark:/67375/WNG-8DN85JG9-W National Science Foundation - No. ECS-0335765 ArticleID:ANIE201108076 Work at Penn State was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences under grant number DE-SC0001087. Work at NREL was supported by the U.S. Department of Energy, under grant number DEAC36-08GO28308. The Penn State Nanofabrication facility is supported by the National Science Foundation under grant number ECS-0335765. We would like to thank Dr. Bangzhi Liu at the Penn State Nanofabrication facility for his help with FE-SEM, TEM, and HR-TEM analyses. U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences - No. DE-SC0001087; No. DEAC36-08GO28308 istex:9585837FA50DA6259D0935343BA5EB23C6B6A7D0 These authors contributed equally to this work. Work at Penn State was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences under grant number DE‐SC0001087. Work at NREL was supported by the U.S. Department of Energy, under grant number DEAC36‐08GO28308. The Penn State Nanofabrication facility is supported by the National Science Foundation under grant number ECS‐0335765. We would like to thank Dr. Bangzhi Liu at the Penn State Nanofabrication facility for his help with FE‐SEM, TEM, and HR‐TEM analyses. USDOE Office of Science, Basic Energy Sciences USDOE Office of Energy Efficiency and Renewable Energy Solar Energy Technologies Program AC36-08GO28308 NREL/JA-5900-54984 |
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| Snippet | A rapid solvothermal approach was used to synthesize aligned 1D single‐crystal rutile TiO2 nanowire (NW) arrays on transparent conducting substrates as... A rapid solvothermal approach was used to synthesize aligned 1D single-crystal rutile TiO(2) nanowire (NW) arrays on transparent conducting substrates as... A rapid solvothermal approach was used to synthesize aligned 1D single-crystal rutile TiO2 nanowire (NW) arrays on transparent conducting substrates as... |
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| SubjectTerms | CHARGE TRANSPORT DEFECTS DIFFUSION diffusion coefficients ELECTRODES MATERIALS SCIENCE metal oxides nanoparticles nanowires OXIDES RUTILE SOLAR CELLS SOLAR ENERGY SUBSTRATES |
| Title | Rapid Charge Transport in Dye-Sensitized Solar Cells Made from Vertically Aligned Single-Crystal Rutile TiO2 Nanowires |
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