CO2-"Neutral" Hydrogen Storage Based on Bicarbonates and Formates

Let the circle be unbroken! One ruthenium catalyst generated in situ facilitates the selective hydrogenation of bicarbonates and carbonates, as well as CO2 and base, to give formates and also the selective dehydrogenation of formates back to bicarbonates. The two reactions can be coupled, leading to...

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Published inAngewandte Chemie International Edition Vol. 50; no. 28; pp. 6411 - 6414
Main Authors Boddien, Albert, Gärtner, Felix, Federsel, Christopher, Sponholz, Peter, Mellmann, Dörthe, Jackstell, Ralf, Junge, Henrik, Beller, Matthias
Format Journal Article
LanguageEnglish
Published Weinheim WILEY-VCH Verlag 04.07.2011
WILEY‐VCH Verlag
Wiley Subscription Services, Inc
EditionInternational ed. in English
Subjects
bicarbonates
formates
homogeneous catalysis
hydrogen storage
ruthenium
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Abstract Let the circle be unbroken! One ruthenium catalyst generated in situ facilitates the selective hydrogenation of bicarbonates and carbonates, as well as CO2 and base, to give formates and also the selective dehydrogenation of formates back to bicarbonates. The two reactions can be coupled, leading to a reversible hydrogen‐storage system. dppm=1,2‐bis(diphenylphosphino)methane.
AbstractList Let the circle be unbroken! One ruthenium catalyst generated in situ facilitates the selective hydrogenation of bicarbonates and carbonates, as well as CO2 and base, to give formates and also the selective dehydrogenation of formates back to bicarbonates. The two reactions can be coupled, leading to a reversible hydrogen‐storage system. dppm=1,2‐bis(diphenylphosphino)methane.
Author Gärtner, Felix
Beller, Matthias
Jackstell, Ralf
Sponholz, Peter
Junge, Henrik
Boddien, Albert
Federsel, Christopher
Mellmann, Dörthe
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Notes This work was supported by the BMBF (Spitzenforschung und Innovation in den neuen Ländern). F.G. thanks the Fonds der Chemischen Industrie (FCI) for a Kekulé grant. We thank Prof. G. Laurenczy (EPFL) for fruitful discussions.
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Snippet Let the circle be unbroken! One ruthenium catalyst generated in situ facilitates the selective hydrogenation of bicarbonates and carbonates, as well as CO2 and...
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SubjectTerms bicarbonates
formates
homogeneous catalysis
hydrogen storage
ruthenium
Title CO2-"Neutral" Hydrogen Storage Based on Bicarbonates and Formates
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