Porous Carbon Membrane‐Supported Atomically Dispersed Pyrrole‐Type FeN4 as Active Sites for Electrochemical Hydrazine Oxidation Reaction
The rational design of catalytically active sites in porous materials is essential in electrocatalysis. Herein, atomically dispersed Fe‐Nx sites supported by hierarchically porous carbon membranes are designed to electrocatalyze the hydrazine oxidation reaction (HzOR), one of the key techniques in e...
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| Published in | Small (Weinheim an der Bergstrasse, Germany) Vol. 16; no. 31; pp. e2002203 - n/a |
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| Abstract | The rational design of catalytically active sites in porous materials is essential in electrocatalysis. Herein, atomically dispersed Fe‐Nx sites supported by hierarchically porous carbon membranes are designed to electrocatalyze the hydrazine oxidation reaction (HzOR), one of the key techniques in electrochemical nitrogen transformation. The high intrinsic catalytic activity of the Fe‐Nx single‐atom catalyst together with the uniquely mixed micro‐/macroporous membrane support positions such an electrode among the best‐known heteroatom‐based carbon anodes for hydrazine fuel cells. Combined with advanced characterization techniques, electrochemical probe experiments, and density functional theory calculation, the pyrrole‐type FeN4 structure is identified as the real catalytic site in HzOR.
Hierarchically porous carbon membrane‐supported atomically dispersed pyrrole‐type FeN4 sites are proposed and verified as real active sites for the hydrazine oxidation reaction. |
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| AbstractList | The rational design of catalytically active sites in porous materials is essential in electrocatalysis. Herein, atomically dispersed Fe-Nx sites supported by hierarchically porous carbon membranes are designed to electrocatalyze the hydrazine oxidation reaction (HzOR), one of the key techniques in electrochemical nitrogen transformation. The high intrinsic catalytic activity of the Fe-Nx single-atom catalyst together with the uniquely mixed micro-/macroporous membrane support positions such an electrode among the best-known heteroatom-based carbon anodes for hydrazine fuel cells. Combined with advanced characterization techniques, electrochemical probe experiments, and density functional theory calculation, the pyrrole-type FeN4 structure is identified as the real catalytic site in HzOR.The rational design of catalytically active sites in porous materials is essential in electrocatalysis. Herein, atomically dispersed Fe-Nx sites supported by hierarchically porous carbon membranes are designed to electrocatalyze the hydrazine oxidation reaction (HzOR), one of the key techniques in electrochemical nitrogen transformation. The high intrinsic catalytic activity of the Fe-Nx single-atom catalyst together with the uniquely mixed micro-/macroporous membrane support positions such an electrode among the best-known heteroatom-based carbon anodes for hydrazine fuel cells. Combined with advanced characterization techniques, electrochemical probe experiments, and density functional theory calculation, the pyrrole-type FeN4 structure is identified as the real catalytic site in HzOR. The rational design of catalytically active sites in porous materials is essential in electrocatalysis. Herein, atomically dispersed Fe‐Nx sites supported by hierarchically porous carbon membranes are designed to electrocatalyze the hydrazine oxidation reaction (HzOR), one of the key techniques in electrochemical nitrogen transformation. The high intrinsic catalytic activity of the Fe‐Nx single‐atom catalyst together with the uniquely mixed micro‐/macroporous membrane support positions such an electrode among the best‐known heteroatom‐based carbon anodes for hydrazine fuel cells. Combined with advanced characterization techniques, electrochemical probe experiments, and density functional theory calculation, the pyrrole‐type FeN4 structure is identified as the real catalytic site in HzOR. The rational design of catalytically active sites in porous materials is essential in electrocatalysis. Herein, atomically dispersed Fe‐Nx sites supported by hierarchically porous carbon membranes are designed to electrocatalyze the hydrazine oxidation reaction (HzOR), one of the key techniques in electrochemical nitrogen transformation. The high intrinsic catalytic activity of the Fe‐Nx single‐atom catalyst together with the uniquely mixed micro‐/macroporous membrane support positions such an electrode among the best‐known heteroatom‐based carbon anodes for hydrazine fuel cells. Combined with advanced characterization techniques, electrochemical probe experiments, and density functional theory calculation, the pyrrole‐type FeN4 structure is identified as the real catalytic site in HzOR. Hierarchically porous carbon membrane‐supported atomically dispersed pyrrole‐type FeN4 sites are proposed and verified as real active sites for the hydrazine oxidation reaction. |
| Author | Zhang, Miao Wang, Yue‐Sheng Sheng, Tian Zhou, Zhi‐You Cui, Pei‐Xin Yuan, Jiayin Liang, Hai‐Wei Tong, Lei Zaghib, Karim Wang, Yu‐Cheng Wang, Hong Ke, Yu‐Qi Sun, Shu‐Hui Wan, Li‐Yang |
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| Snippet | The rational design of catalytically active sites in porous materials is essential in electrocatalysis. Herein, atomically dispersed Fe‐Nx sites supported by... The rational design of catalytically active sites in porous materials is essential in electrocatalysis. Herein, atomically dispersed Fe-Nx sites supported by... |
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| SubjectTerms | Carbon Catalytic activity Density functional theory Dispersion Electrochemical analysis FeN4 active sites Fuel cells hydrazine oxidation Hydrazines Membranes Nanotechnology Oxidation porous carbon membranes Porous materials single atom catalysts |
| Title | Porous Carbon Membrane‐Supported Atomically Dispersed Pyrrole‐Type FeN4 as Active Sites for Electrochemical Hydrazine Oxidation Reaction |
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