Enhanced Water-Splitting Performance of Perovskite SrTaO2N Photoanode Film through Ameliorating Interparticle Charge Transport
Here SrTaO2N has been found to exhibit photoelectrochemical water splitting, with a theoretical solar‐to‐hydrogen efficiency of 14.4%. Ameliorating the interparticle charge transport by H2 annealing, the solar photocurrent of the SrTaO2N(H) granular film at 1.23 V versus reversible hydrogen electrod...
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| Published in | Advanced functional materials Vol. 26; no. 39; pp. 7156 - 7163 |
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| Main Authors | , , , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Blackwell Publishing Ltd
18.10.2016
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| Subjects | |
| Online Access | Get full text |
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| Abstract | Here SrTaO2N has been found to exhibit photoelectrochemical water splitting, with a theoretical solar‐to‐hydrogen efficiency of 14.4%. Ameliorating the interparticle charge transport by H2 annealing, the solar photocurrent of the SrTaO2N(H) granular film at 1.23 V versus reversible hydrogen electrode (RHE) is increased by ≈250% in comparison with the SrTaO2N film. Using an aberration corrected scanning transmission electron microscope and super‐X energy dispersive spectroscopy, the atomic scale observation has proved a decrease of oxygen concentrations in the surface of SrTaO2N(H) particle, which may allow its electrical conductivity to be increased from 0.77 × 10−6 to 2.65 × 10−6 S cm−1 and therefore the charge separation efficiency has been greatly increased by ≈330%. After being modified by Co–Pi water oxidation catalyst, the SrTaO2N(H) photoanode shows a solar photocurrent of 1.1 mA cm−2 and an incident photo‐to‐current efficiency value of ≈20% at 400–460 nm and 1.23 V versus RHE, which suggests that it is a new promising photoanode material for solar water splitting.
SrTaO2N is found to be a new promising photoanode for photoelectrochemical water splitting. The atomic scale observation proves a decrease of oxygen concentrations in the surface of SrTaO2N(H) particle after H2 annealing, which may improve its bulk electrical conductivity and the charge separation efficiency. Consequently, the photoelectrochemical performance of SrTaO2N(H) granular film is enhanced remarkably. |
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| AbstractList | Here SrTaO2N has been found to exhibit photoelectrochemical water splitting, with a theoretical solar‐to‐hydrogen efficiency of 14.4%. Ameliorating the interparticle charge transport by H2 annealing, the solar photocurrent of the SrTaO2N(H) granular film at 1.23 V versus reversible hydrogen electrode (RHE) is increased by ≈250% in comparison with the SrTaO2N film. Using an aberration corrected scanning transmission electron microscope and super‐X energy dispersive spectroscopy, the atomic scale observation has proved a decrease of oxygen concentrations in the surface of SrTaO2N(H) particle, which may allow its electrical conductivity to be increased from 0.77 × 10−6 to 2.65 × 10−6 S cm−1 and therefore the charge separation efficiency has been greatly increased by ≈330%. After being modified by Co–Pi water oxidation catalyst, the SrTaO2N(H) photoanode shows a solar photocurrent of 1.1 mA cm−2 and an incident photo‐to‐current efficiency value of ≈20% at 400–460 nm and 1.23 V versus RHE, which suggests that it is a new promising photoanode material for solar water splitting.
SrTaO2N is found to be a new promising photoanode for photoelectrochemical water splitting. The atomic scale observation proves a decrease of oxygen concentrations in the surface of SrTaO2N(H) particle after H2 annealing, which may improve its bulk electrical conductivity and the charge separation efficiency. Consequently, the photoelectrochemical performance of SrTaO2N(H) granular film is enhanced remarkably. |
| Author | Qian, Qinfeng Wang, Peng Zhao, Xin Yan, Shicheng Li, Zhaosheng Huang, Huiting Chang, Xiaofeng Yu, Zhentao Zou, Zhigang Zhong, Yujiao Fang, Tao |
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| Notes | ArticleID:ADFM201603021 istex:33DB1CBB8FB6F41861480A24BF8E80390DE308AB ark:/67375/WNG-M6H5QGT3-W International Science & Technology Cooperation Program of China - No. 2014DFE00200 National Natural Science Foundation of China - No. 51272102; No. 21473090 National Natural Science Foundation of China - No. 11474147 973 Program - No. 2015CB654900 973 Program - No. 2013CB632404 Natural Science Foundation of Jiangsu Province - No. BK20151383 |
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| PublicationTitle | Advanced functional materials |
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| Snippet | Here SrTaO2N has been found to exhibit photoelectrochemical water splitting, with a theoretical solar‐to‐hydrogen efficiency of 14.4%. Ameliorating the... |
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| SubjectTerms | charge separation efficiency interparticle charge transport photoanodes solar water splitting SrTaO2N |
| Title | Enhanced Water-Splitting Performance of Perovskite SrTaO2N Photoanode Film through Ameliorating Interparticle Charge Transport |
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