Flue gas treatment with ozone oxidation: An overview on NOx, organic pollutants, and mercury
[Display omitted] •Ozone oxidation coupled with post-absorption is firstly reviewed for flue gas treatment.•Simultaneous removal of NOx, SO2, VOCs, and mercury can be achieved by this technology.•Solubility increase and bond breaking are basic principles for pollutants removal by ozone.•This technol...
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| Published in | Chemical engineering journal (Lausanne, Switzerland : 1996) Vol. 382 |
|---|---|
| Main Authors | , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Elsevier B.V
15.02.2020
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| Subjects | |
| Online Access | Get full text |
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| Abstract | [Display omitted]
•Ozone oxidation coupled with post-absorption is firstly reviewed for flue gas treatment.•Simultaneous removal of NOx, SO2, VOCs, and mercury can be achieved by this technology.•Solubility increase and bond breaking are basic principles for pollutants removal by ozone.•This technology is potential to attain ultra-low emission for industrial boiler and furnaces.
Traditional flue gas pollutants treatment technologies are installed with their individual function. Industries usually make simple combination and increase operation load of equipment to face with the increasing stringent environmental stress and emission standard. Especially, these technique routes are not available to industrial boilers and furnaces because of specific conditions, such as unsuitable temperature window, complicated components in flue gas, and flexible operation. Simultaneous removal of multi-pollutants within one or two devices is a prospective direction that can save space occupation and cost. Interestingly, the solubility of NOx and mercury increases with its valance state, and organic pollutants can be degraded into nontoxic small molecules by oxidation. Ozone is a strong gas phase oxidant that can achieve pre-oxidation at low temperature, following by post-absorption to completely remove oxidized products. This review focuses on research progress involved in homogeneous and heterogeneous catalytic oxidation of NOx, organic pollutants, and mercury by ozone, as well as NOx absorption regarding of its full path removal. The reaction mechanism, kinetics, operation parameters, conversion efficiency and ozone residual are all summarized in detail. This paper also systematically reviews various approaches in catalytic ozonation towards improving catalytic activity, selectivity, and stability, as well as lowering temperature, such as active metals, metal loading contents, supports, precursors, and other modification. Finally, the overall technique route of simultaneous removal of multi-pollutants by ozone is analyzed. In conclusion, the ozone oxidation technology is advantaged in flue gas pollutants treatment, including low temperature, no massive adjustment in operation and original devices, saving space, no secondary pollution, N/S sources recovery, and potential to ultra-low emission. |
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| AbstractList | [Display omitted]
•Ozone oxidation coupled with post-absorption is firstly reviewed for flue gas treatment.•Simultaneous removal of NOx, SO2, VOCs, and mercury can be achieved by this technology.•Solubility increase and bond breaking are basic principles for pollutants removal by ozone.•This technology is potential to attain ultra-low emission for industrial boiler and furnaces.
Traditional flue gas pollutants treatment technologies are installed with their individual function. Industries usually make simple combination and increase operation load of equipment to face with the increasing stringent environmental stress and emission standard. Especially, these technique routes are not available to industrial boilers and furnaces because of specific conditions, such as unsuitable temperature window, complicated components in flue gas, and flexible operation. Simultaneous removal of multi-pollutants within one or two devices is a prospective direction that can save space occupation and cost. Interestingly, the solubility of NOx and mercury increases with its valance state, and organic pollutants can be degraded into nontoxic small molecules by oxidation. Ozone is a strong gas phase oxidant that can achieve pre-oxidation at low temperature, following by post-absorption to completely remove oxidized products. This review focuses on research progress involved in homogeneous and heterogeneous catalytic oxidation of NOx, organic pollutants, and mercury by ozone, as well as NOx absorption regarding of its full path removal. The reaction mechanism, kinetics, operation parameters, conversion efficiency and ozone residual are all summarized in detail. This paper also systematically reviews various approaches in catalytic ozonation towards improving catalytic activity, selectivity, and stability, as well as lowering temperature, such as active metals, metal loading contents, supports, precursors, and other modification. Finally, the overall technique route of simultaneous removal of multi-pollutants by ozone is analyzed. In conclusion, the ozone oxidation technology is advantaged in flue gas pollutants treatment, including low temperature, no massive adjustment in operation and original devices, saving space, no secondary pollution, N/S sources recovery, and potential to ultra-low emission. |
| ArticleNumber | 123030 |
| Author | Shao, Jiaming Chen, Guanyi Zhu, Yanqun Wang, Zhihua Yuan, Dingkun Zhang, Zhiman He, Yong Cen, Kefa Lin, Fawei |
| Author_xml | – sequence: 1 givenname: Fawei orcidid: 0000-0001-5461-8277 surname: Lin fullname: Lin, Fawei organization: School of Environmental Science and Engineering, Tianjin University, Tianjin 300072, PR China – sequence: 2 givenname: Zhihua surname: Wang fullname: Wang, Zhihua email: wangzh@zju.edu.cn organization: State Key Laboratory of Clean Energy Utilization, Zhejiang University, Hangzhou 310027, PR China – sequence: 3 givenname: Zhiman surname: Zhang fullname: Zhang, Zhiman organization: School of Environmental Science and Engineering, Tianjin University, Tianjin 300072, PR China – sequence: 4 givenname: Yong surname: He fullname: He, Yong organization: State Key Laboratory of Clean Energy Utilization, Zhejiang University, Hangzhou 310027, PR China – sequence: 5 givenname: Yanqun surname: Zhu fullname: Zhu, Yanqun organization: State Key Laboratory of Clean Energy Utilization, Zhejiang University, Hangzhou 310027, PR China – sequence: 6 givenname: Jiaming surname: Shao fullname: Shao, Jiaming organization: State Key Laboratory of Clean Energy Utilization, Zhejiang University, Hangzhou 310027, PR China – sequence: 7 givenname: Dingkun surname: Yuan fullname: Yuan, Dingkun organization: The Institute for Energy Engineering, China Jiliang University, Hangzhou 310000, PR China – sequence: 8 givenname: Guanyi surname: Chen fullname: Chen, Guanyi organization: School of Environmental Science and Engineering, Tianjin University, Tianjin 300072, PR China – sequence: 9 givenname: Kefa surname: Cen fullname: Cen, Kefa organization: State Key Laboratory of Clean Energy Utilization, Zhejiang University, Hangzhou 310027, PR China |
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| ContentType | Journal Article |
| Copyright | 2019 Elsevier B.V. |
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| DOI | 10.1016/j.cej.2019.123030 |
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| Keywords | Simultaneous removal Ozone oxidation Organic pollutants Flue gas NOx |
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Chem. contributor: fullname: Hsu |
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•Ozone oxidation coupled with post-absorption is firstly reviewed for flue gas treatment.•Simultaneous removal of NOx, SO2, VOCs, and mercury... |
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| SubjectTerms | Flue gas NOx Organic pollutants Ozone oxidation Simultaneous removal |
| Title | Flue gas treatment with ozone oxidation: An overview on NOx, organic pollutants, and mercury |
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