Exceptional Photocatalytic Activities of rGO Modified (B,N) Co‐Doped WO3, Coupled with CdSe QDs for One Photon Z‐Scheme System: A Joint Experimental and DFT Study
Artificial Z‐scheme, a tandem structure with two‐step excitation process, has gained significant attention in energy production and environmental remediation. By effectively connecting and matching the band‐gaps of two different photosystems, it is significant to utilize more photons for excellent p...
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| Published in | Advanced science Vol. 9; no. 2; pp. e2102530 - n/a |
|---|---|
| Main Authors | , , , , , , , , , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Weinheim
John Wiley & Sons, Inc
01.01.2022
John Wiley and Sons Inc Wiley |
| Subjects | |
| Online Access | Get full text |
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| Abstract | Artificial Z‐scheme, a tandem structure with two‐step excitation process, has gained significant attention in energy production and environmental remediation. By effectively connecting and matching the band‐gaps of two different photosystems, it is significant to utilize more photons for excellent photoactivity. Herein, a novel one‐photon (same energy‐two‐photon) Z‐scheme system is constructed between rGO modified boron‐nitrogen co‐doped‐WO3, and coupled CdSe quantum dots‐(QDs). The coctalyst‐0.5%RhxCr2O3(0.5RCr) modified amount‐optimized sample 6%CdSe/1%rGO3%BN‐WO3 revealed an unprecedented visible‐light driven overall‐water‐splitting to produce ≈51 µmol h−1 g−1 H2 and 25.5 µmol h−1 g−1 O2, and it remained unchanged for 5 runs in 30 h. This superior performance is ascribed to the one‐photon Z‐scheme, which simultaneously stimulates a two photocatalysts system, and enhanced charge separation as revealed by various spectroscopy techniques. The density‐functional theory is further utilized to understand the origin of this performance enhancement. This work provides a feasible strategy for constructing an efficient one‐photon Z‐scheme for practical applications.
The design of a novel Z‐scheme system based on a band gap adjusted visible‐light responsive 0.5RCr/6CdSe/1rGO/3BN‐WO3 nanocomposite is successfully constructed via hydrothermal method. This work demonstrates a promising approach to synthesize nanophotocatalysts based on WO3 for visible‐light driven solar energy application. |
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| AbstractList | Artificial Z‐scheme, a tandem structure with two‐step excitation process, has gained significant attention in energy production and environmental remediation. By effectively connecting and matching the band‐gaps of two different photosystems, it is significant to utilize more photons for excellent photoactivity. Herein, a novel one‐photon (same energy‐two‐photon) Z‐scheme system is constructed between rGO modified boron‐nitrogen co‐doped‐WO
3
, and coupled CdSe quantum dots‐(QDs). The coctalyst‐0.5%Rh
x
Cr
2
O
3
(0.5RCr) modified amount‐optimized sample 6%CdSe/1%rGO3%BN‐WO
3
revealed an unprecedented visible‐light driven overall‐water‐splitting to produce ≈51 µmol h
−1
g
−1
H
2
and 25.5 µmol h
−1
g
−1
O
2
, and it remained unchanged for 5 runs in 30 h. This superior performance is ascribed to the one‐photon Z‐scheme, which simultaneously stimulates a two photocatalysts system, and enhanced charge separation as revealed by various spectroscopy techniques. The density‐functional theory is further utilized to understand the origin of this performance enhancement. This work provides a feasible strategy for constructing an efficient one‐photon Z‐scheme for practical applications.
The design of a novel Z‐scheme system based on a band gap adjusted visible‐light responsive 0.5RCr/6CdSe/1rGO/3BN‐WO3 nanocomposite is successfully constructed via hydrothermal method. This work demonstrates a promising approach to synthesize nanophotocatalysts based on WO3 for visible‐light driven solar energy application. Artificial Z‐scheme, a tandem structure with two‐step excitation process, has gained significant attention in energy production and environmental remediation. By effectively connecting and matching the band‐gaps of two different photosystems, it is significant to utilize more photons for excellent photoactivity. Herein, a novel one‐photon (same energy‐two‐photon) Z‐scheme system is constructed between rGO modified boron‐nitrogen co‐doped‐WO3, and coupled CdSe quantum dots‐(QDs). The coctalyst‐0.5%RhxCr2O3(0.5RCr) modified amount‐optimized sample 6%CdSe/1%rGO3%BN‐WO3 revealed an unprecedented visible‐light driven overall‐water‐splitting to produce ≈51 µmol h−1 g−1 H2 and 25.5 µmol h−1 g−1 O2, and it remained unchanged for 5 runs in 30 h. This superior performance is ascribed to the one‐photon Z‐scheme, which simultaneously stimulates a two photocatalysts system, and enhanced charge separation as revealed by various spectroscopy techniques. The density‐functional theory is further utilized to understand the origin of this performance enhancement. This work provides a feasible strategy for constructing an efficient one‐photon Z‐scheme for practical applications. The design of a novel Z‐scheme system based on a band gap adjusted visible‐light responsive 0.5RCr/6CdSe/1rGO/3BN‐WO3 nanocomposite is successfully constructed via hydrothermal method. This work demonstrates a promising approach to synthesize nanophotocatalysts based on WO3 for visible‐light driven solar energy application. Abstract Artificial Z‐scheme, a tandem structure with two‐step excitation process, has gained significant attention in energy production and environmental remediation. By effectively connecting and matching the band‐gaps of two different photosystems, it is significant to utilize more photons for excellent photoactivity. Herein, a novel one‐photon (same energy‐two‐photon) Z‐scheme system is constructed between rGO modified boron‐nitrogen co‐doped‐WO3, and coupled CdSe quantum dots‐(QDs). The coctalyst‐0.5%RhxCr2O3(0.5RCr) modified amount‐optimized sample 6%CdSe/1%rGO3%BN‐WO3 revealed an unprecedented visible‐light driven overall‐water‐splitting to produce ≈51 µmol h−1 g−1 H2 and 25.5 µmol h−1 g−1 O2, and it remained unchanged for 5 runs in 30 h. This superior performance is ascribed to the one‐photon Z‐scheme, which simultaneously stimulates a two photocatalysts system, and enhanced charge separation as revealed by various spectroscopy techniques. The density‐functional theory is further utilized to understand the origin of this performance enhancement. This work provides a feasible strategy for constructing an efficient one‐photon Z‐scheme for practical applications. Artificial Z-scheme, a tandem structure with two-step excitation process, has gained significant attention in energy production and environmental remediation. By effectively connecting and matching the band-gaps of two different photosystems, it is significant to utilize more photons for excellent photoactivity. Herein, a novel one-photon (same energy-two-photon) Z-scheme system is constructed between rGO modified boron-nitrogen co-doped-WO3 , and coupled CdSe quantum dots-(QDs). The coctalyst-0.5%Rhx Cr2 O3 (0.5RCr) modified amount-optimized sample 6%CdSe/1%rGO3%BN-WO3 revealed an unprecedented visible-light driven overall-water-splitting to produce ≈51 µmol h-1 g-1 H2 and 25.5 µmol h-1 g-1 O2 , and it remained unchanged for 5 runs in 30 h. This superior performance is ascribed to the one-photon Z-scheme, which simultaneously stimulates a two photocatalysts system, and enhanced charge separation as revealed by various spectroscopy techniques. The density-functional theory is further utilized to understand the origin of this performance enhancement. This work provides a feasible strategy for constructing an efficient one-photon Z-scheme for practical applications.Artificial Z-scheme, a tandem structure with two-step excitation process, has gained significant attention in energy production and environmental remediation. By effectively connecting and matching the band-gaps of two different photosystems, it is significant to utilize more photons for excellent photoactivity. Herein, a novel one-photon (same energy-two-photon) Z-scheme system is constructed between rGO modified boron-nitrogen co-doped-WO3 , and coupled CdSe quantum dots-(QDs). The coctalyst-0.5%Rhx Cr2 O3 (0.5RCr) modified amount-optimized sample 6%CdSe/1%rGO3%BN-WO3 revealed an unprecedented visible-light driven overall-water-splitting to produce ≈51 µmol h-1 g-1 H2 and 25.5 µmol h-1 g-1 O2 , and it remained unchanged for 5 runs in 30 h. This superior performance is ascribed to the one-photon Z-scheme, which simultaneously stimulates a two photocatalysts system, and enhanced charge separation as revealed by various spectroscopy techniques. The density-functional theory is further utilized to understand the origin of this performance enhancement. This work provides a feasible strategy for constructing an efficient one-photon Z-scheme for practical applications. Artificial Z‐scheme, a tandem structure with two‐step excitation process, has gained significant attention in energy production and environmental remediation. By effectively connecting and matching the band‐gaps of two different photosystems, it is significant to utilize more photons for excellent photoactivity. Herein, a novel one‐photon (same energy‐two‐photon) Z‐scheme system is constructed between rGO modified boron‐nitrogen co‐doped‐WO3, and coupled CdSe quantum dots‐(QDs). The coctalyst‐0.5%RhxCr2O3(0.5RCr) modified amount‐optimized sample 6%CdSe/1%rGO3%BN‐WO3 revealed an unprecedented visible‐light driven overall‐water‐splitting to produce ≈51 µmol h−1 g−1 H2 and 25.5 µmol h−1 g−1 O2, and it remained unchanged for 5 runs in 30 h. This superior performance is ascribed to the one‐photon Z‐scheme, which simultaneously stimulates a two photocatalysts system, and enhanced charge separation as revealed by various spectroscopy techniques. The density‐functional theory is further utilized to understand the origin of this performance enhancement. This work provides a feasible strategy for constructing an efficient one‐photon Z‐scheme for practical applications. |
| Author | Kong, Qingquan Ali, Asad Aligayev, Amil Ali, Sharafat Zada, Amir Bakhtiar, Syedul H. Ali, Sajjad Zu, Xiaotao Liu, Chunming Shah, Rahim Khan, Muslim Shen, Huahai Wu, Xiaoqiang Raziq, Fazal Zarshad, Naghat Qiao, Liang Xia, Xiang |
| AuthorAffiliation | 8 School of Mechanical Engineering Chengdu University Chengdu 610106 P. R. China 1 Yangtze Delta Region Institute (Huzhou) University of Electronic Science and Technology of China Huzhou 313001 P. R. China 2 School of Physics University of Electronic Science and Technology of China Chengdu 610054 P. R. China 4 Department of Physics Southern University of Science and Technology Shenzhen 518055 P. R. China 5 The State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of Technology Wuhan 430070 P. R. China 3 Institute of Nuclear Physics and Chemistry Chinese Academy of Engineering Physics Mianyang 621900 P. R. China 7 Department of Chemistry Kohat University of Science and Technology Kohat KPK 26000 Pakistan 6 Department of Chemistry Abdul Wali Khan University Mardan KPK 23200 Pakistan |
| AuthorAffiliation_xml | – name: 5 The State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of Technology Wuhan 430070 P. R. China – name: 8 School of Mechanical Engineering Chengdu University Chengdu 610106 P. R. China – name: 7 Department of Chemistry Kohat University of Science and Technology Kohat KPK 26000 Pakistan – name: 2 School of Physics University of Electronic Science and Technology of China Chengdu 610054 P. R. China – name: 1 Yangtze Delta Region Institute (Huzhou) University of Electronic Science and Technology of China Huzhou 313001 P. R. China – name: 3 Institute of Nuclear Physics and Chemistry Chinese Academy of Engineering Physics Mianyang 621900 P. R. China – name: 6 Department of Chemistry Abdul Wali Khan University Mardan KPK 23200 Pakistan – name: 4 Department of Physics Southern University of Science and Technology Shenzhen 518055 P. R. China |
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| Snippet | Artificial Z‐scheme, a tandem structure with two‐step excitation process, has gained significant attention in energy production and environmental remediation.... Artificial Z-scheme, a tandem structure with two-step excitation process, has gained significant attention in energy production and environmental remediation.... Abstract Artificial Z‐scheme, a tandem structure with two‐step excitation process, has gained significant attention in energy production and environmental... |
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| StartPage | e2102530 |
| SubjectTerms | Approximation CdSe quantum dots Efficiency expending visible‐light response one‐photon Z‐scheme overall‐water splitting Photocatalysis Quantum dots Semiconductors Solar energy surface modifications WO3 Zinc oxides |
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| Title | Exceptional Photocatalytic Activities of rGO Modified (B,N) Co‐Doped WO3, Coupled with CdSe QDs for One Photon Z‐Scheme System: A Joint Experimental and DFT Study |
| URI | https://onlinelibrary.wiley.com/doi/abs/10.1002%2Fadvs.202102530 https://www.proquest.com/docview/2619605849 https://www.proquest.com/docview/2606935106 https://pubmed.ncbi.nlm.nih.gov/PMC8805570 https://doaj.org/article/2a626cd85fa14ec39dedb8f3a8905cb5 |
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