Si Doping-Induced Electronic Structure Regulation of Single-Atom Fe Sites for Boosted CO2 Electroreduction at Low Overpotentials

• Published in: Research (Washington) Vol. 6; p. 0079
• Main Authors: Cao, Changsheng, Zhou, Shenghua, Zuo, Shouwei, Zhang, Huabin, Chen, Bo, Huang, Junheng, Wu, Xin-Tao, Xu, Qiang, Zhu, Qi-Long
• Format: Journal Article
• Language: English
• Published: AAAS 2023; American Association for the Advancement of Science (AAAS)

Transition metal-based single-atom catalysts (TM-SACs) are promising alternatives to Au- and Ag-based electrocatalysts for CO production through CO2 reduction reaction. However, developing TM-SACs with high activity and selectivity at low overpotentials is challenging. Herein, a novel Fe-based SAC w...