Flexible Sensor Based on Fe 3 O 4 ‐COOH@Ti 3 C 2 T x MXene Rapid‐Gelating Hydrogel for Human Motion Monitoring
Abstract Although hydrogels are still in their infancy, research is primarily focused on optimizing their mechanical, antibacterial, anti‐frost, and water‐retaining properties. However, the rapid preparation of hydrogels without external energy stimulation remains a significant challenge. In this st...
Saved in:
Published in | Advanced materials interfaces Vol. 9; no. 22 |
---|---|
Main Authors | , , , , , , , , |
Format | Journal Article |
Language | English |
Published |
01.08.2022
|
Online Access | Get full text |
Cover
Loading…
Abstract | Abstract
Although hydrogels are still in their infancy, research is primarily focused on optimizing their mechanical, antibacterial, anti‐frost, and water‐retaining properties. However, the rapid preparation of hydrogels without external energy stimulation remains a significant challenge. In this study, a Fe
3
O
4
‐COOH@MXene@silk fibroin@polyacrylamide hybrid hydrogel (FM@SF‐PAAM) is successfully fabricated using an innovative rapid gelation method, which can initiate the gelation process as low as 7 s and formed at an extremely rapid rate at room temperature, without the use of external energy. The as‐obtained FM@SF‐PAAM hybrid hydrogel exhibits excellent electrical conductivity (6.44 × 10
–2
S m
–1
) and mechanical properties, with a maximum strain of 1660%. Additionally, the FM@SF‐PAAM‐based flexible strain sensor can monitor joint movement and emotional changes, such as finger and elbow bending, glaring, smiling, and mouth opening. Thus, the radical polymerization process demonstrates the immense potential for application to nearly all types of MXene‐based hydrogels and is likely to serve as a foundation for the development of flexible hydrogel‐based devices. |
---|---|
AbstractList | Abstract
Although hydrogels are still in their infancy, research is primarily focused on optimizing their mechanical, antibacterial, anti‐frost, and water‐retaining properties. However, the rapid preparation of hydrogels without external energy stimulation remains a significant challenge. In this study, a Fe
3
O
4
‐COOH@MXene@silk fibroin@polyacrylamide hybrid hydrogel (FM@SF‐PAAM) is successfully fabricated using an innovative rapid gelation method, which can initiate the gelation process as low as 7 s and formed at an extremely rapid rate at room temperature, without the use of external energy. The as‐obtained FM@SF‐PAAM hybrid hydrogel exhibits excellent electrical conductivity (6.44 × 10
–2
S m
–1
) and mechanical properties, with a maximum strain of 1660%. Additionally, the FM@SF‐PAAM‐based flexible strain sensor can monitor joint movement and emotional changes, such as finger and elbow bending, glaring, smiling, and mouth opening. Thus, the radical polymerization process demonstrates the immense potential for application to nearly all types of MXene‐based hydrogels and is likely to serve as a foundation for the development of flexible hydrogel‐based devices. |
Author | Fan, Qianxi Liu, Yufei Hou, Chen An, Jia Du, Jihe Hu, Yongqin Yang, Guanghao Fang, Junan Shi, Yuxia |
Author_xml | – sequence: 1 givenname: Yongqin surname: Hu fullname: Hu, Yongqin organization: Key Laboratory of Optoelectronic Technology & Systems (Chongqing University) Ministry of Education Chongqing 400044 China, Centre for Intelligent Sensing Technology College of Optoelectronic Engineering Chongqing University Chongqing 400044 China – sequence: 2 givenname: Chen surname: Hou fullname: Hou, Chen organization: Key Laboratory of Optoelectronic Technology & Systems (Chongqing University) Ministry of Education Chongqing 400044 China, Centre for Intelligent Sensing Technology College of Optoelectronic Engineering Chongqing University Chongqing 400044 China – sequence: 3 givenname: Jihe surname: Du fullname: Du, Jihe organization: Key Laboratory of Optoelectronic Technology & Systems (Chongqing University) Ministry of Education Chongqing 400044 China, Centre for Intelligent Sensing Technology College of Optoelectronic Engineering Chongqing University Chongqing 400044 China – sequence: 4 givenname: Qianxi surname: Fan fullname: Fan, Qianxi organization: Key Laboratory of Optoelectronic Technology & Systems (Chongqing University) Ministry of Education Chongqing 400044 China – sequence: 5 givenname: Junan surname: Fang fullname: Fang, Junan organization: Key Laboratory of Optoelectronic Technology & Systems (Chongqing University) Ministry of Education Chongqing 400044 China, Centre for Intelligent Sensing Technology College of Optoelectronic Engineering Chongqing University Chongqing 400044 China – sequence: 6 givenname: Yuxia surname: Shi fullname: Shi, Yuxia organization: Key Laboratory of Optoelectronic Technology & Systems (Chongqing University) Ministry of Education Chongqing 400044 China – sequence: 7 givenname: Guanghao surname: Yang fullname: Yang, Guanghao organization: Key Laboratory of Optoelectronic Technology & Systems (Chongqing University) Ministry of Education Chongqing 400044 China, Centre for Intelligent Sensing Technology College of Optoelectronic Engineering Chongqing University Chongqing 400044 China – sequence: 8 givenname: Jia surname: An fullname: An, Jia organization: School of Microelectronics Southern University of Science and Technology Shenzhen 518055 China – sequence: 9 givenname: Yufei orcidid: 0000-0003-2988-8843 surname: Liu fullname: Liu, Yufei organization: Key Laboratory of Optoelectronic Technology & Systems (Chongqing University) Ministry of Education Chongqing 400044 China, Centre for Intelligent Sensing Technology College of Optoelectronic Engineering Chongqing University Chongqing 400044 China, Centre for Nano Health College of Science Swansea University Singleton Park Swansea SA2 8PP UK |
BookMark | eNpNkM1Kw0AcxBepYK29ev6_QOp-Jbu5qcE2QktAc_AWdptNWUl3y26F9uYj-Ix9ElMU8TTDzDCH3zUaOe8MQrcEzwjG9E61WzujmFKMuRQXaExJniWCpXj0z1-haYzvGGNCKKGSjVGY9-ZgdW_g1bjoAzyqaFrwDuYGGFTA4fT5VVRVeV_bISiAQg0HWL0ZZ-BF7Ww79AvTq711GyiPbfAb00M3XJUfW-Vg5ffWn8XZvQ_D6AZddqqPZvqrE1TPn-qiTJbV4rl4WCZryUXCea50qlNlpGJCZbmkQqWYZVoTxrTmlDOqujWXbUo6lhEmNRXY5C3ORcZzNkGzn9t18DEG0zW7YLcqHBuCmzOz5sys-WPGvgFmgl-Q |
CitedBy_id | crossref_primary_10_3390_mi13101792 crossref_primary_10_1038_s41570_023_00486_x crossref_primary_10_1021_acsami_3c14210 crossref_primary_10_1002_mame_202200519 crossref_primary_10_1016_j_jcis_2023_12_039 |
Cites_doi | 10.1021/acsnano.9b06134 10.1016/j.cej.2019.121915 10.1002/adma.201102306 10.1002/adfm.201903960 10.1002/adfm.201904507 10.1021/acs.chemmater.9b04041 10.1039/C8MH01561A 10.1016/j.jcis.2020.09.105 10.1021/acsnano.9b08462 10.1016/j.ijbiomac.2021.04.067 10.1021/acsnano.0c08830 10.1021/acsami.0c12239 10.1016/j.microc.2021.106155 10.1016/j.jcis.2020.10.128 10.1007/s40820-022-00827-3 10.1002/adma.201902432 10.1002/adfm.202104536 10.1002/adfm.201703132 10.1088/1361-6528/ac4878 10.1002/adfm.202101957 10.1021/acs.analchem.8b02572 10.1016/j.jpowsour.2016.04.035 10.1016/j.cej.2020.126129 10.1021/acsami.1c05098 10.1021/acsnano.9b06144 10.1021/acsami.9b19721 10.1016/j.bios.2015.11.004 10.1039/C3GC41535J 10.1016/j.biomaterials.2020.120299 10.1039/D0TA11437E 10.1002/admi.202102266 10.1021/acsami.1c04255 10.1016/j.foodchem.2018.04.016 10.1016/j.jcis.2017.07.029 10.1021/acsnano.0c07998 |
ContentType | Journal Article |
DBID | AAYXX CITATION |
DOI | 10.1002/admi.202200487 |
DatabaseName | CrossRef |
DatabaseTitle | CrossRef |
DatabaseTitleList | CrossRef |
DeliveryMethod | fulltext_linktorsrc |
Discipline | Physics |
EISSN | 2196-7350 |
ExternalDocumentID | 10_1002_admi_202200487 |
GroupedDBID | 0R~ 1OC 24P 33P AAESR AAHHS AAIHA AAXRX AAYXX AAZKR ABCUV ABJCF ACAHQ ACCFJ ACCZN ACGFS ACPOU ACXBN ACXQS ADBBV ADKYN ADOZA ADXAS ADZMN ADZOD AEEZP AENEX AEQDE AFBPY AFKRA AIACR AIURR AIWBW AJBDE ALMA_UNASSIGNED_HOLDINGS ALUQN AMYDB ARAPS ARCSS AVUZU AZVAB BENPR BFHJK BGLVJ BMXJE BRXPI CCPQU CITATION DCZOG DPXWK EBS EJD G-S GODZA GROUPED_DOAJ HCIFZ KB. LATKE LEEKS LITHE LOXES LUTES LYRES M7S MEWTI MY~ M~E O9- P2W PDBOC PTHSS R.K ROL SUPJJ WBKPD WOHZO WXSBR WYJ ZZTAW |
ID | FETCH-LOGICAL-c847-449ab5b5ae8a37a69827a5036bb133bb42432afc48d51f36138b270e9d0976493 |
ISSN | 2196-7350 |
IngestDate | Thu Sep 12 17:39:36 EDT 2024 |
IsPeerReviewed | true |
IsScholarly | true |
Issue | 22 |
Language | English |
LinkModel | OpenURL |
MergedId | FETCHMERGED-LOGICAL-c847-449ab5b5ae8a37a69827a5036bb133bb42432afc48d51f36138b270e9d0976493 |
ORCID | 0000-0003-2988-8843 |
ParticipantIDs | crossref_primary_10_1002_admi_202200487 |
PublicationCentury | 2000 |
PublicationDate | 2022-08-00 |
PublicationDateYYYYMMDD | 2022-08-01 |
PublicationDate_xml | – month: 08 year: 2022 text: 2022-08-00 |
PublicationDecade | 2020 |
PublicationTitle | Advanced materials interfaces |
PublicationYear | 2022 |
References | e_1_2_8_28_1 e_1_2_8_29_1 e_1_2_8_24_1 e_1_2_8_25_1 e_1_2_8_26_1 e_1_2_8_27_1 e_1_2_8_3_1 e_1_2_8_2_1 e_1_2_8_5_1 e_1_2_8_4_1 e_1_2_8_7_1 e_1_2_8_6_1 e_1_2_8_9_1 e_1_2_8_8_1 e_1_2_8_20_1 e_1_2_8_21_1 e_1_2_8_22_1 e_1_2_8_23_1 e_1_2_8_1_1 e_1_2_8_17_1 e_1_2_8_18_1 e_1_2_8_19_1 e_1_2_8_13_1 e_1_2_8_14_1 e_1_2_8_35_1 e_1_2_8_15_1 e_1_2_8_16_1 e_1_2_8_32_1 e_1_2_8_10_1 e_1_2_8_31_1 e_1_2_8_11_1 e_1_2_8_34_1 e_1_2_8_12_1 e_1_2_8_33_1 e_1_2_8_30_1 |
References_xml | – ident: e_1_2_8_25_1 doi: 10.1021/acsnano.9b06134 – ident: e_1_2_8_4_1 doi: 10.1016/j.cej.2019.121915 – ident: e_1_2_8_10_1 doi: 10.1002/adma.201102306 – ident: e_1_2_8_15_1 doi: 10.1002/adfm.201903960 – ident: e_1_2_8_14_1 doi: 10.1002/adfm.201904507 – ident: e_1_2_8_1_1 doi: 10.1021/acs.chemmater.9b04041 – ident: e_1_2_8_29_1 doi: 10.1039/C8MH01561A – ident: e_1_2_8_9_1 doi: 10.1016/j.jcis.2020.09.105 – ident: e_1_2_8_13_1 doi: 10.1021/acsnano.9b08462 – ident: e_1_2_8_23_1 doi: 10.1016/j.ijbiomac.2021.04.067 – ident: e_1_2_8_32_1 doi: 10.1021/acsnano.0c08830 – ident: e_1_2_8_28_1 doi: 10.1021/acsami.0c12239 – ident: e_1_2_8_19_1 doi: 10.1016/j.microc.2021.106155 – ident: e_1_2_8_3_1 doi: 10.1016/j.jcis.2020.10.128 – ident: e_1_2_8_5_1 doi: 10.1007/s40820-022-00827-3 – ident: e_1_2_8_16_1 doi: 10.1002/adma.201902432 – ident: e_1_2_8_6_1 doi: 10.1002/adfm.202104536 – ident: e_1_2_8_7_1 doi: 10.1002/adfm.201703132 – ident: e_1_2_8_21_1 doi: 10.1088/1361-6528/ac4878 – ident: e_1_2_8_30_1 doi: 10.1002/adfm.202101957 – ident: e_1_2_8_8_1 doi: 10.1021/acs.analchem.8b02572 – ident: e_1_2_8_11_1 doi: 10.1016/j.jpowsour.2016.04.035 – ident: e_1_2_8_17_1 doi: 10.1016/j.cej.2020.126129 – ident: e_1_2_8_33_1 doi: 10.1021/acsami.1c05098 – ident: e_1_2_8_2_1 doi: 10.1021/acsnano.9b06144 – ident: e_1_2_8_31_1 doi: 10.1021/acsami.9b19721 – ident: e_1_2_8_27_1 doi: 10.1016/j.bios.2015.11.004 – ident: e_1_2_8_22_1 doi: 10.1039/C3GC41535J – ident: e_1_2_8_20_1 doi: 10.1016/j.biomaterials.2020.120299 – ident: e_1_2_8_34_1 doi: 10.1039/D0TA11437E – ident: e_1_2_8_12_1 doi: 10.1002/admi.202102266 – ident: e_1_2_8_35_1 doi: 10.1021/acsami.1c04255 – ident: e_1_2_8_26_1 doi: 10.1016/j.foodchem.2018.04.016 – ident: e_1_2_8_24_1 doi: 10.1016/j.jcis.2017.07.029 – ident: e_1_2_8_18_1 doi: 10.1021/acsnano.0c07998 |
SSID | ssj0001121283 |
Score | 2.2861292 |
Snippet | Abstract
Although hydrogels are still in their infancy, research is primarily focused on optimizing their mechanical, antibacterial, anti‐frost, and... |
SourceID | crossref |
SourceType | Aggregation Database |
Title | Flexible Sensor Based on Fe 3 O 4 ‐COOH@Ti 3 C 2 T x MXene Rapid‐Gelating Hydrogel for Human Motion Monitoring |
Volume | 9 |
hasFullText | 1 |
inHoldings | 1 |
isFullTextHit | |
isPrint | |
link | http://utb.summon.serialssolutions.com/2.0.0/link/0/eLvHCXMwnV1Lj9MwELbKrpC4rHiKt3wAcbBSWsd53VgKIVppqYAUVVwqO7FLDiS7oZUKJy7c-Y38EiZ2nAToYeESVZOkcTKfZr6ZzEwQehQpnzMlmUO5pyBAcbnDPc6cTIH-M1_xLNcFsq_9ZMFOlt5yNPo-qFrabsQ4-7q3r-R_tAoy0GvTJfsPmu3-FATwG_QLW9AwbC-k47iZZtm0Pr2DYLSqyXNwSXmT_o8lccmcMNLVMszm8-Qxm6QF7JgRSlKyI6dLMHTkLT-DhdvjXuniuHJNki95Xa2lbm9sU_2n-os_rRmorc-zI2xtMQFQYHPvehRFrZqarx482uRX5fq86FCZVFvz4r_vSnuhJSfFxw52sUnUvgE074phqgKiXFso11o0sI6-E7hm0uxY7pG1JjkaIM-0Lf9l6c3kWJ5_KsbNpRpLFPQ-zb7H_8PVdQWIZlgzXTXnr7rzL6FDGkQexPCHx-8XHxZ9sm4KHl6PdO2WaweATujT3xcxIDgDppJeRUdtiIGPDV6uoZEsr6PLutQ3-3wD1RY12KAGa9TgqsSxxC6eY4Z_fvvR4OVZWoBghilO8Q5rtGCNFthvcYItTjDgBGucYIMT3OPkJkrjl-kscdovbzgZsBWHsYgLT3hchtwNuB-FNOAecB0hpq4rBKPMpVxlLMy9qXKBEYaCBhMZ5RNgtyxyb6GDsirlbYSVYOBAM28a5op5uYryTLAJ5ZKrEMhvfgc9sU9rdWbmq6z2K-fuhY-8h6706LuPDjb1Vj4A6rgRD1vF_gIk5GkK |
link.rule.ids | 315,786,790,27957,27958 |
linkProvider | Wiley-Blackwell |
openUrl | ctx_ver=Z39.88-2004&ctx_enc=info%3Aofi%2Fenc%3AUTF-8&rfr_id=info%3Asid%2Fsummon.serialssolutions.com&rft_val_fmt=info%3Aofi%2Ffmt%3Akev%3Amtx%3Ajournal&rft.genre=article&rft.atitle=Flexible+Sensor+Based+on+Fe+3+O+4+%E2%80%90COOH%40Ti+3+C+2+T+x+MXene+Rapid%E2%80%90Gelating+Hydrogel+for+Human+Motion+Monitoring&rft.jtitle=Advanced+materials+interfaces&rft.au=Hu%2C+Yongqin&rft.au=Hou%2C+Chen&rft.au=Du%2C+Jihe&rft.au=Fan%2C+Qianxi&rft.date=2022-08-01&rft.issn=2196-7350&rft.eissn=2196-7350&rft.volume=9&rft.issue=22&rft_id=info:doi/10.1002%2Fadmi.202200487&rft.externalDBID=n%2Fa&rft.externalDocID=10_1002_admi_202200487 |
thumbnail_l | http://covers-cdn.summon.serialssolutions.com/index.aspx?isbn=/lc.gif&issn=2196-7350&client=summon |
thumbnail_m | http://covers-cdn.summon.serialssolutions.com/index.aspx?isbn=/mc.gif&issn=2196-7350&client=summon |
thumbnail_s | http://covers-cdn.summon.serialssolutions.com/index.aspx?isbn=/sc.gif&issn=2196-7350&client=summon |