Crystallization Behavior and Luminescence of Inkjet Printing CH 3 NH 3 PbBr 3
Abstract Lead halide perovskites display remarkable optoelectronic properties, like large absorption coefficients, high photoluminescence quantum efficiencies, and long lifetime and diffusion length of photocarriers. This system is easily fabricated using solution processes and inkjet printing is an...
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Published in | Crystal research and technology (1979) Vol. 56; no. 8 |
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Main Authors | , , , , , |
Format | Journal Article |
Language | English |
Published |
01.08.2021
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Online Access | Get full text |
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Abstract | Abstract
Lead halide perovskites display remarkable optoelectronic properties, like large absorption coefficients, high photoluminescence quantum efficiencies, and long lifetime and diffusion length of photocarriers. This system is easily fabricated using solution processes and inkjet printing is an effective way to prepare halide perovskite films and complex patterns. In this work, the crystallization behaviors of inkjet printing CH
3
NH
3
PbBr
3
crystals are systematically investigated with varied I
−
doping, printing times, and solvents. Using
N
,
N
‐dimethylformamide (DMF) solvent, CH
3
NH
3
PbBr
3−
x
I
x
(
x
= 0, 0.14, 0.29, 0.45, 0.59) are printed on the glass and the crystalline grains are developed from the (001) oriented tetragonal in side length of 10–50 µm to dendrite with increasing I
−
concentrations. The crystalline grains are kept tetragonal, while the average crystal size changes from 22 to 89 µm by increasing the number of printing from 10 to 1000 times. DMF and dimethyl sulfoxide (DMSO) are used as solvents for printing CH
3
NH
3
PbBr
3
, and more regular grains are obtained from DMF solvent. Several patterns are printed on glass and papers, and fluorescent two‐dimensional (2D) patterns are observed under the 480 nm excitation. The as‐printed patterns show excellent homogeneity and high reproducibility, indicating that the inkjet printing shows broad application prospects in flexible electronics. |
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AbstractList | Abstract
Lead halide perovskites display remarkable optoelectronic properties, like large absorption coefficients, high photoluminescence quantum efficiencies, and long lifetime and diffusion length of photocarriers. This system is easily fabricated using solution processes and inkjet printing is an effective way to prepare halide perovskite films and complex patterns. In this work, the crystallization behaviors of inkjet printing CH
3
NH
3
PbBr
3
crystals are systematically investigated with varied I
−
doping, printing times, and solvents. Using
N
,
N
‐dimethylformamide (DMF) solvent, CH
3
NH
3
PbBr
3−
x
I
x
(
x
= 0, 0.14, 0.29, 0.45, 0.59) are printed on the glass and the crystalline grains are developed from the (001) oriented tetragonal in side length of 10–50 µm to dendrite with increasing I
−
concentrations. The crystalline grains are kept tetragonal, while the average crystal size changes from 22 to 89 µm by increasing the number of printing from 10 to 1000 times. DMF and dimethyl sulfoxide (DMSO) are used as solvents for printing CH
3
NH
3
PbBr
3
, and more regular grains are obtained from DMF solvent. Several patterns are printed on glass and papers, and fluorescent two‐dimensional (2D) patterns are observed under the 480 nm excitation. The as‐printed patterns show excellent homogeneity and high reproducibility, indicating that the inkjet printing shows broad application prospects in flexible electronics. |
Author | Guan, Yimin Shen, Hui Xu, Jiayue Sun, Rui Li, Haixia Du, Yong |
Author_xml | – sequence: 1 givenname: Rui surname: Sun fullname: Sun, Rui organization: Institute of Crystal Growth School of Materials Science and Engineering Shanghai Institute of Technology Shanghai 201418 China – sequence: 2 givenname: Haixia surname: Li fullname: Li, Haixia organization: Institute of Crystal Growth School of Materials Science and Engineering Shanghai Institute of Technology Shanghai 201418 China – sequence: 3 givenname: Yimin surname: Guan fullname: Guan, Yimin organization: Shanghai Industrial μTechnology Research Institute Shanghai 201800 China – sequence: 4 givenname: Yong surname: Du fullname: Du, Yong organization: Institute of Crystal Growth School of Materials Science and Engineering Shanghai Institute of Technology Shanghai 201418 China – sequence: 5 givenname: Hui orcidid: 0000-0003-4968-977X surname: Shen fullname: Shen, Hui organization: Institute of Crystal Growth School of Materials Science and Engineering Shanghai Institute of Technology Shanghai 201418 China – sequence: 6 givenname: Jiayue surname: Xu fullname: Xu, Jiayue organization: Institute of Crystal Growth School of Materials Science and Engineering Shanghai Institute of Technology Shanghai 201418 China |
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Lead halide perovskites display remarkable optoelectronic properties, like large absorption coefficients, high photoluminescence quantum efficiencies,... |
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Title | Crystallization Behavior and Luminescence of Inkjet Printing CH 3 NH 3 PbBr 3 |
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