Construction of visible light–responsive Z-scheme CdS/BiOI photocatalyst with enhanced photocatalytic CO 2 reduction activity

Abstract Rational construction of Z-scheme photocatalysts and exploration of the Z-scheme charge transfer mechanism have drawn much attention in the field of CO 2 reduction because of its great potential to alleviate energy crisis and environmental problems. In this study, a series of Z-scheme CdS/B...

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Published inJournal of materials research Vol. 34; no. 23; pp. 3907 - 3917
Main Authors Zhou, Rong-Hui, Wei, Zhi-He, Li, Yan-Yang, Li, Zhong-Jun, Yao, Hong-Chang
Format Journal Article
LanguageEnglish
Published 16.12.2019
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Abstract Abstract Rational construction of Z-scheme photocatalysts and exploration of the Z-scheme charge transfer mechanism have drawn much attention in the field of CO 2 reduction because of its great potential to alleviate energy crisis and environmental problems. In this study, a series of Z-scheme CdS/BiOI composites were constructed by depositing CdS nanoparticles on the surface of BiOI nanosheets. The synthesized materials were characterized comprehensively, and their photoreduction CO 2 activities were evaluated. The results show that the composites exhibit higher photoreduction CO 2 activity under visible light irradiation (λ > 400 nm) than pure CdS and BiOI. The yields of CO and CH 4 for the optimal composite after 3 h irradiation are 3.32 and 0.54 μmol/g, respectively. The improved photocatalytic activity is attributed to Z-scheme transfer mode of the photogenerated charges in the composites. The mechanism of CO 2 reduction is proposed and verified experimentally.
AbstractList Abstract Rational construction of Z-scheme photocatalysts and exploration of the Z-scheme charge transfer mechanism have drawn much attention in the field of CO 2 reduction because of its great potential to alleviate energy crisis and environmental problems. In this study, a series of Z-scheme CdS/BiOI composites were constructed by depositing CdS nanoparticles on the surface of BiOI nanosheets. The synthesized materials were characterized comprehensively, and their photoreduction CO 2 activities were evaluated. The results show that the composites exhibit higher photoreduction CO 2 activity under visible light irradiation (λ > 400 nm) than pure CdS and BiOI. The yields of CO and CH 4 for the optimal composite after 3 h irradiation are 3.32 and 0.54 μmol/g, respectively. The improved photocatalytic activity is attributed to Z-scheme transfer mode of the photogenerated charges in the composites. The mechanism of CO 2 reduction is proposed and verified experimentally.
Author Yao, Hong-Chang
Zhou, Rong-Hui
Wei, Zhi-He
Li, Yan-Yang
Li, Zhong-Jun
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