Synthesis, luminescence properties, and growth mechanisms of YF 3 :Yb 3+ /Er 3+ nanoplates
Anisotropically structured upconversion nanocrystals capable of exhibiting bright upconversion emission properties are a promising new class of high performance optical materials. In this study, we investigate a facile synthetic method for the new nanoplate structure of YF 3 :Yb 3+ /Er 3+ with enhan...
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| Published in | Journal of materials chemistry. C, Materials for optical and electronic devices Vol. 3; no. 39; pp. 10107 - 10113 |
|---|---|
| Main Authors | , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
2015
|
| Online Access | Get full text |
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| Abstract | Anisotropically structured upconversion nanocrystals capable of exhibiting bright upconversion emission properties are a promising new class of high performance optical materials. In this study, we investigate a facile synthetic method for the new nanoplate structure of YF
3
:Yb
3+
/Er
3+
with enhanced luminescence intensity. The shape of YF
3
:Yb
3+
/Er
3+
nanocrystals can be controlled by changing the synthesis conditions of the NaOH concentration, reaction time, and surfactant. The concentration of NaOH determines the final structure of YF
3
:Yb
3+
/Er
3+
. By increasing the NaOH concentration from 0.25 mmol to 2.5 mmol, YF
3
:Yb
3+
/Er
3+
nanoplates transform into NaYF
4
:Yb
3+
/Er
3+
nanoparticles; in the absence of NaOH, the nanoplate structure of YF
3
:Yb
3+
/Er
3+
changes to particles. The YF
3
:Yb
3+
/Er
3+
nanoplates show luminescence efficiency much greater than that of the spherical YF
3
:Yb
3+
/Er
3+
nanocrystals. |
|---|---|
| AbstractList | Anisotropically structured upconversion nanocrystals capable of exhibiting bright upconversion emission properties are a promising new class of high performance optical materials. In this study, we investigate a facile synthetic method for the new nanoplate structure of YF
3
:Yb
3+
/Er
3+
with enhanced luminescence intensity. The shape of YF
3
:Yb
3+
/Er
3+
nanocrystals can be controlled by changing the synthesis conditions of the NaOH concentration, reaction time, and surfactant. The concentration of NaOH determines the final structure of YF
3
:Yb
3+
/Er
3+
. By increasing the NaOH concentration from 0.25 mmol to 2.5 mmol, YF
3
:Yb
3+
/Er
3+
nanoplates transform into NaYF
4
:Yb
3+
/Er
3+
nanoparticles; in the absence of NaOH, the nanoplate structure of YF
3
:Yb
3+
/Er
3+
changes to particles. The YF
3
:Yb
3+
/Er
3+
nanoplates show luminescence efficiency much greater than that of the spherical YF
3
:Yb
3+
/Er
3+
nanocrystals. |
| Author | Lee, Byeong Hoon Lee, Joong Hee Suh, Yung Doug Lim, Dong-Kwon Murali, G. Lee, Jae Myeong Lee, Seung Hee Mishra, R. K. Nam, Sang-Hwan |
| Author_xml | – sequence: 1 givenname: G. surname: Murali fullname: Murali, G. organization: Applied Materials Institute for BIN Convergence, Department of BIN Fusion Technology and Department of Polymer-Nano Science and Technology, Chonbuk National University, Jeonju, Korea – sequence: 2 givenname: Byeong Hoon surname: Lee fullname: Lee, Byeong Hoon organization: Applied Materials Institute for BIN Convergence, Department of BIN Fusion Technology and Department of Polymer-Nano Science and Technology, Chonbuk National University, Jeonju, Korea – sequence: 3 givenname: R. K. surname: Mishra fullname: Mishra, R. K. organization: Applied Materials Institute for BIN Convergence, Department of BIN Fusion Technology and Department of Polymer-Nano Science and Technology, Chonbuk National University, Jeonju, Korea – sequence: 4 givenname: Jae Myeong surname: Lee fullname: Lee, Jae Myeong organization: Applied Materials Institute for BIN Convergence, Department of BIN Fusion Technology and Department of Polymer-Nano Science and Technology, Chonbuk National University, Jeonju, Korea – sequence: 5 givenname: Sang-Hwan surname: Nam fullname: Nam, Sang-Hwan organization: Laboratory for Advanced Molecular Probing (LAMP), Korea Research Institute of Chemical Technology, Daejeon 305-600, South Korea – sequence: 6 givenname: Yung Doug surname: Suh fullname: Suh, Yung Doug organization: Laboratory for Advanced Molecular Probing (LAMP), Korea Research Institute of Chemical Technology, Daejeon 305-600, South Korea, School of Chemical Engineering – sequence: 7 givenname: Dong-Kwon surname: Lim fullname: Lim, Dong-Kwon organization: KU-KIST Graduate School of Converging Science and Technology, Korea University, Seongbuk-gu, Korea – sequence: 8 givenname: Joong Hee surname: Lee fullname: Lee, Joong Hee organization: Applied Materials Institute for BIN Convergence, Department of BIN Fusion Technology and Department of Polymer-Nano Science and Technology, Chonbuk National University, Jeonju, Korea – sequence: 9 givenname: Seung Hee surname: Lee fullname: Lee, Seung Hee organization: Applied Materials Institute for BIN Convergence, Department of BIN Fusion Technology and Department of Polymer-Nano Science and Technology, Chonbuk National University, Jeonju, Korea |
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