Grape juice: an effective liquid additive for significant enhancement of thermoelectric performance of Cu 2 Se
The reduction of thermal conductivity and enhancement of electrical properties is the ultimate goal for achieving high-performance thermoelectric materials. In this paper, a high thermoelectric performance is demonstrated when grape juice is used as an additive to Cu 2 Se. High temperature processin...
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| Published in | Journal of materials chemistry. A, Materials for energy and sustainability Vol. 8; no. 33; pp. 16913 - 16919 |
|---|---|
| Main Authors | , , |
| Format | Journal Article |
| Language | English |
| Published |
25.08.2020
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| Online Access | Get full text |
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| Abstract | The reduction of thermal conductivity and enhancement of electrical properties is the ultimate goal for achieving high-performance thermoelectric materials. In this paper, a high thermoelectric performance is demonstrated when grape juice is used as an additive to Cu
2
Se. High temperature processing of the mixture pyrolyzes the sugars in the grape juice and provides a fine-scale and well-mixed dispersion of elemental carbon in the Cu
2
Se matrix. These materials show a significant enhancement of electrical conductivity due to a high hole concentration with little change of the Seebeck coefficient, leading to an ultra-high power factor of 1.3 mW m
−1
K
−2
at 984 K. Microstructural studies reveal that the carbon phase is embedded on the Cu
2
Se grain boundaries and that Cu
2
O nanoparticles are located at the interface between carbon and Cu
2
Se. This results in phonon scattering at the interface which leads to a reduction of thermal conductivity of up to ∼38%. It is proposed that the formation of Cu
2
O also induces Cu deficiencies in Cu
2
Se resulting in greater enhancement of electrical conductivity. As a result, the
zT
is significantly enhanced up to ∼2.5 at 984 K. This study opens up a new avenue for enhancing the properties of thermoelectric materials. |
|---|---|
| AbstractList | The reduction of thermal conductivity and enhancement of electrical properties is the ultimate goal for achieving high-performance thermoelectric materials. In this paper, a high thermoelectric performance is demonstrated when grape juice is used as an additive to Cu
2
Se. High temperature processing of the mixture pyrolyzes the sugars in the grape juice and provides a fine-scale and well-mixed dispersion of elemental carbon in the Cu
2
Se matrix. These materials show a significant enhancement of electrical conductivity due to a high hole concentration with little change of the Seebeck coefficient, leading to an ultra-high power factor of 1.3 mW m
−1
K
−2
at 984 K. Microstructural studies reveal that the carbon phase is embedded on the Cu
2
Se grain boundaries and that Cu
2
O nanoparticles are located at the interface between carbon and Cu
2
Se. This results in phonon scattering at the interface which leads to a reduction of thermal conductivity of up to ∼38%. It is proposed that the formation of Cu
2
O also induces Cu deficiencies in Cu
2
Se resulting in greater enhancement of electrical conductivity. As a result, the
zT
is significantly enhanced up to ∼2.5 at 984 K. This study opens up a new avenue for enhancing the properties of thermoelectric materials. |
| Author | Nazrul Islam, Sheik Md Kazi Cortie, Michael B. Wang, Xiaolin |
| Author_xml | – sequence: 1 givenname: Sheik Md Kazi orcidid: 0000-0001-7272-2713 surname: Nazrul Islam fullname: Nazrul Islam, Sheik Md Kazi organization: Institute for Superconducting and Electronic Materials, Australian Institute for Innovative Materials, University of Wollongong, North Wollongong, Australia – sequence: 2 givenname: Michael B. orcidid: 0000-0003-3202-6398 surname: Cortie fullname: Cortie, Michael B. organization: School of Mathematical and Physical Sciences, University of Technology Sydney, Australia – sequence: 3 givenname: Xiaolin orcidid: 0000-0003-4150-0848 surname: Wang fullname: Wang, Xiaolin organization: Institute for Superconducting and Electronic Materials, Australian Institute for Innovative Materials, University of Wollongong, North Wollongong, Australia |
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| StartPage | 16913 |
| Title | Grape juice: an effective liquid additive for significant enhancement of thermoelectric performance of Cu 2 Se |
| Volume | 8 |
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