Biochars derived from bamboo and rice straw for sorption of basic red dyes

The primary purpose of this study is to eliminate Basic Red 46 dye from aqueous solutions utilizing batch experiments by adsorption on biochars prepared from bamboo and rice straw biomass. Biochars prepared from bamboo (B), and rice straw (R) was pyrolyzed at 500°C (B500 and R500). Scanning Electron...

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Published inPloS one Vol. 16; no. 7; p. e0254637
Main Authors Sackey, Ebenezer Ampofo, Song, Yali, Yu, Ya, Zhuang, Haifeng
Format Journal Article
LanguageEnglish
Published United States Public Library of Science 14.07.2021
Public Library of Science (PLoS)
Subjects
Activated carbon
Adsorbents
Adsorption
Analysis
Analyzers
Aqueous solutions
Azo Compounds
Bamboo
Biology and Life Sciences
Biomass
Charcoal
Civil engineering
Dyes
Dyes and dyeing
Earth Sciences
Ecology and Environmental Sciences
Effluents
Electron microscopy
Electrostatic properties
Equilibrium
Experiments
Fourier transforms
Functional groups
High temperature
Infrared analysis
Interaction parameters
Kinetics
Laboratories
Membrane separation
Organic chemicals
Oryza
Physical Sciences
Pollutants
Porosity
Properties
Research and Analysis Methods
Rice
Rice straw
Scanning electron microscopy
Silicates
Spectroscopy
Straw
Temperature rise
Thermodynamics
Water treatment
X-ray diffraction
China
Zhejiang China
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Abstract The primary purpose of this study is to eliminate Basic Red 46 dye from aqueous solutions utilizing batch experiments by adsorption on biochars prepared from bamboo and rice straw biomass. Biochars prepared from bamboo (B), and rice straw (R) was pyrolyzed at 500°C (B500 and R500). Scanning Electron Microscopy (SEM), Fourier Transform Infrared (FTIR) Spectroscopy, X-ray Diffraction (XRD), and surface area and porosity analyzers were used to characterize the B500 and R500 samples. The characterization results indicated that the biochars possessed an amorphous porous structure with many functional groups consisting primarily of silicates. The adsorption rate of BR46 was evaluated using two kinetic models (pseudo-first-order and pseudo-second-order), and the results indicated that the pseudo-second-order model fitted to the experimental data well (R 2 >0.99). Nearly 24 h was sufficient to achieve equilibrium with the dye adsorption for the two biochars. R500 had a greater adsorption efficiency than B500. As pH levels increased, the dye’s adsorption capability increased as well. The Langmuir and Freundlich isotherm models were used to investigate the equilibrium behavior of BR46 adsorption, and the equilibrium data fitted well with the Langmuir model (R 2 >0.99) compared to the Freundlich model (R 2 >0.89). The maximum adsorption capacities of BR46 are 9.06 mg/g for B500 and 22.12 mg/g for R500, respectively. Additionally, adsorption capacity increased as temperature increased, indicating that adsorption is favored at higher temperatures. The electrostatic interaction is shown to be the dominant mechanism of BR46 adsorption, and BR46 acts as an electron-acceptor, contributing to n-π EDA (Electron Donor-Acceptor) interaction. Thermodynamic parameters for the dye-adsorbent system revealed that the adsorption process is spontaneous and feasible. The values of the adsorption coefficient (K d ) were on the order of 10 2 −10 3 . K d of R500 was greater than that of B500, indicating that R500 had a greater adsorption capacity. The results showed that R500 could be used as a low-cost alternative adsorbent for removing BR46 from effluents.
AbstractList The primary purpose of this study is to eliminate Basic Red 46 dye from aqueous solutions utilizing batch experiments by adsorption on biochars prepared from bamboo and rice straw biomass. Biochars prepared from bamboo (B), and rice straw (R) was pyrolyzed at 500°C (B500 and R500). Scanning Electron Microscopy (SEM), Fourier Transform Infrared (FTIR) Spectroscopy, X-ray Diffraction (XRD), and surface area and porosity analyzers were used to characterize the B500 and R500 samples. The characterization results indicated that the biochars possessed an amorphous porous structure with many functional groups consisting primarily of silicates. The adsorption rate of BR46 was evaluated using two kinetic models (pseudo-first-order and pseudo-second-order), and the results indicated that the pseudo-second-order model fitted to the experimental data well (R2>0.99). Nearly 24 h was sufficient to achieve equilibrium with the dye adsorption for the two biochars. R500 had a greater adsorption efficiency than B500. As pH levels increased, the dye’s adsorption capability increased as well. The Langmuir and Freundlich isotherm models were used to investigate the equilibrium behavior of BR46 adsorption, and the equilibrium data fitted well with the Langmuir model (R2>0.99) compared to the Freundlich model (R2>0.89). The maximum adsorption capacities of BR46 are 9.06 mg/g for B500 and 22.12 mg/g for R500, respectively. Additionally, adsorption capacity increased as temperature increased, indicating that adsorption is favored at higher temperatures. The electrostatic interaction is shown to be the dominant mechanism of BR46 adsorption, and BR46 acts as an electron-acceptor, contributing to n-π EDA (Electron Donor-Acceptor) interaction. Thermodynamic parameters for the dye-adsorbent system revealed that the adsorption process is spontaneous and feasible. The values of the adsorption coefficient (Kd) were on the order of 102−103. Kd of R500 was greater than that of B500, indicating that R500 had a greater adsorption capacity. The results showed that R500 could be used as a low-cost alternative adsorbent for removing BR46 from effluents.
The primary purpose of this study is to eliminate Basic Red 46 dye from aqueous solutions utilizing batch experiments by adsorption on biochars prepared from bamboo and rice straw biomass. Biochars prepared from bamboo (B), and rice straw (R) was pyrolyzed at 500°C (B500 and R500). Scanning Electron Microscopy (SEM), Fourier Transform Infrared (FTIR) Spectroscopy, X-ray Diffraction (XRD), and surface area and porosity analyzers were used to characterize the B500 and R500 samples. The characterization results indicated that the biochars possessed an amorphous porous structure with many functional groups consisting primarily of silicates. The adsorption rate of BR46 was evaluated using two kinetic models (pseudo-first-order and pseudo-second-order), and the results indicated that the pseudo-second-order model fitted to the experimental data well (R 2 >0.99). Nearly 24 h was sufficient to achieve equilibrium with the dye adsorption for the two biochars. R500 had a greater adsorption efficiency than B500. As pH levels increased, the dye’s adsorption capability increased as well. The Langmuir and Freundlich isotherm models were used to investigate the equilibrium behavior of BR46 adsorption, and the equilibrium data fitted well with the Langmuir model (R 2 >0.99) compared to the Freundlich model (R 2 >0.89). The maximum adsorption capacities of BR46 are 9.06 mg/g for B500 and 22.12 mg/g for R500, respectively. Additionally, adsorption capacity increased as temperature increased, indicating that adsorption is favored at higher temperatures. The electrostatic interaction is shown to be the dominant mechanism of BR46 adsorption, and BR46 acts as an electron-acceptor, contributing to n-π EDA (Electron Donor-Acceptor) interaction. Thermodynamic parameters for the dye-adsorbent system revealed that the adsorption process is spontaneous and feasible. The values of the adsorption coefficient (K d ) were on the order of 10 2 −10 3 . K d of R500 was greater than that of B500, indicating that R500 had a greater adsorption capacity. The results showed that R500 could be used as a low-cost alternative adsorbent for removing BR46 from effluents.
The primary purpose of this study is to eliminate Basic Red 46 dye from aqueous solutions utilizing batch experiments by adsorption on biochars prepared from bamboo and rice straw biomass. Biochars prepared from bamboo (B), and rice straw (R) was pyrolyzed at 500°C (B500 and R500). Scanning Electron Microscopy (SEM), Fourier Transform Infrared (FTIR) Spectroscopy, X-ray Diffraction (XRD), and surface area and porosity analyzers were used to characterize the B500 and R500 samples. The characterization results indicated that the biochars possessed an amorphous porous structure with many functional groups consisting primarily of silicates. The adsorption rate of BR46 was evaluated using two kinetic models (pseudo-first-order and pseudo-second-order), and the results indicated that the pseudo-second-order model fitted to the experimental data well (R2>0.99). Nearly 24 h was sufficient to achieve equilibrium with the dye adsorption for the two biochars. R500 had a greater adsorption efficiency than B500. As pH levels increased, the dye's adsorption capability increased as well. The Langmuir and Freundlich isotherm models were used to investigate the equilibrium behavior of BR46 adsorption, and the equilibrium data fitted well with the Langmuir model (R2>0.99) compared to the Freundlich model (R2>0.89). The maximum adsorption capacities of BR46 are 9.06 mg/g for B500 and 22.12 mg/g for R500, respectively. Additionally, adsorption capacity increased as temperature increased, indicating that adsorption is favored at higher temperatures. The electrostatic interaction is shown to be the dominant mechanism of BR46 adsorption, and BR46 acts as an electron-acceptor, contributing to n-π EDA (Electron Donor-Acceptor) interaction. Thermodynamic parameters for the dye-adsorbent system revealed that the adsorption process is spontaneous and feasible. The values of the adsorption coefficient (Kd) were on the order of 102-103. Kd of R500 was greater than that of B500, indicating that R500 had a greater adsorption capacity. The results showed that R500 could be used as a low-cost alternative adsorbent for removing BR46 from effluents.
The primary purpose of this study is to eliminate Basic Red 46 dye from aqueous solutions utilizing batch experiments by adsorption on biochars prepared from bamboo and rice straw biomass. Biochars prepared from bamboo (B), and rice straw (R) was pyrolyzed at 500°C (B500 and R500). Scanning Electron Microscopy (SEM), Fourier Transform Infrared (FTIR) Spectroscopy, X-ray Diffraction (XRD), and surface area and porosity analyzers were used to characterize the B500 and R500 samples. The characterization results indicated that the biochars possessed an amorphous porous structure with many functional groups consisting primarily of silicates. The adsorption rate of BR46 was evaluated using two kinetic models (pseudo-first-order and pseudo-second-order), and the results indicated that the pseudo-second-order model fitted to the experimental data well (R2>0.99). Nearly 24 h was sufficient to achieve equilibrium with the dye adsorption for the two biochars. R500 had a greater adsorption efficiency than B500. As pH levels increased, the dye's adsorption capability increased as well. The Langmuir and Freundlich isotherm models were used to investigate the equilibrium behavior of BR46 adsorption, and the equilibrium data fitted well with the Langmuir model (R2>0.99) compared to the Freundlich model (R2>0.89). The maximum adsorption capacities of BR46 are 9.06 mg/g for B500 and 22.12 mg/g for R500, respectively. Additionally, adsorption capacity increased as temperature increased, indicating that adsorption is favored at higher temperatures. The electrostatic interaction is shown to be the dominant mechanism of BR46 adsorption, and BR46 acts as an electron-acceptor, contributing to n-π EDA (Electron Donor-Acceptor) interaction. Thermodynamic parameters for the dye-adsorbent system revealed that the adsorption process is spontaneous and feasible. The values of the adsorption coefficient (Kd) were on the order of 102-103. Kd of R500 was greater than that of B500, indicating that R500 had a greater adsorption capacity. The results showed that R500 could be used as a low-cost alternative adsorbent for removing BR46 from effluents.The primary purpose of this study is to eliminate Basic Red 46 dye from aqueous solutions utilizing batch experiments by adsorption on biochars prepared from bamboo and rice straw biomass. Biochars prepared from bamboo (B), and rice straw (R) was pyrolyzed at 500°C (B500 and R500). Scanning Electron Microscopy (SEM), Fourier Transform Infrared (FTIR) Spectroscopy, X-ray Diffraction (XRD), and surface area and porosity analyzers were used to characterize the B500 and R500 samples. The characterization results indicated that the biochars possessed an amorphous porous structure with many functional groups consisting primarily of silicates. The adsorption rate of BR46 was evaluated using two kinetic models (pseudo-first-order and pseudo-second-order), and the results indicated that the pseudo-second-order model fitted to the experimental data well (R2>0.99). Nearly 24 h was sufficient to achieve equilibrium with the dye adsorption for the two biochars. R500 had a greater adsorption efficiency than B500. As pH levels increased, the dye's adsorption capability increased as well. The Langmuir and Freundlich isotherm models were used to investigate the equilibrium behavior of BR46 adsorption, and the equilibrium data fitted well with the Langmuir model (R2>0.99) compared to the Freundlich model (R2>0.89). The maximum adsorption capacities of BR46 are 9.06 mg/g for B500 and 22.12 mg/g for R500, respectively. Additionally, adsorption capacity increased as temperature increased, indicating that adsorption is favored at higher temperatures. The electrostatic interaction is shown to be the dominant mechanism of BR46 adsorption, and BR46 acts as an electron-acceptor, contributing to n-π EDA (Electron Donor-Acceptor) interaction. Thermodynamic parameters for the dye-adsorbent system revealed that the adsorption process is spontaneous and feasible. The values of the adsorption coefficient (Kd) were on the order of 102-103. Kd of R500 was greater than that of B500, indicating that R500 had a greater adsorption capacity. The results showed that R500 could be used as a low-cost alternative adsorbent for removing BR46 from effluents.
The primary purpose of this study is to eliminate Basic Red 46 dye from aqueous solutions utilizing batch experiments by adsorption on biochars prepared from bamboo and rice straw biomass. Biochars prepared from bamboo (B), and rice straw (R) was pyrolyzed at 500°C (B500 and R500). Scanning Electron Microscopy (SEM), Fourier Transform Infrared (FTIR) Spectroscopy, X-ray Diffraction (XRD), and surface area and porosity analyzers were used to characterize the B500 and R500 samples. The characterization results indicated that the biochars possessed an amorphous porous structure with many functional groups consisting primarily of silicates. The adsorption rate of BR46 was evaluated using two kinetic models (pseudo-first-order and pseudo-second-order), and the results indicated that the pseudo-second-order model fitted to the experimental data well (R.sup.2 >0.99). Nearly 24 h was sufficient to achieve equilibrium with the dye adsorption for the two biochars. R500 had a greater adsorption efficiency than B500. As pH levels increased, the dye's adsorption capability increased as well. The Langmuir and Freundlich isotherm models were used to investigate the equilibrium behavior of BR46 adsorption, and the equilibrium data fitted well with the Langmuir model (R.sup.2 >0.99) compared to the Freundlich model (R.sup.2 >0.89). The maximum adsorption capacities of BR46 are 9.06 mg/g for B500 and 22.12 mg/g for R500, respectively. Additionally, adsorption capacity increased as temperature increased, indicating that adsorption is favored at higher temperatures. The electrostatic interaction is shown to be the dominant mechanism of BR46 adsorption, and BR46 acts as an electron-acceptor, contributing to n-[qi] EDA (Electron Donor-Acceptor) interaction. Thermodynamic parameters for the dye-adsorbent system revealed that the adsorption process is spontaneous and feasible. The values of the adsorption coefficient (K.sub.d) were on the order of 10.sup.2 -10.sup.3 . K.sub.d of R500 was greater than that of B500, indicating that R500 had a greater adsorption capacity. The results showed that R500 could be used as a low-cost alternative adsorbent for removing BR46 from effluents.
Audience Academic
Author Sackey, Ebenezer Ampofo
Yu, Ya
Zhuang, Haifeng
Song, Yali
AuthorAffiliation 2 Key Laboratory of Recycling and Eco-Treatment of Waste Biomass of Zhejiang Province, Zhejiang University of Science and Technology, Hangzhou, Zhejiang, China
King Saud University, SAUDI ARABIA
1 School of Civil Engineering and Architecture, Zhejiang University of Science and Technology, Hangzhou, Zhejiang, China
AuthorAffiliation_xml – name: 1 School of Civil Engineering and Architecture, Zhejiang University of Science and Technology, Hangzhou, Zhejiang, China
– name: 2 Key Laboratory of Recycling and Eco-Treatment of Waste Biomass of Zhejiang Province, Zhejiang University of Science and Technology, Hangzhou, Zhejiang, China
– name: King Saud University, SAUDI ARABIA
Author_xml – sequence: 1
  givenname: Ebenezer Ampofo
  orcidid: 0000-0002-2713-3458
  surname: Sackey
  fullname: Sackey, Ebenezer Ampofo
– sequence: 2
  givenname: Yali
  surname: Song
  fullname: Song, Yali
– sequence: 3
  givenname: Ya
  surname: Yu
  fullname: Yu, Ya
– sequence: 4
  givenname: Haifeng
  surname: Zhuang
  fullname: Zhuang, Haifeng
BackLink https://www.ncbi.nlm.nih.gov/pubmed/34260652$$D View this record in MEDLINE/PubMed
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ContentType Journal Article
Copyright COPYRIGHT 2021 Public Library of Science
2021 Sackey et al. This is an open access article distributed under the terms of the Creative Commons Attribution License: http://creativecommons.org/licenses/by/4.0/ (the “License”), which permits unrestricted use, distribution, and reproduction in any medium, provided the original author and source are credited. Notwithstanding the ProQuest Terms and Conditions, you may use this content in accordance with the terms of the License.
2021 Sackey et al 2021 Sackey et al
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– notice: 2021 Sackey et al. This is an open access article distributed under the terms of the Creative Commons Attribution License: http://creativecommons.org/licenses/by/4.0/ (the “License”), which permits unrestricted use, distribution, and reproduction in any medium, provided the original author and source are credited. Notwithstanding the ProQuest Terms and Conditions, you may use this content in accordance with the terms of the License.
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DocumentTitleAlternate Biochars derived from bamboo and rice straw for sorption of basic red dyes
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Snippet The primary purpose of this study is to eliminate Basic Red 46 dye from aqueous solutions utilizing batch experiments by adsorption on biochars prepared from...
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SubjectTerms Activated carbon
Adsorbents
Adsorption
Analysis
Analyzers
Aqueous solutions
Azo Compounds
Bamboo
Biology and Life Sciences
Biomass
Charcoal
Civil engineering
Dyes
Dyes and dyeing
Earth Sciences
Ecology and Environmental Sciences
Effluents
Electron microscopy
Electrostatic properties
Equilibrium
Experiments
Fourier transforms
Functional groups
High temperature
Infrared analysis
Interaction parameters
Kinetics
Laboratories
Membrane separation
Organic chemicals
Oryza
Physical Sciences
Pollutants
Porosity
Properties
Research and Analysis Methods
Rice
Rice straw
Scanning electron microscopy
Silicates
Spectroscopy
Straw
Temperature rise
Thermodynamics
Water treatment
X-ray diffraction
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Title Biochars derived from bamboo and rice straw for sorption of basic red dyes
URI https://www.ncbi.nlm.nih.gov/pubmed/34260652
https://www.proquest.com/docview/2551563953
https://www.proquest.com/docview/2552060385
https://pubmed.ncbi.nlm.nih.gov/PMC8279399
https://doaj.org/article/62a0a9aa455149e2aaf9e155e221e715
http://dx.doi.org/10.1371/journal.pone.0254637
Volume 16
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