Cyclohexanedodecol-Assisted Interfacial Engineering for Robust and High-Performance Zinc Metal Anode
Highlights Cyclohexanedodecol (CHD) could facilitate the Zn dendrite-free plating/stripping at a nanoscale. The CHD molecules could effectively modify the hydrated Zn(H 2 O) 6 2+ structure in aqueous Zn ion batteries. The addition of CHD could establish robust protection layers on the Zn electrode s...
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| Published in | Nano-micro letters Vol. 14; no. 1; pp. 110 - 17 |
|---|---|
| Main Authors | , , , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Singapore
Springer Nature Singapore
01.12.2022
Springer Nature B.V SpringerOpen |
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| Abstract | Highlights
Cyclohexanedodecol (CHD) could facilitate the Zn dendrite-free plating/stripping at a nanoscale.
The CHD molecules could effectively modify the hydrated Zn(H
2
O)
6
2+
structure in aqueous Zn ion batteries.
The addition of CHD could establish robust protection layers on the Zn electrode surface.
The CHD-modified electrolytes exhibit long-term cycling stability.
Aqueous zinc-ion batteries (AZIBs) can be one of the most promising electrochemical energy storage devices for being non-flammable, low-cost, and sustainable. However, the challenges of AZIBs, including dendrite growth, hydrogen evolution, corrosion, and passivation of zinc anode during charging and discharging processes, must be overcome to achieve high cycling performance and stability in practical applications. In this work, we utilize a dual-functional organic additive cyclohexanedodecol (CHD) to firstly establish [Zn(H
2
O)
5
(CHD)]
2+
complex ion in an aqueous Zn electrolyte and secondly build a robust protection layer on the Zn surface to overcome these dilemmas. Systematic experiments and theoretical calculations are carried out to interpret the working mechanism of CHD. At a very low concentration of 0.1 mg mL
−1
CHD, long-term reversible Zn plating/stripping could be achieved up to 2200 h at 2 mA cm
−2
, 1000 h at 5 mA cm
−2
, and 650 h at 10 mA cm
−2
at the fixed capacity of 1 mAh cm
−2
. When matched with V
2
O
5
cathode, the resultant AZIBs full cell with the CHD-modified electrolyte presents a high capacity of 175 mAh g
−1
with the capacity retention of 92% after 2000 cycles under 2 A g
−1
. Such a performance could enable the commercialization of AZIBs for applications in grid energy storage and industrial energy storage. |
|---|---|
| AbstractList | Aqueous zinc-ion batteries (AZIBs) can be one of the most promising electrochemical energy storage devices for being non-flammable, low-cost, and sustainable. However, the challenges of AZIBs, including dendrite growth, hydrogen evolution, corrosion, and passivation of zinc anode during charging and discharging processes, must be overcome to achieve high cycling performance and stability in practical applications. In this work, we utilize a dual-functional organic additive cyclohexanedodecol (CHD) to firstly establish [Zn(H2O)5(CHD)]2+ complex ion in an aqueous Zn electrolyte and secondly build a robust protection layer on the Zn surface to overcome these dilemmas. Systematic experiments and theoretical calculations are carried out to interpret the working mechanism of CHD. At a very low concentration of 0.1 mg mL-1 CHD, long-term reversible Zn plating/stripping could be achieved up to 2200 h at 2 mA cm-2, 1000 h at 5 mA cm-2, and 650 h at 10 mA cm-2 at the fixed capacity of 1 mAh cm-2. When matched with V2O5 cathode, the resultant AZIBs full cell with the CHD-modified electrolyte presents a high capacity of 175 mAh g-1 with the capacity retention of 92% after 2000 cycles under 2 A g-1. Such a performance could enable the commercialization of AZIBs for applications in grid energy storage and industrial energy storage.Aqueous zinc-ion batteries (AZIBs) can be one of the most promising electrochemical energy storage devices for being non-flammable, low-cost, and sustainable. However, the challenges of AZIBs, including dendrite growth, hydrogen evolution, corrosion, and passivation of zinc anode during charging and discharging processes, must be overcome to achieve high cycling performance and stability in practical applications. In this work, we utilize a dual-functional organic additive cyclohexanedodecol (CHD) to firstly establish [Zn(H2O)5(CHD)]2+ complex ion in an aqueous Zn electrolyte and secondly build a robust protection layer on the Zn surface to overcome these dilemmas. Systematic experiments and theoretical calculations are carried out to interpret the working mechanism of CHD. At a very low concentration of 0.1 mg mL-1 CHD, long-term reversible Zn plating/stripping could be achieved up to 2200 h at 2 mA cm-2, 1000 h at 5 mA cm-2, and 650 h at 10 mA cm-2 at the fixed capacity of 1 mAh cm-2. When matched with V2O5 cathode, the resultant AZIBs full cell with the CHD-modified electrolyte presents a high capacity of 175 mAh g-1 with the capacity retention of 92% after 2000 cycles under 2 A g-1. Such a performance could enable the commercialization of AZIBs for applications in grid energy storage and industrial energy storage. Aqueous zinc-ion batteries (AZIBs) can be one of the most promising electrochemical energy storage devices for being non-flammable, low-cost, and sustainable. However, the challenges of AZIBs, including dendrite growth, hydrogen evolution, corrosion, and passivation of zinc anode during charging and discharging processes, must be overcome to achieve high cycling performance and stability in practical applications. In this work, we utilize a dual-functional organic additive cyclohexanedodecol (CHD) to firstly establish [Zn(H 2 O) 5 (CHD)] 2+ complex ion in an aqueous Zn electrolyte and secondly build a robust protection layer on the Zn surface to overcome these dilemmas. Systematic experiments and theoretical calculations are carried out to interpret the working mechanism of CHD. At a very low concentration of 0.1 mg mL −1 CHD, long-term reversible Zn plating/stripping could be achieved up to 2200 h at 2 mA cm −2 , 1000 h at 5 mA cm −2 , and 650 h at 10 mA cm −2 at the fixed capacity of 1 mAh cm −2 . When matched with V 2 O 5 cathode, the resultant AZIBs full cell with the CHD-modified electrolyte presents a high capacity of 175 mAh g −1 with the capacity retention of 92% after 2000 cycles under 2 A g −1 . Such a performance could enable the commercialization of AZIBs for applications in grid energy storage and industrial energy storage. HighlightsCyclohexanedodecol (CHD) could facilitate the Zn dendrite-free plating/stripping at a nanoscale.The CHD molecules could effectively modify the hydrated Zn(H2O)62+ structure in aqueous Zn ion batteries.The addition of CHD could establish robust protection layers on the Zn electrode surface.The CHD-modified electrolytes exhibit long-term cycling stability.Aqueous zinc-ion batteries (AZIBs) can be one of the most promising electrochemical energy storage devices for being non-flammable, low-cost, and sustainable. However, the challenges of AZIBs, including dendrite growth, hydrogen evolution, corrosion, and passivation of zinc anode during charging and discharging processes, must be overcome to achieve high cycling performance and stability in practical applications. In this work, we utilize a dual-functional organic additive cyclohexanedodecol (CHD) to firstly establish [Zn(H2O)5(CHD)]2+ complex ion in an aqueous Zn electrolyte and secondly build a robust protection layer on the Zn surface to overcome these dilemmas. Systematic experiments and theoretical calculations are carried out to interpret the working mechanism of CHD. At a very low concentration of 0.1 mg mL−1 CHD, long-term reversible Zn plating/stripping could be achieved up to 2200 h at 2 mA cm−2, 1000 h at 5 mA cm−2, and 650 h at 10 mA cm−2 at the fixed capacity of 1 mAh cm−2. When matched with V2O5 cathode, the resultant AZIBs full cell with the CHD-modified electrolyte presents a high capacity of 175 mAh g−1 with the capacity retention of 92% after 2000 cycles under 2 A g−1. Such a performance could enable the commercialization of AZIBs for applications in grid energy storage and industrial energy storage. Abstract Aqueous zinc-ion batteries (AZIBs) can be one of the most promising electrochemical energy storage devices for being non-flammable, low-cost, and sustainable. However, the challenges of AZIBs, including dendrite growth, hydrogen evolution, corrosion, and passivation of zinc anode during charging and discharging processes, must be overcome to achieve high cycling performance and stability in practical applications. In this work, we utilize a dual-functional organic additive cyclohexanedodecol (CHD) to firstly establish [Zn(H2O)5(CHD)]2+ complex ion in an aqueous Zn electrolyte and secondly build a robust protection layer on the Zn surface to overcome these dilemmas. Systematic experiments and theoretical calculations are carried out to interpret the working mechanism of CHD. At a very low concentration of 0.1 mg mL−1 CHD, long-term reversible Zn plating/stripping could be achieved up to 2200 h at 2 mA cm−2, 1000 h at 5 mA cm−2, and 650 h at 10 mA cm−2 at the fixed capacity of 1 mAh cm−2. When matched with V2O5 cathode, the resultant AZIBs full cell with the CHD-modified electrolyte presents a high capacity of 175 mAh g−1 with the capacity retention of 92% after 2000 cycles under 2 A g−1. Such a performance could enable the commercialization of AZIBs for applications in grid energy storage and industrial energy storage. Highlights Cyclohexanedodecol (CHD) could facilitate the Zn dendrite-free plating/stripping at a nanoscale. The CHD molecules could effectively modify the hydrated Zn(H 2 O) 6 2+ structure in aqueous Zn ion batteries. The addition of CHD could establish robust protection layers on the Zn electrode surface. The CHD-modified electrolytes exhibit long-term cycling stability. Aqueous zinc-ion batteries (AZIBs) can be one of the most promising electrochemical energy storage devices for being non-flammable, low-cost, and sustainable. However, the challenges of AZIBs, including dendrite growth, hydrogen evolution, corrosion, and passivation of zinc anode during charging and discharging processes, must be overcome to achieve high cycling performance and stability in practical applications. In this work, we utilize a dual-functional organic additive cyclohexanedodecol (CHD) to firstly establish [Zn(H 2 O) 5 (CHD)] 2+ complex ion in an aqueous Zn electrolyte and secondly build a robust protection layer on the Zn surface to overcome these dilemmas. Systematic experiments and theoretical calculations are carried out to interpret the working mechanism of CHD. At a very low concentration of 0.1 mg mL −1 CHD, long-term reversible Zn plating/stripping could be achieved up to 2200 h at 2 mA cm −2 , 1000 h at 5 mA cm −2 , and 650 h at 10 mA cm −2 at the fixed capacity of 1 mAh cm −2 . When matched with V 2 O 5 cathode, the resultant AZIBs full cell with the CHD-modified electrolyte presents a high capacity of 175 mAh g −1 with the capacity retention of 92% after 2000 cycles under 2 A g −1 . Such a performance could enable the commercialization of AZIBs for applications in grid energy storage and industrial energy storage. Cyclohexanedodecol (CHD) could facilitate the Zn dendrite-free plating/stripping at a nanoscale. The CHD molecules could effectively modify the hydrated Zn(H 2 O) 6 2+ structure in aqueous Zn ion batteries. The addition of CHD could establish robust protection layers on the Zn electrode surface. The CHD-modified electrolytes exhibit long-term cycling stability. Aqueous zinc-ion batteries (AZIBs) can be one of the most promising electrochemical energy storage devices for being non-flammable, low-cost, and sustainable. However, the challenges of AZIBs, including dendrite growth, hydrogen evolution, corrosion, and passivation of zinc anode during charging and discharging processes, must be overcome to achieve high cycling performance and stability in practical applications. In this work, we utilize a dual-functional organic additive cyclohexanedodecol (CHD) to firstly establish [Zn(H 2 O) 5 (CHD)] 2+ complex ion in an aqueous Zn electrolyte and secondly build a robust protection layer on the Zn surface to overcome these dilemmas. Systematic experiments and theoretical calculations are carried out to interpret the working mechanism of CHD. At a very low concentration of 0.1 mg mL −1 CHD, long-term reversible Zn plating/stripping could be achieved up to 2200 h at 2 mA cm −2 , 1000 h at 5 mA cm −2 , and 650 h at 10 mA cm −2 at the fixed capacity of 1 mAh cm −2 . When matched with V 2 O 5 cathode, the resultant AZIBs full cell with the CHD-modified electrolyte presents a high capacity of 175 mAh g −1 with the capacity retention of 92% after 2000 cycles under 2 A g −1 . Such a performance could enable the commercialization of AZIBs for applications in grid energy storage and industrial energy storage. Aqueous zinc-ion batteries (AZIBs) can be one of the most promising electrochemical energy storage devices for being non-flammable, low-cost, and sustainable. However, the challenges of AZIBs, including dendrite growth, hydrogen evolution, corrosion, and passivation of zinc anode during charging and discharging processes, must be overcome to achieve high cycling performance and stability in practical applications. In this work, we utilize a dual-functional organic additive cyclohexanedodecol (CHD) to firstly establish [Zn(H O) (CHD)] complex ion in an aqueous Zn electrolyte and secondly build a robust protection layer on the Zn surface to overcome these dilemmas. Systematic experiments and theoretical calculations are carried out to interpret the working mechanism of CHD. At a very low concentration of 0.1 mg mL CHD, long-term reversible Zn plating/stripping could be achieved up to 2200 h at 2 mA cm , 1000 h at 5 mA cm , and 650 h at 10 mA cm at the fixed capacity of 1 mAh cm . When matched with V O cathode, the resultant AZIBs full cell with the CHD-modified electrolyte presents a high capacity of 175 mAh g with the capacity retention of 92% after 2000 cycles under 2 A g . Such a performance could enable the commercialization of AZIBs for applications in grid energy storage and industrial energy storage. |
| ArticleNumber | 110 |
| Author | Lai, Chao Zhang, Shao-Jian Wu, Zhenzhen Sun, Chuang Li, Meng Zhang, Shanqing Tian, Yuhui Li, Chengpeng Lin, Zhan Chen, Hao Kiefel, Milton |
| Author_xml | – sequence: 1 givenname: Zhenzhen surname: Wu fullname: Wu, Zhenzhen organization: Centre for Clean Environment and Energy, School of Environment and Science, Griffith University – sequence: 2 givenname: Meng surname: Li fullname: Li, Meng organization: Centre for Clean Environment and Energy, School of Environment and Science, Griffith University – sequence: 3 givenname: Yuhui surname: Tian fullname: Tian, Yuhui organization: Centre for Clean Environment and Energy, School of Environment and Science, Griffith University – sequence: 4 givenname: Hao surname: Chen fullname: Chen, Hao organization: Centre for Clean Environment and Energy, School of Environment and Science, Griffith University – sequence: 5 givenname: Shao-Jian surname: Zhang fullname: Zhang, Shao-Jian organization: Guangzhou Key Laboratory of Clean Transportation Energy Chemistry, School of Chemical Engineering and Light Industry, Guangdong University of Technology – sequence: 6 givenname: Chuang surname: Sun fullname: Sun, Chuang organization: School of Chemistry and Materials Science, Jiangsu Normal University – sequence: 7 givenname: Chengpeng surname: Li fullname: Li, Chengpeng organization: Institute for Glycomics, Griffith University – sequence: 8 givenname: Milton surname: Kiefel fullname: Kiefel, Milton organization: Institute for Glycomics, Griffith University – sequence: 9 givenname: Chao surname: Lai fullname: Lai, Chao organization: School of Chemistry and Materials Science, Jiangsu Normal University – sequence: 10 givenname: Zhan surname: Lin fullname: Lin, Zhan email: zhanlin@gdut.edu.cn organization: Guangzhou Key Laboratory of Clean Transportation Energy Chemistry, School of Chemical Engineering and Light Industry, Guangdong University of Technology – sequence: 11 givenname: Shanqing surname: Zhang fullname: Zhang, Shanqing email: s.zhang@griffith.edu.au organization: Centre for Clean Environment and Energy, School of Environment and Science, Griffith University |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/35441329$$D View this record in MEDLINE/PubMed |
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| Keywords | Zn dendrite Cyclohexanedodecol Aqueous Zn-ion battery Zn corrosion Hydrogen evolution |
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| Snippet | Highlights
Cyclohexanedodecol (CHD) could facilitate the Zn dendrite-free plating/stripping at a nanoscale.
The CHD molecules could effectively modify the... Aqueous zinc-ion batteries (AZIBs) can be one of the most promising electrochemical energy storage devices for being non-flammable, low-cost, and sustainable.... HighlightsCyclohexanedodecol (CHD) could facilitate the Zn dendrite-free plating/stripping at a nanoscale.The CHD molecules could effectively modify the... Cyclohexanedodecol (CHD) could facilitate the Zn dendrite-free plating/stripping at a nanoscale. The CHD molecules could effectively modify the hydrated Zn(H 2... Abstract Aqueous zinc-ion batteries (AZIBs) can be one of the most promising electrochemical energy storage devices for being non-flammable, low-cost, and... |
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| SubjectTerms | Anodes Aqueous Zn-ion battery Commercialization Cycles Cyclohexanedodecol Dendritic structure Electrolytes Energy storage Engineering Flammability Hydrogen evolution Industrial energy Nanoscale Science and Technology Nanotechnology Nanotechnology and Microengineering Plating Rechargeable batteries Robustness Storage batteries Zinc Zinc Anodes Zn corrosion Zn dendrite |
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| Title | Cyclohexanedodecol-Assisted Interfacial Engineering for Robust and High-Performance Zinc Metal Anode |
| URI | https://link.springer.com/article/10.1007/s40820-022-00846-0 https://www.ncbi.nlm.nih.gov/pubmed/35441329 https://www.proquest.com/docview/2656121949 https://www.proquest.com/docview/2652865374 https://pubmed.ncbi.nlm.nih.gov/PMC9019003 https://doaj.org/article/0d5c0c104a014845ba97ed467191cdbf |
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