Facile Solid-State Growth of 3D Well-Interconnected Nitrogen-Rich Carbon Nanotube-Graphene Hybrid Architectures for Lithium-Sulfur Batteries
Constructing 3D carbon structures built from carbon nanotubes (CNTs) and graphene has been considered as an effective approach to achieve superior properties in energy conversion and storage because of the synergistic combination of the advantages of each building block. Herein, a facile solid‐state...
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| Published in | Advanced functional materials Vol. 26; no. 7; pp. 1112 - 1119 |
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| Main Authors | , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Blackwell Publishing Ltd
16.02.2016
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| Subjects | |
| Online Access | Get full text |
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| Abstract | Constructing 3D carbon structures built from carbon nanotubes (CNTs) and graphene has been considered as an effective approach to achieve superior properties in energy conversion and storage because of the synergistic combination of the advantages of each building block. Herein, a facile solid‐state growth strategy is reported for the first time to fabricate highly nitrogen doped CNT–graphene 3D nanostructures without the necessity to use chemical vapor deposition. As cathode hosts for lithium–sulfur batteries, the hybrid architectures exhibit reversible capacities of 1314 and 922 mAh g−1 at 0.2 and 1 C, respectively, and a capacity retention of 97% after 200 cycles at a high rate of 2 C, revealing their great potential for energy storage application.
Using a facile and green solid‐state growth strategy, 3D, well‐interconnected, highly nitrogen‐doped carbon nanotube–graphene hybrid structures are designed and fabricated by using Ni foam as growth substrate and catalyst, glucose as carbon sources, and dicyandiamide as nitrogen sources. When used as cathode hosts for Li–S batteries, the obtained product shows superior lithium‐storage capability. |
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| AbstractList | Constructing 3D carbon structures built from carbon nanotubes (CNTs) and graphene has been considered as an effective approach to achieve superior properties in energy conversion and storage because of the synergistic combination of the advantages of each building block. Herein, a facile solid‐state growth strategy is reported for the first time to fabricate highly nitrogen doped CNT–graphene 3D nanostructures without the necessity to use chemical vapor deposition. As cathode hosts for lithium–sulfur batteries, the hybrid architectures exhibit reversible capacities of 1314 and 922 mAh g
−1
at 0.2 and 1 C, respectively, and a capacity retention of 97% after 200 cycles at a high rate of 2 C, revealing their great potential for energy storage application. Constructing 3D carbon structures built from carbon nanotubes (CNTs) and graphene has been considered as an effective approach to achieve superior properties in energy conversion and storage because of the synergistic combination of the advantages of each building block. Herein, a facile solid-state growth strategy is reported for the first time to fabricate highly nitrogen doped CNT-graphene 3D nanostructures without the necessity to use chemical vapor deposition. As cathode hosts for lithium-sulfur batteries, the hybrid architectures exhibit reversible capacities of 1314 and 922 mAh g super(-1) at 0.2 and 1 C, respectively, and a capacity retention of 97% after 200 cycles at a high rate of 2 C, revealing their great potential for energy storage application. Using a facile and green solid-state growth strategy, 3D, well-interconnected, highly nitrogen-doped carbon nanotube-graphene hybrid structures are designed and fabricated by using Ni foam as growth substrate and catalyst, glucose as carbon sources, and dicyandiamide as nitrogen sources. When used as cathode hosts for Li-S batteries, the obtained product shows superior lithium-storage capability. Constructing 3D carbon structures built from carbon nanotubes (CNTs) and graphene has been considered as an effective approach to achieve superior properties in energy conversion and storage because of the synergistic combination of the advantages of each building block. Herein, a facile solid‐state growth strategy is reported for the first time to fabricate highly nitrogen doped CNT–graphene 3D nanostructures without the necessity to use chemical vapor deposition. As cathode hosts for lithium–sulfur batteries, the hybrid architectures exhibit reversible capacities of 1314 and 922 mAh g−1 at 0.2 and 1 C, respectively, and a capacity retention of 97% after 200 cycles at a high rate of 2 C, revealing their great potential for energy storage application. Using a facile and green solid‐state growth strategy, 3D, well‐interconnected, highly nitrogen‐doped carbon nanotube–graphene hybrid structures are designed and fabricated by using Ni foam as growth substrate and catalyst, glucose as carbon sources, and dicyandiamide as nitrogen sources. When used as cathode hosts for Li–S batteries, the obtained product shows superior lithium‐storage capability. |
| Author | Ding, Yuan-Li Maier, Joachim Yu, Yan Kopold, Peter Hahn, Kersten van Aken, Peter A. |
| Author_xml | – sequence: 1 givenname: Yuan-Li surname: Ding fullname: Ding, Yuan-Li organization: Max Planck Institute for Solid State Research, Heisenbergstrasse 1, 70569, Stuttgart, Germany – sequence: 2 givenname: Peter surname: Kopold fullname: Kopold, Peter organization: Max Planck Institute for Solid State Research, Heisenbergstrasse 1, 70569, Stuttgart, Germany – sequence: 3 givenname: Kersten surname: Hahn fullname: Hahn, Kersten organization: Max Planck Institute for Solid State Research, Heisenbergstrasse 1, 70569, Stuttgart, Germany – sequence: 4 givenname: Peter A. surname: van Aken fullname: van Aken, Peter A. organization: Max Planck Institute for Solid State Research, Heisenbergstrasse 1, 70569, Stuttgart, Germany – sequence: 5 givenname: Joachim surname: Maier fullname: Maier, Joachim organization: Max Planck Institute for Solid State Research, Heisenbergstrasse 1, 70569, Stuttgart, Germany – sequence: 6 givenname: Yan surname: Yu fullname: Yu, Yan email: yanyumse@ustc.edu.cn organization: Max Planck Institute for Solid State Research, Heisenbergstrasse 1, 70569, Stuttgart, Germany |
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| Copyright | 2015 WILEY‐VCH Verlag GmbH & Co. KGaA, Weinheim |
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| Notes | Alexander von Humboldt Foundation New Century Excellent Talents in University - No. NCET-12-0515 Collaborative Innovation Center of Suzhou Nano Science and Technology istex:23076938E15582D4F85CC2283207EC7C61B698DC European Union Seventh Framework Programme - No. FP7/2007-2013; No. 312483 ArticleID:ADFM201504294 ark:/67375/WNG-0Q414394-H Recruitment Program of Global Experts Fundamental Research Funds for the Central Universities - No. WK2060140014; No. WK2060140016 National Natural Science Foundation of China - No. 21171015; No. 21373195 ObjectType-Article-1 SourceType-Scholarly Journals-1 ObjectType-Feature-2 content type line 23 |
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| PublicationDate | February 16, 2016 |
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| PublicationTitle | Advanced functional materials |
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| Publisher | Blackwell Publishing Ltd |
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| Title | Facile Solid-State Growth of 3D Well-Interconnected Nitrogen-Rich Carbon Nanotube-Graphene Hybrid Architectures for Lithium-Sulfur Batteries |
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