Metal-Organic Framework-Derived Honeycomb-Like Open Porous Nanostructures as Precious-Metal-Free Catalysts for Highly Efficient Oxygen Electroreduction
Honeycomb‐like porous carbon nanostructures are rationally constructed from a metal–organic framework composite. The unique architecture with uniformly distributed high‐density active sites significantly enhances the electrocatalytic performance by increasing the accessible active sites and enhancin...
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| Published in | Advanced materials (Weinheim) Vol. 28; no. 30; pp. 6391 - 6398 |
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| Main Authors | , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Germany
Blackwell Publishing Ltd
01.08.2016
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| Subjects | |
| Online Access | Get full text |
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| Abstract | Honeycomb‐like porous carbon nanostructures are rationally constructed from a metal–organic framework composite. The unique architecture with uniformly distributed high‐density active sites significantly enhances the electrocatalytic performance by increasing the accessible active sites and enhancing mass transport of the gas and electrolyte, rendering the resulting catalyst adequate in reaching the desired catalytic performance afforded by Pt for the oxygen reduction reaction. |
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| AbstractList | Honeycomb-like porous carbon nanostructures are rationally constructed from a metal-organic framework composite. The unique architecture with uniformly distributed high-density active sites significantly enhances the electrocatalytic performance by increasing the accessible active sites and enhancing mass transport of the gas and electrolyte, rendering the resulting catalyst adequate in reaching the desired catalytic performance afforded by Pt for the oxygen reduction reaction.Honeycomb-like porous carbon nanostructures are rationally constructed from a metal-organic framework composite. The unique architecture with uniformly distributed high-density active sites significantly enhances the electrocatalytic performance by increasing the accessible active sites and enhancing mass transport of the gas and electrolyte, rendering the resulting catalyst adequate in reaching the desired catalytic performance afforded by Pt for the oxygen reduction reaction. Honeycomb‐like porous carbon nanostructures are rationally constructed from a metal–organic framework composite. The unique architecture with uniformly distributed high‐density active sites significantly enhances the electrocatalytic performance by increasing the accessible active sites and enhancing mass transport of the gas and electrolyte, rendering the resulting catalyst adequate in reaching the desired catalytic performance afforded by Pt for the oxygen reduction reaction. |
| Author | Xia, Wei Akita, Tomoki Xu, Qiang Zhu, Qi-Long Zou, Ruqiang |
| Author_xml | – sequence: 1 givenname: Qi-Long surname: Zhu fullname: Zhu, Qi-Long organization: National Institute of Advanced Industrial Science and Technology (AIST), Osaka, 563-8577, Ikeda, Japan – sequence: 2 givenname: Wei surname: Xia fullname: Xia, Wei organization: Beijing Key Lab of Theory and Technology for Advanced Battery Materials, Department of Material Science and Engineering, College of Engineering, Peking University, 100871, Beijing, China – sequence: 3 givenname: Tomoki surname: Akita fullname: Akita, Tomoki organization: National Institute of Advanced Industrial Science and Technology (AIST), Osaka, 563-8577, Ikeda, Japan – sequence: 4 givenname: Ruqiang surname: Zou fullname: Zou, Ruqiang email: rzou@pku.edu.cn organization: Beijing Key Lab of Theory and Technology for Advanced Battery Materials, Department of Material Science and Engineering, College of Engineering, Peking University, 100871, Beijing, China – sequence: 5 givenname: Qiang surname: Xu fullname: Xu, Qiang email: rzou@pku.edu.cn organization: National Institute of Advanced Industrial Science and Technology (AIST), Osaka, 563-8577, Ikeda, Japan |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/27166878$$D View this record in MEDLINE/PubMed |
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| Snippet | Honeycomb‐like porous carbon nanostructures are rationally constructed from a metal–organic framework composite. The unique architecture with uniformly... Honeycomb-like porous carbon nanostructures are rationally constructed from a metal-organic framework composite. The unique architecture with uniformly... |
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| SubjectTerms | Accessibility Carbon Catalysis Catalysts cobalt sulfide metal-organic frameworks Nanostructure Oxygen oxygen reduction porous carbon Reduction (electrolytic) Rendering |
| Title | Metal-Organic Framework-Derived Honeycomb-Like Open Porous Nanostructures as Precious-Metal-Free Catalysts for Highly Efficient Oxygen Electroreduction |
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