Alloying effect on the order–disorder transformation in tetragonal FeNi
Tetragonal ( L1 0 ) FeNi is a promising material for high-performance rare-earth-free permanent magnets. Pure tetragonal FeNi is very difficult to synthesize due to its low chemical order–disorder transition temperature ( ≈ 593 K), and thus one must consider alternative non-equilibrium processing r...
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| Published in | Scientific reports Vol. 11; no. 1; pp. 5253 - 9 |
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| Main Authors | , , , |
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04.03.2021
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| Abstract | Tetragonal (
L1
0
) FeNi is a promising material for high-performance rare-earth-free permanent magnets. Pure tetragonal FeNi is very difficult to synthesize due to its low chemical order–disorder transition temperature (
≈
593
K), and thus one must consider alternative non-equilibrium processing routes and alloy design strategies that make the formation of tetragonal FeNi feasible. In this paper, we investigate by density functional theory as implemented in the exact muffin-tin orbitals method whether alloying FeNi with a suitable element can have a positive impact on the phase formation and ordering properties while largely maintaining its attractive intrinsic magnetic properties. We find that small amount of non-magnetic (Al and Ti) or magnetic (Cr and Co) elements increase the order–disorder transition temperature. Adding Mo to the Co-doped system further enhances the ordering temperature while the Curie temperature is decreased only by a few degrees. Our results show that alloying is a viable route to stabilizing the ordered tetragonal phase of FeNi. |
|---|---|
| AbstractList | Tetragonal (L10) FeNi is a promising material for high-performance rare-earth-free permanent magnets. Pure tetragonal FeNi is very difficult to synthesize due to its low chemical order-disorder transition temperature (approximate to 593 K), and thus one must consider alternative non-equilibrium processing routes and alloy design strategies that make the formation of tetragonal FeNi feasible. In this paper, we investigate by density functional theory as implemented in the exact muffin-tin orbitals method whether alloying FeNi with a suitable element can have a positive impact on the phase formation and ordering properties while largely maintaining its attractive intrinsic magnetic properties. We find that small amount of non-magnetic (Al and Ti) or magnetic (Cr and Co) elements increase the order-disorder transition temperature. Adding Mo to the Co-doped system further enhances the ordering temperature while the Curie temperature is decreased only by a few degrees. Our results show that alloying is a viable route to stabilizing the ordered tetragonal phase of FeNi. Tetragonal ( \documentclass[12pt]{minimal} \usepackage{amsmath} \usepackage{wasysym} \usepackage{amsfonts} \usepackage{amssymb} \usepackage{amsbsy} \usepackage{mathrsfs} \usepackage{upgreek} \setlength{\oddsidemargin}{-69pt} \begin{document}$${\hbox{L1}}_{0}$$\end{document} L1 0 ) FeNi is a promising material for high-performance rare-earth-free permanent magnets. Pure tetragonal FeNi is very difficult to synthesize due to its low chemical order–disorder transition temperature ( \documentclass[12pt]{minimal} \usepackage{amsmath} \usepackage{wasysym} \usepackage{amsfonts} \usepackage{amssymb} \usepackage{amsbsy} \usepackage{mathrsfs} \usepackage{upgreek} \setlength{\oddsidemargin}{-69pt} \begin{document}$$\approx {593}$$\end{document} ≈ 593 K), and thus one must consider alternative non-equilibrium processing routes and alloy design strategies that make the formation of tetragonal FeNi feasible. In this paper, we investigate by density functional theory as implemented in the exact muffin-tin orbitals method whether alloying FeNi with a suitable element can have a positive impact on the phase formation and ordering properties while largely maintaining its attractive intrinsic magnetic properties. We find that small amount of non-magnetic (Al and Ti) or magnetic (Cr and Co) elements increase the order–disorder transition temperature. Adding Mo to the Co-doped system further enhances the ordering temperature while the Curie temperature is decreased only by a few degrees. Our results show that alloying is a viable route to stabilizing the ordered tetragonal phase of FeNi. Tetragonal ( L1 0 ) FeNi is a promising material for high-performance rare-earth-free permanent magnets. Pure tetragonal FeNi is very difficult to synthesize due to its low chemical order–disorder transition temperature ( ≈ 593 K), and thus one must consider alternative non-equilibrium processing routes and alloy design strategies that make the formation of tetragonal FeNi feasible. In this paper, we investigate by density functional theory as implemented in the exact muffin-tin orbitals method whether alloying FeNi with a suitable element can have a positive impact on the phase formation and ordering properties while largely maintaining its attractive intrinsic magnetic properties. We find that small amount of non-magnetic (Al and Ti) or magnetic (Cr and Co) elements increase the order–disorder transition temperature. Adding Mo to the Co-doped system further enhances the ordering temperature while the Curie temperature is decreased only by a few degrees. Our results show that alloying is a viable route to stabilizing the ordered tetragonal phase of FeNi. Tetragonal ([Formula: see text]) FeNi is a promising material for high-performance rare-earth-free permanent magnets. Pure tetragonal FeNi is very difficult to synthesize due to its low chemical order-disorder transition temperature ([Formula: see text] K), and thus one must consider alternative non-equilibrium processing routes and alloy design strategies that make the formation of tetragonal FeNi feasible. In this paper, we investigate by density functional theory as implemented in the exact muffin-tin orbitals method whether alloying FeNi with a suitable element can have a positive impact on the phase formation and ordering properties while largely maintaining its attractive intrinsic magnetic properties. We find that small amount of non-magnetic (Al and Ti) or magnetic (Cr and Co) elements increase the order-disorder transition temperature. Adding Mo to the Co-doped system further enhances the ordering temperature while the Curie temperature is decreased only by a few degrees. Our results show that alloying is a viable route to stabilizing the ordered tetragonal phase of FeNi. Tetragonal ( $${\hbox{L1}}_{0}$$ L1 0 ) FeNi is a promising material for high-performance rare-earth-free permanent magnets. Pure tetragonal FeNi is very difficult to synthesize due to its low chemical order–disorder transition temperature ( $$\approx {593}$$ ≈ 593 K), and thus one must consider alternative non-equilibrium processing routes and alloy design strategies that make the formation of tetragonal FeNi feasible. In this paper, we investigate by density functional theory as implemented in the exact muffin-tin orbitals method whether alloying FeNi with a suitable element can have a positive impact on the phase formation and ordering properties while largely maintaining its attractive intrinsic magnetic properties. We find that small amount of non-magnetic (Al and Ti) or magnetic (Cr and Co) elements increase the order–disorder transition temperature. Adding Mo to the Co-doped system further enhances the ordering temperature while the Curie temperature is decreased only by a few degrees. Our results show that alloying is a viable route to stabilizing the ordered tetragonal phase of FeNi. Tetragonal ([Formula: see text]) FeNi is a promising material for high-performance rare-earth-free permanent magnets. Pure tetragonal FeNi is very difficult to synthesize due to its low chemical order-disorder transition temperature ([Formula: see text] K), and thus one must consider alternative non-equilibrium processing routes and alloy design strategies that make the formation of tetragonal FeNi feasible. In this paper, we investigate by density functional theory as implemented in the exact muffin-tin orbitals method whether alloying FeNi with a suitable element can have a positive impact on the phase formation and ordering properties while largely maintaining its attractive intrinsic magnetic properties. We find that small amount of non-magnetic (Al and Ti) or magnetic (Cr and Co) elements increase the order-disorder transition temperature. Adding Mo to the Co-doped system further enhances the ordering temperature while the Curie temperature is decreased only by a few degrees. Our results show that alloying is a viable route to stabilizing the ordered tetragonal phase of FeNi.Tetragonal ([Formula: see text]) FeNi is a promising material for high-performance rare-earth-free permanent magnets. Pure tetragonal FeNi is very difficult to synthesize due to its low chemical order-disorder transition temperature ([Formula: see text] K), and thus one must consider alternative non-equilibrium processing routes and alloy design strategies that make the formation of tetragonal FeNi feasible. In this paper, we investigate by density functional theory as implemented in the exact muffin-tin orbitals method whether alloying FeNi with a suitable element can have a positive impact on the phase formation and ordering properties while largely maintaining its attractive intrinsic magnetic properties. We find that small amount of non-magnetic (Al and Ti) or magnetic (Cr and Co) elements increase the order-disorder transition temperature. Adding Mo to the Co-doped system further enhances the ordering temperature while the Curie temperature is decreased only by a few degrees. Our results show that alloying is a viable route to stabilizing the ordered tetragonal phase of FeNi. Tetragonal (L10) FeNi is a promising material for high-performance rare-earth-free permanent magnets. Pure tetragonal FeNi is very difficult to synthesize due to its low chemical order–disorder transition temperature (≈593 K), and thus one must consider alternative non-equilibrium processing routes and alloy design strategies that make the formation of tetragonal FeNi feasible. In this paper, we investigate by density functional theory as implemented in the exact muffin-tin orbitals method whether alloying FeNi with a suitable element can have a positive impact on the phase formation and ordering properties while largely maintaining its attractive intrinsic magnetic properties. We find that small amount of non-magnetic (Al and Ti) or magnetic (Cr and Co) elements increase the order–disorder transition temperature. Adding Mo to the Co-doped system further enhances the ordering temperature while the Curie temperature is decreased only by a few degrees. Our results show that alloying is a viable route to stabilizing the ordered tetragonal phase of FeNi. Abstract Tetragonal ( $${\hbox{L1}}_{0}$$ L1 0 ) FeNi is a promising material for high-performance rare-earth-free permanent magnets. Pure tetragonal FeNi is very difficult to synthesize due to its low chemical order–disorder transition temperature ( $$\approx {593}$$ ≈ 593 K), and thus one must consider alternative non-equilibrium processing routes and alloy design strategies that make the formation of tetragonal FeNi feasible. In this paper, we investigate by density functional theory as implemented in the exact muffin-tin orbitals method whether alloying FeNi with a suitable element can have a positive impact on the phase formation and ordering properties while largely maintaining its attractive intrinsic magnetic properties. We find that small amount of non-magnetic (Al and Ti) or magnetic (Cr and Co) elements increase the order–disorder transition temperature. Adding Mo to the Co-doped system further enhances the ordering temperature while the Curie temperature is decreased only by a few degrees. Our results show that alloying is a viable route to stabilizing the ordered tetragonal phase of FeNi. |
| ArticleNumber | 5253 |
| Author | Vitos, Levente Gutfleisch, Oliver Tian, Li-Yun Eriksson, Olle |
| Author_xml | – sequence: 1 givenname: Li-Yun surname: Tian fullname: Tian, Li-Yun email: liyunt@kth.se organization: Applied Materials Physics, Department of Materials Science and Engineering, Royal Institute of Technology, Division of Materials Theory, Department of Physics and Astronomy, Uppsala University – sequence: 2 givenname: Oliver surname: Gutfleisch fullname: Gutfleisch, Oliver organization: Institute of Materials Science, Technische Universität Darmstadt – sequence: 3 givenname: Olle surname: Eriksson fullname: Eriksson, Olle organization: Division of Materials Theory, Department of Physics and Astronomy, Uppsala University, School of Science and Engineering, Örebro University – sequence: 4 givenname: Levente surname: Vitos fullname: Vitos, Levente email: levente@kth.se organization: Applied Materials Physics, Department of Materials Science and Engineering, Royal Institute of Technology, Division of Materials Theory, Department of Physics and Astronomy, Uppsala University, Research Institute for Solid State Physics and Optics, Wigner Research Center for Physics |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/33664353$$D View this record in MEDLINE/PubMed https://urn.kb.se/resolve?urn=urn:nbn:se:kth:diva-293481$$DView record from Swedish Publication Index https://urn.kb.se/resolve?urn=urn:nbn:se:oru:diva-90252$$DView record from Swedish Publication Index https://urn.kb.se/resolve?urn=urn:nbn:se:uu:diva-442102$$DView record from Swedish Publication Index |
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| CitedBy_id | crossref_primary_10_1016_j_jmmm_2024_172455 crossref_primary_10_1103_PhysRevMaterials_6_025402 crossref_primary_10_1016_j_jallcom_2022_166029 crossref_primary_10_3390_met14101125 crossref_primary_10_1038_s41524_024_01435_y crossref_primary_10_1109_TMAG_2022_3142849 crossref_primary_10_1103_PhysRevB_105_134428 crossref_primary_10_1016_j_jallcom_2023_171132 crossref_primary_10_1080_21663831_2022_2117576 |
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| Snippet | Tetragonal (
L1
0
) FeNi is a promising material for high-performance rare-earth-free permanent magnets. Pure tetragonal FeNi is very difficult to synthesize... Tetragonal ( $${\hbox{L1}}_{0}$$ L1 0 ) FeNi is a promising material for high-performance rare-earth-free permanent magnets. Pure tetragonal FeNi is very... Tetragonal ([Formula: see text]) FeNi is a promising material for high-performance rare-earth-free permanent magnets. Pure tetragonal FeNi is very difficult to... Tetragonal (L10) FeNi is a promising material for high-performance rare-earth-free permanent magnets. Pure tetragonal FeNi is very difficult to synthesize due... Tetragonal ( \documentclass[12pt]{minimal} \usepackage{amsmath} \usepackage{wasysym} \usepackage{amsfonts} \usepackage{amssymb} \usepackage{amsbsy}... Abstract Tetragonal ( $${\hbox{L1}}_{0}$$ L1 0 ) FeNi is a promising material for high-performance rare-earth-free permanent magnets. Pure tetragonal FeNi is... |
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| SubjectTerms | 639/301 639/4077 Alloys Equilibrium Humanities and Social Sciences Investigations Magnetic properties Magnetism Materials science multidisciplinary Physics Science Science (multidisciplinary) Temperature Tin Transition temperatures |
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| Title | Alloying effect on the order–disorder transformation in tetragonal FeNi |
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