Revealing the Critical Role of the HOMO Alignment on Maximizing Current Extraction and Suppressing Energy Loss in Organic Solar Cells
For state-of-the-art organic solar cells (OSCs) consisting of a large-bandgap polymer donor and a near-infrared (NIR) molecular acceptor, the control of the HOMO offset is the key to simultaneously achieve small energy loss (Eloss) and high photocurrent. However, the relationship between HOMO offset...
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| Published in | iScience Vol. 19; no. C; pp. 883 - 893 |
|---|---|
| Main Authors | , , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
United States
Elsevier Inc
27.09.2019
Elsevier |
| Subjects | |
| Online Access | Get full text |
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| Abstract | For state-of-the-art organic solar cells (OSCs) consisting of a large-bandgap polymer donor and a near-infrared (NIR) molecular acceptor, the control of the HOMO offset is the key to simultaneously achieve small energy loss (Eloss) and high photocurrent. However, the relationship between HOMO offsets and the efficiency for hole separation is quite elusive so far, which requires a comprehensive understanding on how small the driving force can effectively perform the charge separation while obtaining a high photovoltage to ensure high OSC performance. By designing a new family of ZITI-X NIR acceptors (X = S, C, N) with a high structural similarity and matching them with polymer donor J71 forming reduced HOMO offsets, we systematically investigated and established the relationship among the photovoltaic performance, energy loss, and hole-transfer kinetics. We achieved the highest PCEavgs of 14.05 ± 0.21% in a ternary system (J71:ZITI-C:ZITI-N) that best optimize the balance between driving force and energy loss.
[Display omitted]
•NIR acceptors with high structural similarity and variable HOMO levels were designed•We achieved the highest PCE of 14.36% by combining J71, ZITI-C, and ZITI-N acceptors•We revealed the importance of the optimized driving force on the device performance
Energy Storage; Materials Characterization; Solid State Physics |
|---|---|
| AbstractList | For state-of-the-art organic solar cells (OSCs) consisting of a large-bandgap polymer donor and a near-infrared (NIR) molecular acceptor, the control of the HOMO offset is the key to simultaneously achieve small energy loss (
E
loss
) and high photocurrent. However, the relationship between HOMO offsets and the efficiency for hole separation is quite elusive so far, which requires a comprehensive understanding on how small the driving force can effectively perform the charge separation while obtaining a high photovoltage to ensure high OSC performance. By designing a new family of ZITI-X NIR acceptors (X = S, C, N) with a high structural similarity and matching them with polymer donor J71 forming reduced HOMO offsets, we systematically investigated and established the relationship among the photovoltaic performance, energy loss, and hole-transfer kinetics. We achieved the highest PCE
avg
s of 14.05 ± 0.21% in a ternary system (J71:ZITI-C:ZITI-N) that best optimize the balance between driving force and energy loss.
•
NIR acceptors with high structural similarity and variable HOMO levels were designed
•
We achieved the highest PCE of 14.36% by combining J71, ZITI-C, and ZITI-N acceptors
•
We revealed the importance of the optimized driving force on the device performance
Energy Storage; Materials Characterization; Solid State Physics For state-of-the-art organic solar cells (OSCs) consisting of a large-bandgap polymer donor and a near-infrared (NIR) molecular acceptor, the control of the HOMO offset is the key to simultaneously achieve small energy loss (Eloss) and high photocurrent. However, the relationship between HOMO offsets and the efficiency for hole separation is quite elusive so far, which requires a comprehensive understanding on how small the driving force can effectively perform the charge separation while obtaining a high photovoltage to ensure high OSC performance. By designing a new family of ZITI-X NIR acceptors (X = S, C, N) with a high structural similarity and matching them with polymer donor J71 forming reduced HOMO offsets, we systematically investigated and established the relationship among the photovoltaic performance, energy loss, and hole-transfer kinetics. We achieved the highest PCEavgs of 14.05 ± 0.21% in a ternary system (J71:ZITI-C:ZITI-N) that best optimize the balance between driving force and energy loss.For state-of-the-art organic solar cells (OSCs) consisting of a large-bandgap polymer donor and a near-infrared (NIR) molecular acceptor, the control of the HOMO offset is the key to simultaneously achieve small energy loss (Eloss) and high photocurrent. However, the relationship between HOMO offsets and the efficiency for hole separation is quite elusive so far, which requires a comprehensive understanding on how small the driving force can effectively perform the charge separation while obtaining a high photovoltage to ensure high OSC performance. By designing a new family of ZITI-X NIR acceptors (X = S, C, N) with a high structural similarity and matching them with polymer donor J71 forming reduced HOMO offsets, we systematically investigated and established the relationship among the photovoltaic performance, energy loss, and hole-transfer kinetics. We achieved the highest PCEavgs of 14.05 ± 0.21% in a ternary system (J71:ZITI-C:ZITI-N) that best optimize the balance between driving force and energy loss. For state-of-the-art organic solar cells (OSCs) consisting of a large-bandgap polymer donor and a near-infrared (NIR) molecular acceptor, the control of the HOMO offset is the key to simultaneously achieve small energy loss (E ) and high photocurrent. However, the relationship between HOMO offsets and the efficiency for hole separation is quite elusive so far, which requires a comprehensive understanding on how small the driving force can effectively perform the charge separation while obtaining a high photovoltage to ensure high OSC performance. By designing a new family of ZITI-X NIR acceptors (X = S, C, N) with a high structural similarity and matching them with polymer donor J71 forming reduced HOMO offsets, we systematically investigated and established the relationship among the photovoltaic performance, energy loss, and hole-transfer kinetics. We achieved the highest PCE s of 14.05 ± 0.21% in a ternary system (J71:ZITI-C:ZITI-N) that best optimize the balance between driving force and energy loss. For state-of-the-art organic solar cells (OSCs) consisting of a large-bandgap polymer donor and a near-infrared (NIR) molecular acceptor, the control of the HOMO offset is the key to simultaneously achieve small energy loss (Eloss) and high photocurrent. However, the relationship between HOMO offsets and the efficiency for hole separation is quite elusive so far, which requires a comprehensive understanding on how small the driving force can effectively perform the charge separation while obtaining a high photovoltage to ensure high OSC performance. By designing a new family of ZITI-X NIR acceptors (X = S, C, N) with a high structural similarity and matching them with polymer donor J71 forming reduced HOMO offsets, we systematically investigated and established the relationship among the photovoltaic performance, energy loss, and hole-transfer kinetics. We achieved the highest PCEavgs of 14.05 ± 0.21% in a ternary system (J71:ZITI-C:ZITI-N) that best optimize the balance between driving force and energy loss. [Display omitted] •NIR acceptors with high structural similarity and variable HOMO levels were designed•We achieved the highest PCE of 14.36% by combining J71, ZITI-C, and ZITI-N acceptors•We revealed the importance of the optimized driving force on the device performance Energy Storage; Materials Characterization; Solid State Physics For state-of-the-art organic solar cells (OSCs) consisting of a large-bandgap polymer donor and a near-infrared (NIR) molecular acceptor, the control of the HOMO offset is the key to simultaneously achieve small energy loss (Eloss) and high photocurrent. However, the relationship between HOMO offsets and the efficiency for hole separation is quite elusive so far, which requires a comprehensive understanding on how small the driving force can effectively perform the charge separation while obtaining a high photovoltage to ensure high OSC performance. By designing a new family of ZITI-X NIR acceptors (X = S, C, N) with a high structural similarity and matching them with polymer donor J71 forming reduced HOMO offsets, we systematically investigated and established the relationship among the photovoltaic performance, energy loss, and hole-transfer kinetics. We achieved the highest PCEavgs of 14.05 ± 0.21% in a ternary system (J71:ZITI-C:ZITI-N) that best optimize the balance between driving force and energy loss. : Energy Storage; Materials Characterization; Solid State Physics Subject Areas: Energy Storage, Materials Characterization, Solid State Physics For state-of-the-art organic solar cells (OSCs) consisting of a large-bandgap polymer donor and a near infrared (NIR) molecular acceptor, the control of the HOMO offset is the key to simultaneously achieve small energy loss (Eloss) and high photocurrent. However, the relationship between HOMO offsets and the efficiency for hole separation is quite elusive so far, which requires a comprehensive understanding on how small the driving force can effectively perform the charge separation while obtaining a high photovoltage to ensure high OSC performance. By designing a new family of ZITI-X NIR acceptors (X = S, C, N) with a high structural similarity and matching them with polymer donor J71 forming reduced HOMO offsets, we systematically investigated and established the relationship among the photovoltaic performance, energy loss, and hole-transfer kinetics. We achieved the highest PCEavgs of 14.05 G 0.21% in a ternary system (J71:ZITI-C:ZITI-N) that best optimize the balance between driving force and energy loss. For state-of-the-art organic solar cells (OSCs) consisting of a large-bandgap polymer donor and a near-infrared (NIR) molecular acceptor, the control of the HOMO offset is the key to simultaneously achieve small energy loss (Eloss) and high photocurrent. However, the relationship between HOMO offsets and the efficiency for hole separation is quite elusive so far, which requires a comprehensive understanding on how small the driving force can effectively perform the charge separation while obtaining a high photovoltage to ensure high OSC performance. By designing a new family of ZITI-X NIR acceptors (X = S, C, N) with a high structural similarity and matching them with polymer donor J71 forming reduced HOMO offsets, we systematically investigated and established the relationship among the photovoltaic performance, energy loss, and hole-transfer kinetics. We achieved the highest PCEavgs of 14.05 ± 0.21% in a ternary system (J71:ZITI-C:ZITI-N) that best optimize the balance between driving force and energy loss. |
| Author | Liu, Yanfeng Zhu, Xiaozhang Zhou, Guanqing Zhang, Jianyun Liu, Feng Xu, Shengjie Liu, Wenrui Zhang, Fengling Zhu, Haiming Zhang, Ming |
| AuthorAffiliation | 2 School of Chemical Sciences, University of Chinese Academy of Sciences, Beijing 100190, China 5 Department of Chemistry, Zhejiang University, Hangzhou 310027, China 3 Department of Physics, Chemistry and Biology (IFM), Linköping University, Linköping SE-581 83, Sweden 1 Beijing National Laboratory for Molecular Sciences, CAS Key Laboratory of Organic Solids, Institute of Chemistry, Chinese Academy of Sciences, Beijing 100190, China 4 School of Chemistry and Chemical Engineering, and Center for Advanced Electronic Materials and Devices, Shanghai Jiao Tong University, Shanghai 200240, China |
| AuthorAffiliation_xml | – name: 4 School of Chemistry and Chemical Engineering, and Center for Advanced Electronic Materials and Devices, Shanghai Jiao Tong University, Shanghai 200240, China – name: 3 Department of Physics, Chemistry and Biology (IFM), Linköping University, Linköping SE-581 83, Sweden – name: 5 Department of Chemistry, Zhejiang University, Hangzhou 310027, China – name: 2 School of Chemical Sciences, University of Chinese Academy of Sciences, Beijing 100190, China – name: 1 Beijing National Laboratory for Molecular Sciences, CAS Key Laboratory of Organic Solids, Institute of Chemistry, Chinese Academy of Sciences, Beijing 100190, China |
| Author_xml | – sequence: 1 givenname: Jianyun surname: Zhang fullname: Zhang, Jianyun organization: Beijing National Laboratory for Molecular Sciences, CAS Key Laboratory of Organic Solids, Institute of Chemistry, Chinese Academy of Sciences, Beijing 100190, China – sequence: 2 givenname: Wenrui surname: Liu fullname: Liu, Wenrui organization: Beijing National Laboratory for Molecular Sciences, CAS Key Laboratory of Organic Solids, Institute of Chemistry, Chinese Academy of Sciences, Beijing 100190, China – sequence: 3 givenname: Ming surname: Zhang fullname: Zhang, Ming organization: School of Chemistry and Chemical Engineering, and Center for Advanced Electronic Materials and Devices, Shanghai Jiao Tong University, Shanghai 200240, China – sequence: 4 givenname: Yanfeng surname: Liu fullname: Liu, Yanfeng organization: Department of Physics, Chemistry and Biology (IFM), Linköping University, Linköping SE-581 83, Sweden – sequence: 5 givenname: Guanqing surname: Zhou fullname: Zhou, Guanqing organization: School of Chemistry and Chemical Engineering, and Center for Advanced Electronic Materials and Devices, Shanghai Jiao Tong University, Shanghai 200240, China – sequence: 6 givenname: Shengjie surname: Xu fullname: Xu, Shengjie email: xushengjie@iccas.ac.cn organization: Beijing National Laboratory for Molecular Sciences, CAS Key Laboratory of Organic Solids, Institute of Chemistry, Chinese Academy of Sciences, Beijing 100190, China – sequence: 7 givenname: Fengling surname: Zhang fullname: Zhang, Fengling organization: Department of Physics, Chemistry and Biology (IFM), Linköping University, Linköping SE-581 83, Sweden – sequence: 8 givenname: Haiming surname: Zhu fullname: Zhu, Haiming organization: Department of Chemistry, Zhejiang University, Hangzhou 310027, China – sequence: 9 givenname: Feng surname: Liu fullname: Liu, Feng email: fengliu82@sjtu.edu.cn organization: School of Chemistry and Chemical Engineering, and Center for Advanced Electronic Materials and Devices, Shanghai Jiao Tong University, Shanghai 200240, China – sequence: 10 givenname: Xiaozhang orcidid: 0000-0002-6812-0856 surname: Zhu fullname: Zhu, Xiaozhang email: xzzhu@iccas.ac.cn organization: Beijing National Laboratory for Molecular Sciences, CAS Key Laboratory of Organic Solids, Institute of Chemistry, Chinese Academy of Sciences, Beijing 100190, China |
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| Title | Revealing the Critical Role of the HOMO Alignment on Maximizing Current Extraction and Suppressing Energy Loss in Organic Solar Cells |
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