Perovskite microcells fabricated using swelling-induced crack propagation for colored solar windows
Perovskite microcells have a great potential to be applied to diverse types of optoelectronic devices including light-emitting diodes, photodetectors, and solar cells. Although several perovskite fabrication methods have been researched, perovskite microcells without a significant efficiency drop du...
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| Published in | Nature Communications Vol. 13; no. 1; pp. 1946 - 10 |
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| Main Authors | , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
London
Springer Science and Business Media LLC
11.04.2022
Nature Publishing Group UK Nature Publishing Group Nature Portfolio |
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| Online Access | Get full text |
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| Abstract | Perovskite microcells have a great potential to be applied to diverse types of optoelectronic devices including light-emitting diodes, photodetectors, and solar cells. Although several perovskite fabrication methods have been researched, perovskite microcells without a significant efficiency drop during the patterning and fabrication process could not be developed yet. We herein report the fabrication of high-efficiency perovskite microcells using swelling-induced crack propagation and the application of the microcells to colored solar windows. The key procedure is a swelling-induced lift-off process that leads to patterned perovskite films with high-quality interfaces. Thus, a power conversion efficiency (PCE) of 20.1 % could be achieved with the perovskite microcell, which is nearly same as the PCE of our unpatterned perovskite photovoltaic device (PV). The semi-transparent PV based on microcells exhibited a light utilization efficiency of 4.67 and a color rendering index of 97.5 %. The metal–insulator–metal structure deposited on the semi-transparent PV enabled to fabricate solar windows with vivid colors and high color purity.
Perovskite microcells can be applied to various types of optoelectronic devices. Here, authors report high efficiency perovskite microcells fabricated using swelling-induced crack propagation and demonstrate solar windows using the microcells. |
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| AbstractList | Perovskite microcells have a great potential to be applied to diverse types of optoelectronic devices including light-emitting diodes, photodetectors, and solar cells. Although several perovskite fabrication methods have been researched, perovskite microcells without a significant efficiency drop during the patterning and fabrication process could not be developed yet. We herein report the fabrication of high-efficiency perovskite microcells using swelling-induced crack propagation and the application of the microcells to colored solar windows. The key procedure is a swelling-induced lift-off process that leads to patterned perovskite films with high-quality interfaces. Thus, a power conversion efficiency (PCE) of 20.1 % could be achieved with the perovskite microcell, which is nearly same as the PCE of our unpatterned perovskite photovoltaic device (PV). The semi-transparent PV based on microcells exhibited a light utilization efficiency of 4.67 and a color rendering index of 97.5 %. The metal-insulator-metal structure deposited on the semi-transparent PV enabled to fabricate solar windows with vivid colors and high color purity.Perovskite microcells have a great potential to be applied to diverse types of optoelectronic devices including light-emitting diodes, photodetectors, and solar cells. Although several perovskite fabrication methods have been researched, perovskite microcells without a significant efficiency drop during the patterning and fabrication process could not be developed yet. We herein report the fabrication of high-efficiency perovskite microcells using swelling-induced crack propagation and the application of the microcells to colored solar windows. The key procedure is a swelling-induced lift-off process that leads to patterned perovskite films with high-quality interfaces. Thus, a power conversion efficiency (PCE) of 20.1 % could be achieved with the perovskite microcell, which is nearly same as the PCE of our unpatterned perovskite photovoltaic device (PV). The semi-transparent PV based on microcells exhibited a light utilization efficiency of 4.67 and a color rendering index of 97.5 %. The metal-insulator-metal structure deposited on the semi-transparent PV enabled to fabricate solar windows with vivid colors and high color purity. Perovskite microcells have a great potential to be applied to diverse types of optoelectronic devices including light-emitting diodes, photodetectors, and solar cells. Although several perovskite fabrication methods have been researched, perovskite microcells without a significant efficiency drop during the patterning and fabrication process could not be developed yet. We herein report the fabrication of high-efficiency perovskite microcells using swelling-induced crack propagation and the application of the microcells to colored solar windows. The key procedure is a swelling-induced lift-off process that leads to patterned perovskite films with high-quality interfaces. Thus, a power conversion efficiency (PCE) of 20.1 % could be achieved with the perovskite microcell, which is nearly same as the PCE of our unpatterned perovskite photovoltaic device (PV). The semi-transparent PV based on microcells exhibited a light utilization efficiency of 4.67 and a color rendering index of 97.5 %. The metal-insulator-metal structure deposited on the semi-transparent PV enabled to fabricate solar windows with vivid colors and high color purity. Perovskite microcells have a great potential to be applied to diverse types of optoelectronic devices including light-emitting diodes, photodetectors, and solar cells. Although several perovskite fabrication methods have been researched, perovskite microcells without a significant efficiency drop during the patterning and fabrication process could not be developed yet. We herein report the fabrication of high-efficiency perovskite microcells using swelling-induced crack propagation and the application of the microcells to colored solar windows. The key procedure is a swelling-induced lift-off process that leads to patterned perovskite films with high-quality interfaces. Thus, a power conversion efficiency (PCE) of 20.1 % could be achieved with the perovskite microcell, which is nearly same as the PCE of our unpatterned perovskite photovoltaic device (PV). The semi-transparent PV based on microcells exhibited a light utilization efficiency of 4.67 and a color rendering index of 97.5 %. The metal–insulator–metal structure deposited on the semi-transparent PV enabled to fabricate solar windows with vivid colors and high color purity. Perovskite microcells can be applied to various types of optoelectronic devices. Here, authors report high efficiency perovskite microcells fabricated using swelling-induced crack propagation and demonstrate solar windows using the microcells. Perovskite microcells have a great potential to be applied to diverse types of optoelectronic devices including light-emitting diodes, photodetectors, and solar cells. Although several perovskite fabrication methods have been researched, perovskite microcells without a significant efficiency drop during the patterning and fabrication process could not be developed yet. We herein report the fabrication of high-efficiency perovskite microcells using swelling-induced crack propagation and the application of the microcells to colored solar windows. The key procedure is a swelling-induced lift-off process that leads to patterned perovskite films with high-quality interfaces. Thus, a power conversion efficiency (PCE) of 20.1 % could be achieved with the perovskite microcell, which is nearly same as the PCE of our unpatterned perovskite photovoltaic device (PV). The semi-transparent PV based on microcells exhibited a light utilization efficiency of 4.67 and a color rendering index of 97.5 %. The metal–insulator–metal structure deposited on the semi-transparent PV enabled to fabricate solar windows with vivid colors and high color purity.Perovskite microcells can be applied to various types of optoelectronic devices. Here, authors report high efficiency perovskite microcells fabricated using swelling-induced crack propagation and demonstrate solar windows using the microcells. Perovskite microcells can be applied to various types of optoelectronic devices. Here, authors report high efficiency perovskite microcells fabricated using swelling-induced crack propagation and demonstrate solar windows using the microcells. |
| ArticleNumber | 1946 |
| Author | Woongchan Lee Joo Hwan Ko Jinhong Park Yeong Jae Kim Young Min Song Huiwon Yun Dae-Hyeong Kim Young Jin Yoo Dong Hoe Kim |
| Author_xml | – sequence: 1 givenname: Woongchan surname: Lee fullname: Lee, Woongchan organization: Center for Nanoparticle Research, Institute for Basic Science (IBS), School of Chemical and Biological Engineering, Institute of Chemical Processes, Seoul National University – sequence: 2 givenname: Young Jin orcidid: 0000-0002-6490-2324 surname: Yoo fullname: Yoo, Young Jin organization: School of Electrical Engineering and Computer Science, Gwangju Institute of Science and Technology – sequence: 3 givenname: Jinhong surname: Park fullname: Park, Jinhong organization: Center for Nanoparticle Research, Institute for Basic Science (IBS), School of Chemical and Biological Engineering, Institute of Chemical Processes, Seoul National University – sequence: 4 givenname: Joo Hwan surname: Ko fullname: Ko, Joo Hwan organization: School of Electrical Engineering and Computer Science, Gwangju Institute of Science and Technology – sequence: 5 givenname: Yeong Jae surname: Kim fullname: Kim, Yeong Jae organization: School of Electrical Engineering and Computer Science, Gwangju Institute of Science and Technology – sequence: 6 givenname: Huiwon surname: Yun fullname: Yun, Huiwon organization: Center for Nanoparticle Research, Institute for Basic Science (IBS), School of Chemical and Biological Engineering, Institute of Chemical Processes, Seoul National University – sequence: 7 givenname: Dong Hoe orcidid: 0000-0001-8909-2076 surname: Kim fullname: Kim, Dong Hoe email: donghoekim@korea.ac.kr organization: Department of Materials Science and Engineering, Korea University – sequence: 8 givenname: Young Min orcidid: 0000-0002-4473-6883 surname: Song fullname: Song, Young Min email: ymsong@gist.ac.kr organization: School of Electrical Engineering and Computer Science, Gwangju Institute of Science and Technology – sequence: 9 givenname: Dae-Hyeong orcidid: 0000-0002-4722-1893 surname: Kim fullname: Kim, Dae-Hyeong email: dkim98@snu.ac.kr organization: Center for Nanoparticle Research, Institute for Basic Science (IBS), School of Chemical and Biological Engineering, Institute of Chemical Processes, Seoul National University, Department of Materials Science and Engineering, Seoul National University |
| BackLink | https://cir.nii.ac.jp/crid/1874243915830148224$$DView record in CiNii https://www.ncbi.nlm.nih.gov/pubmed/35410337$$D View this record in MEDLINE/PubMed |
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| Snippet | Perovskite microcells have a great potential to be applied to diverse types of optoelectronic devices including light-emitting diodes, photodetectors, and... Perovskite microcells can be applied to various types of optoelectronic devices. Here, authors report high efficiency perovskite microcells fabricated using... |
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| StartPage | 1946 |
| SubjectTerms | 142/126 639/301/299/946 639/301/930/543 Color Crack propagation Efficiency Energy conversion efficiency Fabrication Humanities and Social Sciences Interfaces Light emitting diodes multidisciplinary Optoelectronic devices Perovskites Photovoltaic cells Photovoltaics Propagation Q Science Science (multidisciplinary) Solar cells Swelling |
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| Title | Perovskite microcells fabricated using swelling-induced crack propagation for colored solar windows |
| URI | https://cir.nii.ac.jp/crid/1874243915830148224 https://link.springer.com/article/10.1038/s41467-022-29602-z https://www.ncbi.nlm.nih.gov/pubmed/35410337 https://www.proquest.com/docview/2649218088 https://www.proquest.com/docview/2649589082 https://pubmed.ncbi.nlm.nih.gov/PMC9001655 https://doaj.org/article/96ffad06480444d4b65b6ab214543627 |
| Volume | 13 |
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