Functional Supramolecular Polymers

Supramolecular polymers can be random and entangled coils with the mechanical properties of plastics and elastomers, but with great capacity for processability, recycling, and self-healing due to their reversible monomer-to-polymer transitions. At the other extreme, supramolecular polymers can be fo...

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Published in	Science (American Association for the Advancement of Science) Vol. 335; no. 6070; pp. 813 - 817
Main Authors	Aida, T., Meijer, E. W., Stupp, S. I.
Format	Journal Article
Language	English
Published	Washington, DC American Association for the Advancement of Science 17.02.2012 The American Association for the Advancement of Science
Subjects	Animals Applied sciences Biomimetic Materials - chemistry Chemical bonding Chemical bonds Coils Dynamics Electronics Exact sciences and technology Forecasting Humans Hydrogen bonds Materials Materials science Mechanical properties Molecular chains Molecular interactions Molecular Structure Molecules Monomers Nanofibers Nanotubes Organic polymers Physicochemistry of polymers Polymers Polymers - chemistry Properties and characterization Receptors Recycling REVIEW Self assembly Semiconductors Signal Transduction Structure, morphology and analysis Supramolecular polymers Conducting polymers Self assembly State of the art Conducting material Supramolecular structure Elastomer Mechanical properties Polymer Biomaterial Technological properties Functional polymer
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Abstract	Supramolecular polymers can be random and entangled coils with the mechanical properties of plastics and elastomers, but with great capacity for processability, recycling, and self-healing due to their reversible monomer-to-polymer transitions. At the other extreme, supramolecular polymers can be formed by self-assembly among designed subunits to yield shape-persistent and highly ordered filaments. The use of strong and directional interactions among molecular subunits can achieve not only rich dynamic behavior but also high degrees of internal order that are not known in ordinary polymers. They can resemble, for example, the ordered and dynamic one-dimensional supramolecular assemblies of the cell cytoskeleton and possess useful biological and electronic functions.
AbstractList	Supramolecular polymers can be random and entangled coils with the mechanical properties of plastics and elastomers, but with great capacity for processability, recycling, and self-healing due to their reversible monomer-to-polymer transitions. At the other extreme, supramolecular polymers can be formed by self-assembly among designed subunits to yield shape-persistent and highly ordered filaments. The use of strong and directional interactions among molecular subunits can achieve not only rich dynamic behavior but also high degrees of internal order that are not known in ordinary polymers. They can resemble, for example, the ordered and dynamic one-dimensional supramolecular assemblies of the cell cytoskeleton and possess useful biological and electronic functions. While polymers are constructed from chemically bonded units, supramolecular polymers arise through reversible linkages, such as hydrogen bonding and electrostatic interactions. Recent advances in the field of supramolecular polymer science have moved from a fundamental understanding of assembly properties to the introduction of functionality, in order to exploit the particular features of this class of materials. Aida et al. (p. 813) review the specific features of supramolecular polymers that can lead to applications in a variety of fields, including: materials--in which processability and self-healing properties are of interest; biomedicine--in which the concerns are dynamic functionality and biodegradability; and hierarchical assembly and electronic systems--with an interest in unidirectionality of charge flow. Supramolecular polymers can be random and entangled coils with the mechanical properties of plastics and elastomers, but with great capacity for processability, recycling, and self-healing due to their reversible monomer-to-polymer transitions. At the other extreme, supramolecular polymers can be formed by self-assembly among designed subunits to yield shape-persistent and highly ordered filaments. The use of strong and directional interactions among molecular subunits can achieve not only rich dynamic behavior but also high degrees of internal order that are not known in ordinary polymers. They can resemble, for example, the ordered and dynamic one-dimensional supramolecular assemblies of the cell cytoskeleton and possess useful biological and electronic functions. [PUBLICATION ABSTRACT] Supramolecular Polymers Explained While polymers are constructed from chemically bonded units, supramolecular polymers arise through reversible linkages, such as hydrogen bonding and electrostatic interactions. Recent advances in the field of supramolecular polymer science have moved from a fundamental understanding of assembly properties to the introduction of functionality, in order to exploit the particular features of this class of materials. Aida et al. (p. 813 ) review the specific features of supramolecular polymers that can lead to applications in a variety of fields, including: materials—in which processability and self-healing properties are of interest; biomedicine—in which the concerns are dynamic functionality and biodegradability; and hierarchical assembly and electronic systems—with an interest in unidirectionality of charge flow. Supramolecular polymers can be random and entangled coils with the mechanical properties of plastics and elastomers, but with great capacity for processability, recycling, and self-healing due to their reversible monomer-to-polymer transitions. At the other extreme, supramolecular polymers can be formed by self-assembly among designed subunits to yield shape-persistent and highly ordered filaments. The use of strong and directional interactions among molecular subunits can achieve not only rich dynamic behavior but also high degrees of internal order that are not known in ordinary polymers. They can resemble, for example, the ordered and dynamic one-dimensional supramolecular assemblies of the cell cytoskeleton and possess useful biological and electronic functions.
Author	Stupp, S. I. Aida, T. Meijer, E. W.
AuthorAffiliation	3 Institute for Complex Molecular Systems, Eindhoven University of Technology, Post Office Box 513, 5600 MB Eindhoven, Netherlands 5 Department of Chemistry, Northwestern University, 2220 Campus Drive, Evanston, Illinois 60208 2 RIKEN Advanced Science Institute, 2-1 Hirosawa, Wako, Saitama 351-0198, Japan 4 Department of Materials Science and Engineering, Northwestern University, 2220 Campus Drive, Evanston, Illinois 60208 6 Department of Medicine, Northwestern University, Chicago, Illinois 60611 1 Department of Chemistry and Biotechnology, School of Engineering, The University of Tokyo, 7-3-1 Hongo, Bunkyo, Tokyo 113-8656, Japan 7 Institute for BioNanotechnology in Medicine, Northwestern University, 303 E. Superior, Chicago, Illinois 60611
AuthorAffiliation_xml	– name: 5 Department of Chemistry, Northwestern University, 2220 Campus Drive, Evanston, Illinois 60208 – name: 1 Department of Chemistry and Biotechnology, School of Engineering, The University of Tokyo, 7-3-1 Hongo, Bunkyo, Tokyo 113-8656, Japan – name: 3 Institute for Complex Molecular Systems, Eindhoven University of Technology, Post Office Box 513, 5600 MB Eindhoven, Netherlands – name: 6 Department of Medicine, Northwestern University, Chicago, Illinois 60611 – name: 7 Institute for BioNanotechnology in Medicine, Northwestern University, 303 E. Superior, Chicago, Illinois 60611 – name: 2 RIKEN Advanced Science Institute, 2-1 Hirosawa, Wako, Saitama 351-0198, Japan – name: 4 Department of Materials Science and Engineering, Northwestern University, 2220 Campus Drive, Evanston, Illinois 60208
Author_xml	– sequence: 1 givenname: T. surname: Aida fullname: Aida, T. – sequence: 2 givenname: E. W. surname: Meijer fullname: Meijer, E. W. – sequence: 3 givenname: S. I. surname: Stupp fullname: Stupp, S. I.
BackLink	http://pascal-francis.inist.fr/vibad/index.php?action=getRecordDetail&idt=25564959$$DView record in Pascal Francis https://www.ncbi.nlm.nih.gov/pubmed/22344437$$D View this record in MEDLINE/PubMed
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ContentType	Journal Article
Copyright	Copyright © 2012 American Association for the Advancement of Science 2015 INIST-CNRS Copyright © 2012, American Association for the Advancement of Science
Copyright_xml	– notice: Copyright © 2012 American Association for the Advancement of Science – notice: 2015 INIST-CNRS – notice: Copyright © 2012, American Association for the Advancement of Science
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Keywords	Conducting polymers Self assembly State of the art Conducting material Supramolecular structure Elastomer Mechanical properties Polymer Biomaterial Technological properties Functional polymer
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Snippet	Supramolecular polymers can be random and entangled coils with the mechanical properties of plastics and elastomers, but with great capacity for... Supramolecular Polymers Explained While polymers are constructed from chemically bonded units, supramolecular polymers arise through reversible linkages, such... While polymers are constructed from chemically bonded units, supramolecular polymers arise through reversible linkages, such as hydrogen bonding and...
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SubjectTerms	Animals Applied sciences Biomimetic Materials - chemistry Chemical bonding Chemical bonds Coils Dynamics Electronics Exact sciences and technology Forecasting Humans Hydrogen bonds Materials Materials science Mechanical properties Molecular chains Molecular interactions Molecular Structure Molecules Monomers Nanofibers Nanotubes Organic polymers Physicochemistry of polymers Polymers Polymers - chemistry Properties and characterization Receptors Recycling REVIEW Self assembly Semiconductors Signal Transduction Structure, morphology and analysis Supramolecular polymers
Title	Functional Supramolecular Polymers
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