Operando monitoring of ion activities in aqueous batteries with plasmonic fiber-optic sensors
Understanding ion transport kinetics and electrolyte-electrode interactions at electrode surfaces of batteries in operation is essential to determine their performance and state of health. However, it remains a challenging task to capture in real time the details of surface-localized and rapid ion t...
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| Published in | Nature communications Vol. 13; no. 1; pp. 547 - 11 |
|---|---|
| Main Authors | , , , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
London
Springer Nature Limited
27.01.2022
Nature Publishing Group UK Nature Publishing Group Nature Portfolio |
| Subjects | |
| Online Access | Get full text |
| ISSN | 2041-1723 2041-1723 |
| DOI | 10.1038/s41467-022-28267-y |
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| Abstract | Understanding ion transport kinetics and electrolyte-electrode interactions at electrode surfaces of batteries in operation is essential to determine their performance and state of health. However, it remains a challenging task to capture in real time the details of surface-localized and rapid ion transport at the microscale. To address this, a promising approach based on an optical fiber plasmonic sensor capable of being inserted near the electrode surface of a working battery to monitor its electrochemical kinetics without disturbing its operation is demonstrated using aqueous Zn-ion batteries as an example. The miniature and chemically inert sensor detects perturbations of surface plasmon waves propagating on its surface to rapidly screen localized electrochemical events on a sub-μm-scale thickness adjacent to the electrode interface. A stable and reproducible correlation between the real-time ion insertions over charge-discharge cycles and the optical plasmon response has been observed and quantified. This new operando measurement tool will provide crucial additional capabilities to battery monitoring methods and help guide the design of better batteries with improved electro-chemistries. NRC publication: Yes |
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| AbstractList | Understanding ion transport kinetics and electrolyte-electrode interactions at electrode surfaces of batteries in operation is essential to determine their performance and state of health. However, it remains a challenging task to capture in real time the details of surface-localized and rapid ion transport at the microscale. To address this, a promising approach based on an optical fiber plasmonic sensor capable of being inserted near the electrode surface of a working battery to monitor its electrochemical kinetics without disturbing its operation is demonstrated using aqueous Zn-ion batteries as an example. The miniature and chemically inert sensor detects perturbations of surface plasmon waves propagating on its surface to rapidly screen localized electrochemical events on a sub-μm-scale thickness adjacent to the electrode interface. A stable and reproducible correlation between the real-time ion insertions over charge-discharge cycles and the optical plasmon response has been observed and quantified. This new operando measurement tool will provide crucial additional capabilities to battery monitoring methods and help guide the design of better batteries with improved electro-chemistries. Understanding ion transport kinetics and electrolyte-electrode interactions at electrode surfaces of batteries in operation is essential to determine their performance and state of health. However, it remains a challenging task to capture in real time the details of surface-localized and rapid ion transport at the microscale. To address this, a promising approach based on an optical fiber plasmonic sensor capable of being inserted near the electrode surface of a working battery to monitor its electrochemical kinetics without disturbing its operation is demonstrated using aqueous Zn-ion batteries as an example. The miniature and chemically inert sensor detects perturbations of surface plasmon waves propagating on its surface to rapidly screen localized electrochemical events on a sub-μm-scale thickness adjacent to the electrode interface. A stable and reproducible correlation between the real-time ion insertions over charge-discharge cycles and the optical plasmon response has been observed and quantified. This new operando measurement tool will provide crucial additional capabilities to battery monitoring methods and help guide the design of better batteries with improved electro-chemistries.Understanding ion transport kinetics and electrolyte-electrode interactions at electrode surfaces of batteries in operation is essential to determine their performance and state of health. However, it remains a challenging task to capture in real time the details of surface-localized and rapid ion transport at the microscale. To address this, a promising approach based on an optical fiber plasmonic sensor capable of being inserted near the electrode surface of a working battery to monitor its electrochemical kinetics without disturbing its operation is demonstrated using aqueous Zn-ion batteries as an example. The miniature and chemically inert sensor detects perturbations of surface plasmon waves propagating on its surface to rapidly screen localized electrochemical events on a sub-μm-scale thickness adjacent to the electrode interface. A stable and reproducible correlation between the real-time ion insertions over charge-discharge cycles and the optical plasmon response has been observed and quantified. This new operando measurement tool will provide crucial additional capabilities to battery monitoring methods and help guide the design of better batteries with improved electro-chemistries. Understanding ion transport kinetics and electrolyte-electrode interactions at electrode surfaces of batteries in operation is essential to determine their performance and state of health. However, it remains a challenging task to capture in real time the details of surface-localized and rapid ion transport at the microscale. To address this, a promising approach based on an optical fiber plasmonic sensor capable of being inserted near the electrode surface of a working battery to monitor its electrochemical kinetics without disturbing its operation is demonstrated using aqueous Zn-ion batteries as an example. The miniature and chemically inert sensor detects perturbations of surface plasmon waves propagating on its surface to rapidly screen localized electrochemical events on a sub-μm-scale thickness adjacent to the electrode interface. A stable and reproducible correlation between the real-time ion insertions over charge-discharge cycles and the optical plasmon response has been observed and quantified. This new operando measurement tool will provide crucial additional capabilities to battery monitoring methods and help guide the design of better batteries with improved electro-chemistries.Operando tracking the ion dynamics/states of battery is critical to understanding of electrolyte-electrode interactions. Here the authors propose to use the surface plasmon waves to rapidly screen localized electrochemical events on a sub-μm-scale thickness adjacent to the electrode interface, without perturbing battery operation. Understanding ion transport kinetics and electrolyte-electrode interactions at electrode surfaces of batteries in operation is essential to determine their performance and state of health. However, it remains a challenging task to capture in real time the details of surface-localized and rapid ion transport at the microscale. To address this, a promising approach based on an optical fiber plasmonic sensor capable of being inserted near the electrode surface of a working battery to monitor its electrochemical kinetics without disturbing its operation is demonstrated using aqueous Zn-ion batteries as an example. The miniature and chemically inert sensor detects perturbations of surface plasmon waves propagating on its surface to rapidly screen localized electrochemical events on a sub-μm-scale thickness adjacent to the electrode interface. A stable and reproducible correlation between the real-time ion insertions over charge-discharge cycles and the optical plasmon response has been observed and quantified. This new operando measurement tool will provide crucial additional capabilities to battery monitoring methods and help guide the design of better batteries with improved electro-chemistries. Operando tracking the ion dynamics/states of battery is critical to understanding of electrolyte-electrode interactions. Here the authors propose to use the surface plasmon waves to rapidly screen localized electrochemical events on a sub-μm-scale thickness adjacent to the electrode interface, without perturbing battery operation. Operando tracking the ion dynamics/states of battery is critical to understanding of electrolyte-electrode interactions. Here the authors propose to use the surface plasmon waves to rapidly screen localized electrochemical events on a sub-μm-scale thickness adjacent to the electrode interface, without perturbing battery operation. |
| ArticleNumber | 547 |
| Author | Liu, Fu Albert, Jacques Han, Xile Liu, Qiyu Xiao, Gaozhi Wang, Runlin Li, Kaiwei Guo, Tuan Zhang, Haozhe Lu, Xihong Liu, Xiaoqing |
| Author_xml | – sequence: 1 fullname: Wang, Runlin – sequence: 2 fullname: Zhang, Haozhe – sequence: 3 fullname: Liu, Qiyu – sequence: 4 fullname: Liu, Fu – sequence: 5 fullname: Han, Xile – sequence: 6 fullname: Liu, Xiaoqing – sequence: 7 fullname: Li, Kaiwei – sequence: 8 fullname: Xiao, Gaozhi – sequence: 9 fullname: Albert, Jacques – sequence: 10 fullname: Lu, Xihong – sequence: 11 fullname: Guo, Tuan |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/35087063$$D View this record in MEDLINE/PubMed |
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| Snippet | Understanding ion transport kinetics and electrolyte-electrode interactions at electrode surfaces of batteries in operation is essential to determine their... Operando tracking the ion dynamics/states of battery is critical to understanding of electrolyte-electrode interactions. Here the authors propose to use the... |
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| SubjectTerms | 639/4077/4079/891 639/624/1075/1083 639/638/161/891 639/638/675 Electrochemistry Electrodes Electrolytes Fiber optics Humanities and Social Sciences Ion dynamics Ion transport Kinetics Monitoring Monitoring methods multidisciplinary Optical fibers Perturbation Plasmonics Real time Rechargeable batteries Science Science (multidisciplinary) Thickness Wave propagation |
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| Title | Operando monitoring of ion activities in aqueous batteries with plasmonic fiber-optic sensors |
| URI | https://nrc-publications.canada.ca/eng/view/object/?id=7637c56a-5038-453e-b8e9-c5e4b4a2f0cc https://link.springer.com/article/10.1038/s41467-022-28267-y https://www.ncbi.nlm.nih.gov/pubmed/35087063 https://www.proquest.com/docview/2623201395 https://www.proquest.com/docview/2623891649 https://pubmed.ncbi.nlm.nih.gov/PMC8795113 https://doaj.org/article/b70856260dab468f9f0441eee9cddfae |
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