Natural attenuation processes for remediation of arsenic contaminated soils and groundwater

Arsenic (As) contamination presents a hazard in many countries. Natural attenuation (NA) of As-contaminated soils and groundwater may be a cost-effective in situ remedial option. It relies on the site intrinsic assimilative capacity and allows in-place cleanup. Sorption to solid phases is the princi...

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Published in	Journal of hazardous materials Vol. 138; no. 3; pp. 459 - 470
Main Authors	Wang, Suiling, Mulligan, Catherine N.
Format	Journal Article
Language	English
Published	Amsterdam Elsevier B.V 01.12.2006 Elsevier
Subjects	Applied sciences Arsenic Arsenic - chemistry Arsenic - metabolism Biodegradation, Environmental Biotransformation Chemical engineering Decontamination. Miscellaneous Enhanced natural attenuation Exact sciences and technology Groundwaters Hyperaccumulation Immobilization In situ remediation Natural water pollution Oxidation-Reduction Pollution Safety Soil and sediments pollution Soil Pollutants - chemistry Soil Pollutants - metabolism Water Pollutants, Chemical - chemistry Water Pollutants, Chemical - metabolism Water treatment and pollution Immobilization Hyperaccumulation Arsenic Enhanced natural attenuation Biotransformation In situ remediation Microbial activity Organic matter In situ Mobility Soil pollution Aquifers Transport process Decontamination Selfpurification pH Bioremediation Mathematical model Hazard Speciation Ground water Pollutant behavior Sediments Long term Contamination Phytoremediation Sorption Surveillance Redox potential
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Abstract	Arsenic (As) contamination presents a hazard in many countries. Natural attenuation (NA) of As-contaminated soils and groundwater may be a cost-effective in situ remedial option. It relies on the site intrinsic assimilative capacity and allows in-place cleanup. Sorption to solid phases is the principal mechanism immobilizing As in soils and removing it from groundwater. Hydroxides of iron, aluminum and manganese, clay and sulfide minerals, and natural organic matter are commonly associated with soils and aquifer sediments, and have been shown to be significant As adsorbents. The extent of sorption is influenced by As speciation and the site geochemical conditions such as pH, redox potential, and the co-occurring ions. Microbial activity may catalyze the transformation of As species, or mediate redox reactions thus influencing As mobility. Plants that are capable of hyperaccumulating As may translocate As from contaminated soils and groundwater to their tissues, providing the basis for phytoremediation. However, NA is subject to hydrological changes and may take substantial periods of time, thus requiring long-term monitoring. The current understanding of As NA processes remains limited. Sufficient site characterization is critical to the success of NA. Further research is required to develop conceptual and mathematical models to predict the fate and transport of As and to evaluate the site NA capacity. Engineering enhanced NA using environmentally benign products may be an effective alternative.
AbstractList	Arsenic (As) contamination presents a hazard in many countries. Natural attenuation (NA) of As-contaminated soils and groundwater may be a cost-effective in situ remedial option. It relies on the site intrinsic assimilative capacity and allows in-place cleanup. Sorption to solid phases is the principal mechanism immobilizing As in soils and removing it from groundwater. Hydroxides of iron, aluminum and manganese, clay and sulfide minerals, and natural organic matter are commonly associated with soils and aquifer sediments, and have been shown to be significant As adsorbents. The extent of sorption is influenced by As speciation and the site geochemical conditions such as pH, redox potential, and the co-occurring ions. Microbial activity may catalyze the transformation of As species, or mediate redox reactions thus influencing As mobility. Plants that are capable of hyperaccumulating As may translocate As from contaminated soils and groundwater to their tissues, providing the basis for phytoremediation. However, NA is subject to hydrological changes and may take substantial periods of time, thus requiring long-term monitoring. The current understanding of As NA processes remains limited. Sufficient site characterization is critical to the success of NA. Further research is required to develop conceptual and mathematical models to predict the fate and transport of As and to evaluate the site NA capacity. Engineering enhanced NA using environmentally benign products may be an effective alternative.Arsenic (As) contamination presents a hazard in many countries. Natural attenuation (NA) of As-contaminated soils and groundwater may be a cost-effective in situ remedial option. It relies on the site intrinsic assimilative capacity and allows in-place cleanup. Sorption to solid phases is the principal mechanism immobilizing As in soils and removing it from groundwater. Hydroxides of iron, aluminum and manganese, clay and sulfide minerals, and natural organic matter are commonly associated with soils and aquifer sediments, and have been shown to be significant As adsorbents. The extent of sorption is influenced by As speciation and the site geochemical conditions such as pH, redox potential, and the co-occurring ions. Microbial activity may catalyze the transformation of As species, or mediate redox reactions thus influencing As mobility. Plants that are capable of hyperaccumulating As may translocate As from contaminated soils and groundwater to their tissues, providing the basis for phytoremediation. However, NA is subject to hydrological changes and may take substantial periods of time, thus requiring long-term monitoring. The current understanding of As NA processes remains limited. Sufficient site characterization is critical to the success of NA. Further research is required to develop conceptual and mathematical models to predict the fate and transport of As and to evaluate the site NA capacity. Engineering enhanced NA using environmentally benign products may be an effective alternative. Natural attenuation (NA) process for remediation of arsenic (As) contaminated soils and groundwater was studied. Hydroxides of iron, aluminum and manganese, clay and sulfide minerals, and natural organic matter were commonly associated with soils and aquifer sediments. The extent of sorption was influenced by As speciation and the site geochemical conditions namely, pH, redox potential, and the co-occurring ions. Microbial activity might catalyze the transformation of As species, or mediate redox reactions, which influenced As mobility. Plants that were capable of hyperaccumulating As might translocate As from contaminated soils and groundwater to their tissues, which provided basis for phytoremediation. The results concluded that future research is required to develop conceptual and mathematical models to predict the fate and transport of As and the evaluate the site NA capacity. Arsenic (As) contamination presents a hazard in many countries. Natural attenuation (NA) of As-contaminated soils and groundwater may be a cost- effective in situ remedial option. It relies on the site intrinsic assimilative capacity and allows in-place cleanup. Sorption to solid phases is the principal mechanism immobilizing As in soils and removing it from groundwater. Hydroxides of iron, aluminum and manganese, clay and sulfide minerals, and natural organic matter are commonly associated with soils and aquifer sediments, and have been shown to be significant As adsorbents. The extent of sorption is influenced by As speciation and the site geochemical conditions such as pH, redox potential, and the co-occurring ions. Microbial activity may catalyze the transformation of As species, or mediate redox reactions thus influencing As mobility. Plants that are capable of hyperaccumulating As may translocate As from contaminated soils and groundwater to their tissues, providing the basis for phytoremediation. However, NA is subject to hydrological changes and may take substantial periods of time, thus requiring long-term monitoring. The current understanding of As NA processes remains limited. Sufficient site characterization is critical to the success of NA. Further research is required to develop conceptual and mathematical models to predict the fate and transport of As and to evaluate the site NA capacity. Engineering enhanced NA using environmentally benign products may be an effective alternative. Arsenic (As) contamination presents a hazard in many countries. Natural attenuation (NA) of As-contaminated soils and groundwater may be a cost-effective in situ remedial option. It relies on the site intrinsic assimilative capacity and allows in-place cleanup. Sorption to solid phases is the principal mechanism immobilizing As in soils and removing it from groundwater. Hydroxides of iron, aluminum and manganese, clay and sulfide minerals, and natural organic matter are commonly associated with soils and aquifer sediments, and have been shown to be significant As adsorbents. The extent of sorption is influenced by As speciation and the site geochemical conditions such as pH, redox potential, and the co-occurring ions. Microbial activity may catalyze the transformation of As species, or mediate redox reactions thus influencing As mobility. Plants that are capable of hyperaccumulating As may translocate As from contaminated soils and groundwater to their tissues, providing the basis for phytoremediation. However, NA is subject to hydrological changes and may take substantial periods of time, thus requiring long-term monitoring. The current understanding of As NA processes remains limited. Sufficient site characterization is critical to the success of NA. Further research is required to develop conceptual and mathematical models to predict the fate and transport of As and to evaluate the site NA capacity. Engineering enhanced NA using environmentally benign products may be an effective alternative.
Author	Wang, Suiling Mulligan, Catherine N.
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Keywords	Immobilization Hyperaccumulation Arsenic Enhanced natural attenuation Biotransformation In situ remediation Microbial activity Organic matter In situ Mobility Soil pollution Aquifers Transport process Decontamination Selfpurification pH Bioremediation Mathematical model Hazard Speciation Ground water Pollutant behavior Sediments Long term Contamination Phytoremediation Sorption Surveillance Redox potential
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Snippet	Arsenic (As) contamination presents a hazard in many countries. Natural attenuation (NA) of As-contaminated soils and groundwater may be a cost-effective in... Arsenic (As) contamination presents a hazard in many countries. Natural attenuation (NA) of As-contaminated soils and groundwater may be a cost-effective in... Natural attenuation (NA) process for remediation of arsenic (As) contaminated soils and groundwater was studied. Hydroxides of iron, aluminum and manganese,... Arsenic (As) contamination presents a hazard in many countries. Natural attenuation (NA) of As-contaminated soils and groundwater may be a cost- effective in...
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SubjectTerms	Applied sciences Arsenic Arsenic - chemistry Arsenic - metabolism Biodegradation, Environmental Biotransformation Chemical engineering Decontamination. Miscellaneous Enhanced natural attenuation Exact sciences and technology Groundwaters Hyperaccumulation Immobilization In situ remediation Natural water pollution Oxidation-Reduction Pollution Safety Soil and sediments pollution Soil Pollutants - chemistry Soil Pollutants - metabolism Water Pollutants, Chemical - chemistry Water Pollutants, Chemical - metabolism Water treatment and pollution
Title	Natural attenuation processes for remediation of arsenic contaminated soils and groundwater
URI	https://dx.doi.org/10.1016/j.jhazmat.2006.09.048 https://www.ncbi.nlm.nih.gov/pubmed/17049728 https://www.proquest.com/docview/14795599 https://www.proquest.com/docview/19777043 https://www.proquest.com/docview/29554828 https://www.proquest.com/docview/29805704 https://www.proquest.com/docview/68126326
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