Adsorption of chromium (VI) by ethylenediamine-modified cross-linked magnetic chitosan resin: Isotherms, kinetics and thermodynamics
The adsorption of chromium (VI) ions from aqueous solution by ethylenediamine-modified cross-linked magnetic chitosan resin (EMCMCR) was studied in a batch adsorption system. Chromium (VI) removal is pH dependent and the optimum adsorption was observed at pH 2.0. The adsorption rate was extremely fa...
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| Published in | Journal of hazardous materials Vol. 185; no. 1; pp. 306 - 314 |
|---|---|
| Main Authors | , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Kidlington
Elsevier B.V
15.01.2011
Elsevier |
| Subjects | |
| Online Access | Get full text |
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| Abstract | The adsorption of chromium (VI) ions from aqueous solution by ethylenediamine-modified cross-linked magnetic chitosan resin (EMCMCR) was studied in a batch adsorption system. Chromium (VI) removal is pH dependent and the optimum adsorption was observed at pH 2.0. The adsorption rate was extremely fast and the equilibrium was established within 6–10
min. The adsorption data could be well interpreted by the Langmuir and Temkin model. The maximum adsorption capacities obtained from the Langmuir model are 51.813
mg
g
−1, 48.780
mg
g
−1 and 45.872
mg
g
−1 at 293, 303 and 313
K, respectively. The adsorption process could be described by pseudo-second-order kinetic model. The intraparticle diffusion study revealed that film diffusion might be involved in the present case. Thermodynamic parameters revealed the feasibility, spontaneity and exothermic nature of adsorption. The sorbents were successfully regenerated using 0.1
N NaOH solutions. |
|---|---|
| AbstractList | The adsorption of chromium (VI) ions from aqueous solution by ethylenediamine-modified cross-linked magnetic chitosan resin (EMCMCR) was studied in a batch adsorption system. Chromium (VI) removal is pH dependent and the optimum adsorption was observed at pH 2.0. The adsorption rate was extremely fast and the equilibrium was established within 6-10min. The adsorption data could be well interpreted by the Langmuir and Temkin model. The maximum adsorption capacities obtained from the Langmuir model are 51.813mgg(-1), 48.780mgg(-1) and 45.872mgg(-1) at 293, 303 and 313K, respectively. The adsorption process could be described by pseudo-second-order kinetic model. The intraparticle diffusion study revealed that film diffusion might be involved in the present case. Thermodynamic parameters revealed the feasibility, spontaneity and exothermic nature of adsorption. The sorbents were successfully regenerated using 0.1N NaOH solutions.The adsorption of chromium (VI) ions from aqueous solution by ethylenediamine-modified cross-linked magnetic chitosan resin (EMCMCR) was studied in a batch adsorption system. Chromium (VI) removal is pH dependent and the optimum adsorption was observed at pH 2.0. The adsorption rate was extremely fast and the equilibrium was established within 6-10min. The adsorption data could be well interpreted by the Langmuir and Temkin model. The maximum adsorption capacities obtained from the Langmuir model are 51.813mgg(-1), 48.780mgg(-1) and 45.872mgg(-1) at 293, 303 and 313K, respectively. The adsorption process could be described by pseudo-second-order kinetic model. The intraparticle diffusion study revealed that film diffusion might be involved in the present case. Thermodynamic parameters revealed the feasibility, spontaneity and exothermic nature of adsorption. The sorbents were successfully regenerated using 0.1N NaOH solutions. The adsorption of chromium (VI) ions from aqueous solution by ethylenediamine-modified cross-linked magnetic chitosan resin (EMCMCR) was studied in a batch adsorption system. Chromium (VI) removal is pH dependent and the optimum adsorption was observed at pH 2.0. The adsorption rate was extremely fast and the equilibrium was established within 6-10min. The adsorption data could be well interpreted by the Langmuir and Temkin model. The maximum adsorption capacities obtained from the Langmuir model are 51.813mgg(-1), 48.780mgg(-1) and 45.872mgg(-1) at 293, 303 and 313K, respectively. The adsorption process could be described by pseudo-second-order kinetic model. The intraparticle diffusion study revealed that film diffusion might be involved in the present case. Thermodynamic parameters revealed the feasibility, spontaneity and exothermic nature of adsorption. The sorbents were successfully regenerated using 0.1N NaOH solutions. The adsorption of chromium (VI) ions from aqueous solution by ethylenediamine-modified cross-linked magnetic chitosan resin (EMCMCR) was studied in a batch adsorption system. Chromium (VI) removal is pH dependent and the optimum adsorption was observed at pH 2.0. The adsorption rate was extremely fast and the equilibrium was established within 6–10 min. The adsorption data could be well interpreted by the Langmuir and Temkin model. The maximum adsorption capacities obtained from the Langmuir model are 51.813 mg g −1, 48.780 mg g −1 and 45.872 mg g −1 at 293, 303 and 313 K, respectively. The adsorption process could be described by pseudo-second-order kinetic model. The intraparticle diffusion study revealed that film diffusion might be involved in the present case. Thermodynamic parameters revealed the feasibility, spontaneity and exothermic nature of adsorption. The sorbents were successfully regenerated using 0.1 N NaOH solutions. The adsorption of chromium (VI) ions from aqueous solution by ethylenediamine-modified cross-linked magnetic chitosan resin (EMCMCR) was studied in a batch adsorption system. Chromium (VI) removal is pH dependent and the optimum adsorption was observed at pH 2.0. The adsorption rate was extremely fast and the equilibrium was established within 6–10min. The adsorption data could be well interpreted by the Langmuir and Temkin model. The maximum adsorption capacities obtained from the Langmuir model are 51.813mgg⁻¹, 48.780mgg⁻¹ and 45.872mgg⁻¹ at 293, 303 and 313K, respectively. The adsorption process could be described by pseudo-second-order kinetic model. The intraparticle diffusion study revealed that film diffusion might be involved in the present case. Thermodynamic parameters revealed the feasibility, spontaneity and exothermic nature of adsorption. The sorbents were successfully regenerated using 0.1N NaOH solutions. The adsorption of chromium (VI) ions from aqueous solution by ethylenediamine-modified cross-linked magnetic chitosan resin (EMCMCR) was studied in a batch adsorption system. Chromium (VI) removal is pH dependent and the optimum adsorption was observed at pH 2.0. The adsorption rate was extremely fast and the equilibrium was established within 6-10min. The adsorption data could be well interpreted by the Langmuir and Temkin model. The maximum adsorption capacities obtained from the Langmuir model are 51.813mgga degree 1, 48.780mgga degree 1 and 45.872mgga degree 1 at 293, 303 and 313K, respectively. The adsorption process could be described by pseudo-second-order kinetic model. The intraparticle diffusion study revealed that film diffusion might be involved in the present case. Thermodynamic parameters revealed the feasibility, spontaneity and exothermic nature of adsorption. The sorbents were successfully regenerated using 0.1N NaOH solutions. |
| Author | Wang, Jing-song Liu, Yun-guo Bao, Zheng-lei Zeng, Xiao-xia Long, Fei Hu, Xin-jiang Li, Xin Zeng, Guang-ming Chen, An-wei |
| Author_xml | – sequence: 1 givenname: Xin-jiang surname: Hu fullname: Hu, Xin-jiang organization: College of Environmental Science and Engineering, Hunan University, Changsha 410082, PR China – sequence: 2 givenname: Jing-song surname: Wang fullname: Wang, Jing-song organization: School of Urban Construction, University of South China, Hengyang, Hunan 421001, PR China – sequence: 3 givenname: Yun-guo surname: Liu fullname: Liu, Yun-guo email: hnuese@126.com organization: College of Environmental Science and Engineering, Hunan University, Changsha 410082, PR China – sequence: 4 givenname: Xin surname: Li fullname: Li, Xin organization: College of Environmental Science and Engineering, Hunan University, Changsha 410082, PR China – sequence: 5 givenname: Guang-ming surname: Zeng fullname: Zeng, Guang-ming organization: College of Environmental Science and Engineering, Hunan University, Changsha 410082, PR China – sequence: 6 givenname: Zheng-lei surname: Bao fullname: Bao, Zheng-lei organization: School of Urban Construction, University of South China, Hengyang, Hunan 421001, PR China – sequence: 7 givenname: Xiao-xia surname: Zeng fullname: Zeng, Xiao-xia organization: College of Environmental Science and Engineering, Hunan University, Changsha 410082, PR China – sequence: 8 givenname: An-wei surname: Chen fullname: Chen, An-wei organization: College of Environmental Science and Engineering, Hunan University, Changsha 410082, PR China – sequence: 9 givenname: Fei surname: Long fullname: Long, Fei organization: College of Environmental Science and Engineering, Hunan University, Changsha 410082, PR China |
| BackLink | http://pascal-francis.inist.fr/vibad/index.php?action=getRecordDetail&idt=23819525$$DView record in Pascal Francis https://www.ncbi.nlm.nih.gov/pubmed/20889258$$D View this record in MEDLINE/PubMed |
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| SubjectTerms | Adsorption Algorithms Applied sciences Chemical engineering chemistry chitosan Chitosan - chemistry Chromium Chromium (VI) Chromium - chemistry Cross-Linking Reagents Crosslinking Diffusion EMCMCR Equilibrium isotherm Ethylenediamines Ethylenediamines - chemistry Exact sciences and technology heat production Hydrogen-Ion Concentration ions Kinetics Langmuir-Blodgett films Magnetics Mathematical models Microscopy, Electron, Scanning Models, Chemical Pollution Polymers sodium hydroxide sorption isotherms Temperature Thermodynamics |
| Title | Adsorption of chromium (VI) by ethylenediamine-modified cross-linked magnetic chitosan resin: Isotherms, kinetics and thermodynamics |
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