Efficient Conversion of Lignin to Electricity Using a Novel Direct Biomass Fuel Cell Mediated by Polyoxometalates at Low Temperatures
A novel polyoxometalates (POMs) mediated direct biomass fuel cell (DBFC) was used in this study to directly convert lignin to electricity at low temperatures with high power output and Faradaic efficiency. When phosphomolybdic acid H3PMo12O40 (PMo12) was used as the electron and proton carrier in th...
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| Published in | ChemSusChem Vol. 9; no. 2; pp. 197 - 207 |
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| Main Authors | , |
| Format | Journal Article |
| Language | English |
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Germany
Blackwell Publishing Ltd
01.01.2016
Wiley Subscription Services, Inc |
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| Abstract | A novel polyoxometalates (POMs) mediated direct biomass fuel cell (DBFC) was used in this study to directly convert lignin to electricity at low temperatures with high power output and Faradaic efficiency. When phosphomolybdic acid H3PMo12O40 (PMo12) was used as the electron and proton carrier in the anode solution with a carbon electrode, and O2 was directly used as the final electron acceptor under the catalysis of Pt, the peak power density reached 0.96 mW cm−2, 560 times higher than that of phenol‐fueled microbial fuel cells (MFCs). When the cathode reaction was catalyzed by PMo12, the power density could be greatly enhanced to 5 mW cm−2. Continuous operation demonstrated that this novel fuel cell was promising as a stable electrochemical power source. Structure analysis of the lignin indicated that the hydroxyl group content was reduced whereas the carbonyl group content increased. Both condensation and depolymerization takes place during the PMo12 oxidation of lignin.
POMs full of energy! Polyoxometalates (POMs) mediated direct biomass fuel cells (DBFC) are used to directly convert lignin to electricity at low temperatures with high power output and Faradaic efficiency. Continuous operation demonstrated that the fuel cells are promising as a stable electrochemical power sources. Both condensation and depolymerization took place during the POM oxidation of lignin. |
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| AbstractList | A novel polyoxometalates (POMs) mediated direct biomass fuel cell (DBFC) was used in this study to directly convert lignin to electricity at low temperatures with high power output and Faradaic efficiency. When phosphomolybdic acid H3 PMo12 O40 (PMo12) was used as the electron and proton carrier in the anode solution with a carbon electrode, and O2 was directly used as the final electron acceptor under the catalysis of Pt, the peak power density reached 0.96 mW cm(-2), 560 times higher than that of phenol-fueled microbial fuel cells (MFCs). When the cathode reaction was catalyzed by PMo12, the power density could be greatly enhanced to 5 mW cm(-2). Continuous operation demonstrated that this novel fuel cell was promising as a stable electrochemical power source. Structure analysis of the lignin indicated that the hydroxyl group content was reduced whereas the carbonyl group content increased. Both condensation and depolymerization takes place during the PMo12 oxidation of lignin.A novel polyoxometalates (POMs) mediated direct biomass fuel cell (DBFC) was used in this study to directly convert lignin to electricity at low temperatures with high power output and Faradaic efficiency. When phosphomolybdic acid H3 PMo12 O40 (PMo12) was used as the electron and proton carrier in the anode solution with a carbon electrode, and O2 was directly used as the final electron acceptor under the catalysis of Pt, the peak power density reached 0.96 mW cm(-2), 560 times higher than that of phenol-fueled microbial fuel cells (MFCs). When the cathode reaction was catalyzed by PMo12, the power density could be greatly enhanced to 5 mW cm(-2). Continuous operation demonstrated that this novel fuel cell was promising as a stable electrochemical power source. Structure analysis of the lignin indicated that the hydroxyl group content was reduced whereas the carbonyl group content increased. Both condensation and depolymerization takes place during the PMo12 oxidation of lignin. A novel polyoxometalates (POMs) mediated direct biomass fuel cell (DBFC) was used in this study to directly convert lignin to electricity at low temperatures with high power output and Faradaic efficiency. When phosphomolybdic acid H3PMo12O40 (PMo12) was used as the electron and proton carrier in the anode solution with a carbon electrode, and O2 was directly used as the final electron acceptor under the catalysis of Pt, the peak power density reached 0.96mWcm-2, 560times higher than that of phenol-fueled microbial fuel cells (MFCs). When the cathode reaction was catalyzed by PMo12, the power density could be greatly enhanced to 5mWcm-2. Continuous operation demonstrated that this novel fuel cell was promising as a stable electrochemical power source. Structure analysis of the lignin indicated that the hydroxyl group content was reduced whereas the carbonyl group content increased. Both condensation and depolymerization takes place during the PMo12 oxidation of lignin. A novel polyoxometalates (POMs) mediated direct biomass fuel cell (DBFC) was used in this study to directly convert lignin to electricity at low temperatures with high power output and Faradaic efficiency. When phosphomolybdic acid H 3 PMo 12 O 40 (PMo 12 ) was used as the electron and proton carrier in the anode solution with a carbon electrode, and O 2 was directly used as the final electron acceptor under the catalysis of Pt, the peak power density reached 0.96 mW cm −2 , 560 times higher than that of phenol‐fueled microbial fuel cells (MFCs). When the cathode reaction was catalyzed by PMo 12 , the power density could be greatly enhanced to 5 mW cm −2 . Continuous operation demonstrated that this novel fuel cell was promising as a stable electrochemical power source. Structure analysis of the lignin indicated that the hydroxyl group content was reduced whereas the carbonyl group content increased. Both condensation and depolymerization takes place during the PMo 12 oxidation of lignin. A novel polyoxometalates (POMs) mediated direct biomass fuel cell (DBFC) was used in this study to directly convert lignin to electricity at low temperatures with high power output and Faradaic efficiency. When phosphomolybdic acid H sub(3)PMo sub(12)O sub(40 ) (PMo sub(12)) was used as the electron and proton carrier in the anode solution with a carbon electrode, and O sub(2) was directly used as the final electron acceptor under the catalysis of Pt, the peak power density reached 0.96mWcm super(-2), 560times higher than that of phenol-fueled microbial fuel cells (MFCs). When the cathode reaction was catalyzed by PMo sub(12), the power density could be greatly enhanced to 5mWcm super(-2). Continuous operation demonstrated that this novel fuel cell was promising as a stable electrochemical power source. Structure analysis of the lignin indicated that the hydroxyl group content was reduced whereas the carbonyl group content increased. Both condensation and depolymerization takes place during the PMo sub(12) oxidation of lignin. POMs full of energy! Polyoxometalates (POMs) mediated direct biomass fuel cells (DBFC) are used to directly convert lignin to electricity at low temperatures with high power output and Faradaic efficiency. Continuous operation demonstrated that the fuel cells are promising as a stable electrochemical power sources. Both condensation and depolymerization took place during the POM oxidation of lignin. A novel polyoxometalates (POMs) mediated direct biomass fuel cell (DBFC) was used in this study to directly convert lignin to electricity at low temperatures with high power output and Faradaic efficiency. When phosphomolybdic acid H3PMo12O40 (PMo12) was used as the electron and proton carrier in the anode solution with a carbon electrode, and O2 was directly used as the final electron acceptor under the catalysis of Pt, the peak power density reached 0.96 mW cm−2, 560 times higher than that of phenol‐fueled microbial fuel cells (MFCs). When the cathode reaction was catalyzed by PMo12, the power density could be greatly enhanced to 5 mW cm−2. Continuous operation demonstrated that this novel fuel cell was promising as a stable electrochemical power source. Structure analysis of the lignin indicated that the hydroxyl group content was reduced whereas the carbonyl group content increased. Both condensation and depolymerization takes place during the PMo12 oxidation of lignin. POMs full of energy! Polyoxometalates (POMs) mediated direct biomass fuel cells (DBFC) are used to directly convert lignin to electricity at low temperatures with high power output and Faradaic efficiency. Continuous operation demonstrated that the fuel cells are promising as a stable electrochemical power sources. Both condensation and depolymerization took place during the POM oxidation of lignin. A novel polyoxometalates (POMs) mediated direct biomass fuel cell (DBFC) was used in this study to directly convert lignin to electricity at low temperatures with high power output and Faradaic efficiency. When phosphomolybdic acid H3 PMo12 O40 (PMo12) was used as the electron and proton carrier in the anode solution with a carbon electrode, and O2 was directly used as the final electron acceptor under the catalysis of Pt, the peak power density reached 0.96 mW cm(-2), 560 times higher than that of phenol-fueled microbial fuel cells (MFCs). When the cathode reaction was catalyzed by PMo12, the power density could be greatly enhanced to 5 mW cm(-2). Continuous operation demonstrated that this novel fuel cell was promising as a stable electrochemical power source. Structure analysis of the lignin indicated that the hydroxyl group content was reduced whereas the carbonyl group content increased. Both condensation and depolymerization takes place during the PMo12 oxidation of lignin. |
| Author | Zhao, Xuebing Zhu, J. Y. |
| Author_xml | – sequence: 1 givenname: Xuebing surname: Zhao fullname: Zhao, Xuebing organization: Department of Chemical Engineering, Tsinghua University, Beijing, P.R. China – sequence: 2 givenname: J. Y. surname: Zhu fullname: Zhu, J. Y. email: jzhu@fs.fed.us organization: Department of Biological Systems Engineering, University of Wisconsin, Madison, WI, USA |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/26692572$$D View this record in MEDLINE/PubMed |
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| Keywords | power density direct biomass fuel cells phosphomolybdic acids lignins polyoxometalates |
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| Snippet | A novel polyoxometalates (POMs) mediated direct biomass fuel cell (DBFC) was used in this study to directly convert lignin to electricity at low temperatures... |
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| SubjectTerms | Bioelectric Energy Sources Biomass Catalysis direct biomass fuel cells Electrodes Fuel cells Industrial Waste Lignin Lignin - chemistry lignins Oxidants - chemistry Oxidation-Reduction phosphomolybdic acids polyoxometalates power density Temperature Tungsten Compounds - chemistry |
| Title | Efficient Conversion of Lignin to Electricity Using a Novel Direct Biomass Fuel Cell Mediated by Polyoxometalates at Low Temperatures |
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