Pairwise frictional profile between particles determines discontinuous shear thickening transition in non-colloidal suspensions
The process by which sheared suspensions go through a dramatic change in viscosity is known as discontinuous shear thickening. Although well-characterized on the macroscale, the microscopic mechanisms at play in this transition are still poorly understood. Here, by developing new experimental proced...
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| Published in | Nature communications Vol. 8; no. 1; pp. 15633 - 7 |
|---|---|
| Main Authors | , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
London
Nature Publishing Group UK
31.05.2017
Nature Publishing Group Nature Portfolio |
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| Abstract | The process by which sheared suspensions go through a dramatic change in viscosity is known as discontinuous shear thickening. Although well-characterized on the macroscale, the microscopic mechanisms at play in this transition are still poorly understood. Here, by developing new experimental procedures based on quartz-tuning fork atomic force microscopy, we measure the pairwise frictional profile between approaching pairs of polyvinyl chloride and cornstarch particles in solvent. We report a clear transition from a low-friction regime, where pairs of particles support a finite normal load, while interacting purely hydrodynamically, to a high-friction regime characterized by hard repulsive contact between the particles and sliding friction. Critically, we show that the normal stress needed to enter the frictional regime at nanoscale matches the critical stress at which shear thickening occurs for macroscopic suspensions. Our experiments bridge nano and macroscales and provide long needed demonstration of the role of frictional forces in discontinuous shear thickening.
Shear thickening characterizes liquid suspensions of particles that reversibly solidify subject to stress. Here, Comtet
et al
. show that shear thickening occurs at the transition from lubricated contacts to frictional contacts at a single-particle level, which can be linked to the change in macroscopic rheology. |
|---|---|
| AbstractList | Shear thickening characterizes liquid suspensions of particles that reversibly solidify subject to stress. Here, Comtetet al. show that shear thickening occurs at the transition from lubricated contacts to frictional contacts at a single-particle level, which can be linked to the change in macroscopic rheology. The process by which sheared suspensions go through a dramatic change in viscosity is known as discontinuous shear thickening. Although well-characterized on the macroscale, the microscopic mechanisms at play in this transition are still poorly understood. Here, by developing new experimental procedures based on quartz-tuning fork atomic force microscopy, we measure the pairwise frictional profile between approaching pairs of polyvinyl chloride and cornstarch particles in solvent. We report a clear transition from a low-friction regime, where pairs of particles support a finite normal load, while interacting purely hydrodynamically, to a high-friction regime characterized by hard repulsive contact between the particles and sliding friction. Critically, we show that the normal stress needed to enter the frictional regime at nanoscale matches the critical stress at which shear thickening occurs for macroscopic suspensions. Our experiments bridge nano and macroscales and provide long needed demonstration of the role of frictional forces in discontinuous shear thickening.The process by which sheared suspensions go through a dramatic change in viscosity is known as discontinuous shear thickening. Although well-characterized on the macroscale, the microscopic mechanisms at play in this transition are still poorly understood. Here, by developing new experimental procedures based on quartz-tuning fork atomic force microscopy, we measure the pairwise frictional profile between approaching pairs of polyvinyl chloride and cornstarch particles in solvent. We report a clear transition from a low-friction regime, where pairs of particles support a finite normal load, while interacting purely hydrodynamically, to a high-friction regime characterized by hard repulsive contact between the particles and sliding friction. Critically, we show that the normal stress needed to enter the frictional regime at nanoscale matches the critical stress at which shear thickening occurs for macroscopic suspensions. Our experiments bridge nano and macroscales and provide long needed demonstration of the role of frictional forces in discontinuous shear thickening. The process by which sheared suspensions go through a dramatic change in viscosity is known as discontinuous shear thickening. Although well-characterized on the macroscale, the microscopic mechanisms at play in this transition are still poorly understood. Here, by developing new experimental procedures based on quartz-tuning fork atomic force microscopy, we measure the pairwise frictional profile between approaching pairs of polyvinyl chloride and cornstarch particles in solvent. We report a clear transition from a low-friction regime, where pairs of particles support a finite normal load, while interacting purely hydrodynamically, to a high-friction regime characterized by hard repulsive contact between the particles and sliding friction. Critically, we show that the normal stress needed to enter the frictional regime at nanoscale matches the critical stress at which shear thickening occurs for macroscopic suspensions. Our experiments bridge nano and macroscales and provide long needed demonstration of the role of frictional forces in discontinuous shear thickening The process by which sheared suspensions go through a dramatic change in viscosity is known as discontinuous shear thickening. Although well-characterized on the macroscale, the microscopic mechanisms at play in this transition are still poorly understood. Here, by developing new experimental procedures based on quartz-tuning fork atomic force microscopy, we measure the pairwise frictional profile between approaching pairs of polyvinyl chloride and cornstarch particles in solvent. We report a clear transition from a low-friction regime, where pairs of particles support a finite normal load, while interacting purely hydrodynamically, to a high-friction regime characterized by hard repulsive contact between the particles and sliding friction. Critically, we show that the normal stress needed to enter the frictional regime at nanoscale matches the critical stress at which shear thickening occurs for macroscopic suspensions. Our experiments bridge nano and macroscales and provide long needed demonstration of the role of frictional forces in discontinuous shear thickening. The process by which sheared suspensions go through a dramatic change in viscosity is known as discontinuous shear thickening. Although well-characterized on the macroscale, the microscopic mechanisms at play in this transition are still poorly understood. Here, by developing new experimental procedures based on quartz-tuning fork atomic force microscopy, we measure the pairwise frictional profile between approaching pairs of polyvinyl chloride and cornstarch particles in solvent. We report a clear transition from a low-friction regime, where pairs of particles support a finite normal load, while interacting purely hydrodynamically, to a high-friction regime characterized by hard repulsive contact between the particles and sliding friction. Critically, we show that the normal stress needed to enter the frictional regime at nanoscale matches the critical stress at which shear thickening occurs for macroscopic suspensions. Our experiments bridge nano and macroscales and provide long needed demonstration of the role of frictional forces in discontinuous shear thickening. Shear thickening characterizes liquid suspensions of particles that reversibly solidify subject to stress. Here, Comtet et al . show that shear thickening occurs at the transition from lubricated contacts to frictional contacts at a single-particle level, which can be linked to the change in macroscopic rheology. |
| ArticleNumber | 15633 |
| Author | Bocquet, Lydéric Comtet, Jean Niguès, Antoine Chatté, Guillaume Siria, Alessandro Colin, Annie |
| Author_xml | – sequence: 1 givenname: Jean surname: Comtet fullname: Comtet, Jean organization: Laboratoire de Physique Statistique, Ecole Normale Supérieure, UMR CNRS 8550, PSL Research University – sequence: 2 givenname: Guillaume surname: Chatté fullname: Chatté, Guillaume organization: ESPCI Paris, Sciences et Ingénierie de la Matière Molle, CNRS UMR 7615 10, PSL Research University – sequence: 3 givenname: Antoine surname: Niguès fullname: Niguès, Antoine organization: Laboratoire de Physique Statistique, Ecole Normale Supérieure, UMR CNRS 8550, PSL Research University – sequence: 4 givenname: Lydéric surname: Bocquet fullname: Bocquet, Lydéric organization: Laboratoire de Physique Statistique, Ecole Normale Supérieure, UMR CNRS 8550, PSL Research University – sequence: 5 givenname: Alessandro surname: Siria fullname: Siria, Alessandro organization: Laboratoire de Physique Statistique, Ecole Normale Supérieure, UMR CNRS 8550, PSL Research University – sequence: 6 givenname: Annie surname: Colin fullname: Colin, Annie email: annie.colin@espci.fr organization: ESPCI Paris, Sciences et Ingénierie de la Matière Molle, CNRS UMR 7615 10, PSL Research University, Université de Bordeaux |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/28561032$$D View this record in MEDLINE/PubMed https://hal.science/hal-01544102$$DView record in HAL |
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| Snippet | The process by which sheared suspensions go through a dramatic change in viscosity is known as discontinuous shear thickening. Although well-characterized on... Shear thickening characterizes liquid suspensions of particles that reversibly solidify subject to stress. Here, Comtetet al. show that shear thickening occurs... |
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| SubjectTerms | 639/301 639/766/189 639/766/930 Composite materials Condensed Matter Electron microscopes Fluid mechanics Friction Humanities and Social Sciences Mechanics multidisciplinary Physics Polyvinyl chloride Rheology Science Science (multidisciplinary) Sliding friction Soft Condensed Matter Solvents Viscosity |
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| Title | Pairwise frictional profile between particles determines discontinuous shear thickening transition in non-colloidal suspensions |
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