Earth-Abundant Nanomaterials for Oxygen Reduction

Replacing the rare and precious platinum (Pt) electrocatalysts with earth‐abundant materials for promoting the oxygen reduction reaction (ORR) at the cathode of fuel cells is of great interest in developing high‐performance sustainable energy devices. However, the challenging issues associated with...

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Published in	Angewandte Chemie International Edition Vol. 55; no. 8; pp. 2650 - 2676
Main Authors	Xia, Wei, Mahmood, Asif, Liang, Zibin, Zou, Ruqiang, Guo, Shaojun
Format	Journal Article
Language	English
Published	Germany Blackwell Publishing Ltd 18.02.2016 Wiley Subscription Services, Inc
Edition	International ed. in English
Subjects	Catalysis Catalytic activity Design engineering Design optimization Devices Earth Electrocatalysts Energy Fuel cells Fuels Mass transport Nanomaterials Nanostructure Nanotechnology Oxygen oxygen reduction Oxygen reduction reactions Platinum platinum-free catalysts Renewable energy Sustainable energy Transport properties fuel cells nanostructure electrocatalysts platinum-free catalysts oxygen reduction
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Abstract	Replacing the rare and precious platinum (Pt) electrocatalysts with earth‐abundant materials for promoting the oxygen reduction reaction (ORR) at the cathode of fuel cells is of great interest in developing high‐performance sustainable energy devices. However, the challenging issues associated with non‐Pt materials are still their low intrinsic catalytic activity, limited active sites, and the poor mass transport properties. Recent advances in material sciences and nanotechnology enable rational design of new earth‐abundant materials with optimized composition and fine nanostructure, providing new opportunities for enhancing ORR performance at the molecular level. This Review highlights recent breakthroughs in engineering nanocatalysts based on the earth‐abundant materials for boosting ORR. Pt free: Great efforts have been devoted to designing and optimizing earth‐abundant nanomaterials for use as catalysts for the oxygen reduction reaction (ORR). These new catalysts have improved intrinsic catalytic activity, stability, and selectivity as well as performances nearing that of the classical platinum‐based catalysts. This Review highlights the recent breakthroughs in engineering non‐Pt nanomaterials with advanced structures for enhanced ORR catalysis.
AbstractList	Replacing the rare and precious platinum (Pt) electrocatalysts with earth-abundant materials for promoting the oxygen reduction reaction (ORR) at the cathode of fuel cells is of great interest in developing high-performance sustainable energy devices. However, the challenging issues associated with non-Pt materials are still their low intrinsic catalytic activity, limited active sites, and the poor mass transport properties. Recent advances in material sciences and nanotechnology enable rational design of new earth-abundant materials with optimized composition and fine nanostructure, providing new opportunities for enhancing ORR performance at the molecular level. This Review highlights recent breakthroughs in engineering nanocatalysts based on the earth-abundant materials for boosting ORR.Replacing the rare and precious platinum (Pt) electrocatalysts with earth-abundant materials for promoting the oxygen reduction reaction (ORR) at the cathode of fuel cells is of great interest in developing high-performance sustainable energy devices. However, the challenging issues associated with non-Pt materials are still their low intrinsic catalytic activity, limited active sites, and the poor mass transport properties. Recent advances in material sciences and nanotechnology enable rational design of new earth-abundant materials with optimized composition and fine nanostructure, providing new opportunities for enhancing ORR performance at the molecular level. This Review highlights recent breakthroughs in engineering nanocatalysts based on the earth-abundant materials for boosting ORR. Replacing the rare and precious platinum (Pt) electrocatalysts with earth‐abundant materials for promoting the oxygen reduction reaction (ORR) at the cathode of fuel cells is of great interest in developing high‐performance sustainable energy devices. However, the challenging issues associated with non‐Pt materials are still their low intrinsic catalytic activity, limited active sites, and the poor mass transport properties. Recent advances in material sciences and nanotechnology enable rational design of new earth‐abundant materials with optimized composition and fine nanostructure, providing new opportunities for enhancing ORR performance at the molecular level. This Review highlights recent breakthroughs in engineering nanocatalysts based on the earth‐abundant materials for boosting ORR. Pt free: Great efforts have been devoted to designing and optimizing earth‐abundant nanomaterials for use as catalysts for the oxygen reduction reaction (ORR). These new catalysts have improved intrinsic catalytic activity, stability, and selectivity as well as performances nearing that of the classical platinum‐based catalysts. This Review highlights the recent breakthroughs in engineering non‐Pt nanomaterials with advanced structures for enhanced ORR catalysis. Replacing the rare and precious platinum (Pt) electrocatalysts with earth-abundant materials for promoting the oxygen reduction reaction (ORR) at the cathode of fuel cells is of great interest in developing high-performance sustainable energy devices. However, the challenging issues associated with non-Pt materials are still their low intrinsic catalytic activity, limited active sites, and the poor mass transport properties. Recent advances in material sciences and nanotechnology enable rational design of new earth-abundant materials with optimized composition and fine nanostructure, providing new opportunities for enhancing ORR performance at the molecular level. This Review highlights recent breakthroughs in engineering nanocatalysts based on the earth-abundant materials for boosting ORR.
Author	Xia, Wei Guo, Shaojun Mahmood, Asif Zou, Ruqiang Liang, Zibin
Author_xml	– sequence: 1 givenname: Wei surname: Xia fullname: Xia, Wei organization: Materials Science & Engineering, College of Engineering, Peking University, 100871, Beijing, P. R. China – sequence: 2 givenname: Asif surname: Mahmood fullname: Mahmood, Asif organization: Materials Science & Engineering, College of Engineering, Peking University, 100871, Beijing, P. R. China – sequence: 3 givenname: Zibin surname: Liang fullname: Liang, Zibin organization: Materials Science & Engineering, College of Engineering, Peking University, 100871, Beijing, P. R. China – sequence: 4 givenname: Ruqiang surname: Zou fullname: Zou, Ruqiang email: rzou@pku.edu.cn organization: Materials Science & Engineering, College of Engineering, Peking University, 100871, Beijing, P. R. China – sequence: 5 givenname: Shaojun surname: Guo fullname: Guo, Shaojun email: guosj@pku.edu.cn organization: Materials Science & Engineering, College of Engineering, Peking University, 100871, Beijing, P. R. China
BackLink	https://www.ncbi.nlm.nih.gov/pubmed/26663778$$D View this record in MEDLINE/PubMed
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Copyright	2016 WILEY‐VCH Verlag GmbH & Co. KGaA, Weinheim 2016 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim. 2016 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim
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Keywords	fuel cells nanostructure electrocatalysts platinum-free catalysts oxygen reduction
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Notes	ArticleID:ANIE201504830 Beijing Committee of Science and Technology - No. 2012004 ark:/67375/WNG-Q80DVQ1T-Z National Natural Science Foundation of China - No. 11175006; No. 51322205; No. 21371014 istex:9F98BB82672ED354AE46C8E31B24AA7D677D0756 ObjectType-Article-1 SourceType-Scholarly Journals-1 ObjectType-Feature-2 content type line 14 ObjectType-Review-3 content type line 23
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PublicationTitle	Angewandte Chemie International Edition
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Snippet	Replacing the rare and precious platinum (Pt) electrocatalysts with earth‐abundant materials for promoting the oxygen reduction reaction (ORR) at the cathode... Replacing the rare and precious platinum (Pt) electrocatalysts with earth-abundant materials for promoting the oxygen reduction reaction (ORR) at the cathode...
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SubjectTerms	Catalysis Catalytic activity Design engineering Design optimization Devices Earth Electrocatalysts Energy Fuel cells Fuels Mass transport Nanomaterials Nanostructure Nanotechnology Oxygen oxygen reduction Oxygen reduction reactions Platinum platinum-free catalysts Renewable energy Sustainable energy Transport properties
Title	Earth-Abundant Nanomaterials for Oxygen Reduction
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