纳米Ru催化剂催化喹啉加氢反应

O643; 制备了高分散性负载型5%Ru/C催化剂,采用X射线衍射、 X射线光电子能谱和高分辨透射电镜对催化剂进行了表征.结果表明,所制得的5%Ru/C催化剂分散度高,金属钌的平均粒径小于 5 nm.在喹啉加氢反应中,催化剂显示出很高的催化活性和生成 1,2,3,4-四氢喹啉的选择性,但未检测到十氢喹啉生成.补加新鲜催化剂后, 1,2,3,4-四氢喹啉可全部转化为十氢喹啉.对喹啉加氢机理进行了探讨....

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Published inChinese journal of catalysis Vol. 28; no. 11; pp. 975 - 979
Main Author 陈骏 薛芳 付海燕 樊光银 袁茂林 陈华 李贤均
Format Journal Article
LanguageChinese
Published 四川大学化学学院有机金属络合催化研究所绿色化学与技术教育部重点实验室,四川成都,610064 2007
Subjects
1
2
3
4．四氢喹啉
催化加氧
十氢喹啉
喹啉
活性炭
钌
十氢喹啉
催化加氢
喹啉
1,2,3,4-四氢喹啉
钌
活性炭
Online AccessGet full text
ISSN0253-9837
DOI10.3321/j.issn:0253-9837.2007.11.010

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Abstract O643; 制备了高分散性负载型5%Ru/C催化剂,采用X射线衍射、 X射线光电子能谱和高分辨透射电镜对催化剂进行了表征.结果表明,所制得的5%Ru/C催化剂分散度高,金属钌的平均粒径小于 5 nm.在喹啉加氢反应中,催化剂显示出很高的催化活性和生成 1,2,3,4-四氢喹啉的选择性,但未检测到十氢喹啉生成.补加新鲜催化剂后, 1,2,3,4-四氢喹啉可全部转化为十氢喹啉.对喹啉加氢机理进行了探讨.
AbstractList 制备了高分散性负载型5％Ru／C催化剂，采用X射线衍射、X射线光电子能谱和高分辨透射电镜对催化剂进行了表征．结果表明，所制得的5％Ru／C催化剂分散度高，金属钌的平均粒径小于5nm．在喹啉加氢反应中，催化剂显示出很高的催化活性和生成1，2，3，4．四氢喹啉的选择性，但未检测到十氢喹啉生成．补加新鲜催化剂后，1，2，3，4．四氢喹啉可全部转化为十氢喹啉．对喹啉加氢机理进行了探讨．
O643; 制备了高分散性负载型5%Ru/C催化剂,采用X射线衍射、 X射线光电子能谱和高分辨透射电镜对催化剂进行了表征.结果表明,所制得的5%Ru/C催化剂分散度高,金属钌的平均粒径小于 5 nm.在喹啉加氢反应中,催化剂显示出很高的催化活性和生成 1,2,3,4-四氢喹啉的选择性,但未检测到十氢喹啉生成.补加新鲜催化剂后, 1,2,3,4-四氢喹啉可全部转化为十氢喹啉.对喹啉加氢机理进行了探讨.
Author 陈骏 薛芳 付海燕 樊光银 袁茂林 陈华 李贤均
AuthorAffiliation 四川大学化学学院有机金属络合催化研究所绿色化学与技术教育部重点实验室,四川成都610064
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Author_FL FU Haiyan
LI Xianjun
YUAN Maolin
XUE Fang
CHEN Jun
CHEN Hua
FAN Guangyin
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Issue 11
Keywords 十氢喹啉
催化加氢
喹啉
1,2,3,4-四氢喹啉
钌
活性炭
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Notes decahydroquinoline
ruthenium
catalytic hydrogenation
O643
activated carbon
quinoline
ruthenium; activated carbon; catalytic hydrogenation; quinoline; 1,2,3,4- tetrahydroquinoline;decahydroquinoline
1,2,3,4- tetrahydroquinoline
21-1195/O6
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O643; 制备了高分散性负载型5%Ru/C催化剂,采用X射线衍射、 X射线光电子能谱和高分辨透射电镜对催化剂进行了表征.结果表明,所制得的5%Ru/C催化剂分散度高,金属钌的平均粒径小于 5 nm.在喹啉加氢反应中,催化剂显示出很高的催化活性和生成...
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SubjectTerms 1
2
3
4．四氢喹啉
催化加氧
十氢喹啉
喹啉
活性炭
钌
Title 纳米Ru催化剂催化喹啉加氢反应
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