Simple non-fused electron acceptors for efficient and stable organic solar cells
The flexibility in structural design of organic semiconductors endows organic solar cells (OSCs) not only great function-tunabilities, but also high potential toward practical application. In this work, simple non-fused-ring electron acceptors are developed through two-step synthesis from single aro...
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| Published in | Nature communications Vol. 10; no. 1; pp. 2152 - 9 |
|---|---|
| Main Authors | , , , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
London
Nature Publishing Group UK
14.05.2019
Nature Publishing Group Nature Portfolio |
| Subjects | |
| Online Access | Get full text |
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| Abstract | The flexibility in structural design of organic semiconductors endows organic solar cells (OSCs) not only great function-tunabilities, but also high potential toward practical application. In this work, simple non-fused-ring electron acceptors are developed through two-step synthesis from single aromatic units for constructing efficient OSCs. With the assistance of non-covalent interactions, these rotatable non-fused acceptors (in solution) allow transiting into planar and stackable conformation in condensed solid, promoting acceptors not only feasible solution-processability, but also excellent film characteristics. As results, decent power conversion efficiencies of 10.27% and 13.97% can be achieved in single and tandem OSCs consisting of simple solution-cast blends, in which the fully unfused acceptors exhibit exceptionally low synthetic complexity index. In addition, the unfused acceptor and its based OSCs exhibit promising stabilities under continuous illumination. Overall, this work reveals valuable insights on the structural design of simple and effective electron acceptors with great practical perspectives.
Non-fullerene electron acceptors have pushed the efficiency of organic solar cells up to 15% but they all contain fused rings and are inconvenient to synthetic access. Here Yu et al. develop fully unfused acceptors featuring non-covalent intramolecular interactions, high efficiencies and high stability. |
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| AbstractList | Non-fullerene electron acceptors have pushed the efficiency of organic solar cells up to 15% but they all contain fused rings and are inconvenient to synthetic access. Here Yu et al. develop fully unfused acceptors featuring non-covalent intramolecular interactions, high efficiencies and high stability. The flexibility in structural design of organic semiconductors endows organic solar cells (OSCs) not only great function-tunabilities, but also high potential toward practical application. In this work, simple non-fused-ring electron acceptors are developed through two-step synthesis from single aromatic units for constructing efficient OSCs. With the assistance of non-covalent interactions, these rotatable non-fused acceptors (in solution) allow transiting into planar and stackable conformation in condensed solid, promoting acceptors not only feasible solution-processability, but also excellent film characteristics. As results, decent power conversion efficiencies of 10.27% and 13.97% can be achieved in single and tandem OSCs consisting of simple solution-cast blends, in which the fully unfused acceptors exhibit exceptionally low synthetic complexity index. In addition, the unfused acceptor and its based OSCs exhibit promising stabilities under continuous illumination. Overall, this work reveals valuable insights on the structural design of simple and effective electron acceptors with great practical perspectives.The flexibility in structural design of organic semiconductors endows organic solar cells (OSCs) not only great function-tunabilities, but also high potential toward practical application. In this work, simple non-fused-ring electron acceptors are developed through two-step synthesis from single aromatic units for constructing efficient OSCs. With the assistance of non-covalent interactions, these rotatable non-fused acceptors (in solution) allow transiting into planar and stackable conformation in condensed solid, promoting acceptors not only feasible solution-processability, but also excellent film characteristics. As results, decent power conversion efficiencies of 10.27% and 13.97% can be achieved in single and tandem OSCs consisting of simple solution-cast blends, in which the fully unfused acceptors exhibit exceptionally low synthetic complexity index. In addition, the unfused acceptor and its based OSCs exhibit promising stabilities under continuous illumination. Overall, this work reveals valuable insights on the structural design of simple and effective electron acceptors with great practical perspectives. The flexibility in structural design of organic semiconductors endows organic solar cells (OSCs) not only great function-tunabilities, but also high potential toward practical application. In this work, simple non-fused-ring electron acceptors are developed through two-step synthesis from single aromatic units for constructing efficient OSCs. With the assistance of non-covalent interactions, these rotatable non-fused acceptors (in solution) allow transiting into planar and stackable conformation in condensed solid, promoting acceptors not only feasible solution-processability, but also excellent film characteristics. As results, decent power conversion efficiencies of 10.27% and 13.97% can be achieved in single and tandem OSCs consisting of simple solution-cast blends, in which the fully unfused acceptors exhibit exceptionally low synthetic complexity index. In addition, the unfused acceptor and its based OSCs exhibit promising stabilities under continuous illumination. Overall, this work reveals valuable insights on the structural design of simple and effective electron acceptors with great practical perspectives. The flexibility in structural design of organic semiconductors endows organic solar cells (OSCs) not only great function-tunabilities, but also high potential toward practical application. In this work, simple non-fused-ring electron acceptors are developed through two-step synthesis from single aromatic units for constructing efficient OSCs. With the assistance of non-covalent interactions, these rotatable non-fused acceptors (in solution) allow transiting into planar and stackable conformation in condensed solid, promoting acceptors not only feasible solution-processability, but also excellent film characteristics. As results, decent power conversion efficiencies of 10.27% and 13.97% can be achieved in single and tandem OSCs consisting of simple solution-cast blends, in which the fully unfused acceptors exhibit exceptionally low synthetic complexity index. In addition, the unfused acceptor and its based OSCs exhibit promising stabilities under continuous illumination. Overall, this work reveals valuable insights on the structural design of simple and effective electron acceptors with great practical perspectives. Non-fullerene electron acceptors have pushed the efficiency of organic solar cells up to 15% but they all contain fused rings and are inconvenient to synthetic access. Here Yu et al. develop fully unfused acceptors featuring non-covalent intramolecular interactions, high efficiencies and high stability. The flexibility in structural design of organic semiconductors endows organic solar cells (OSCs) not only great function-tunabilities, but also high potential toward practical application. In this work, simple non-fused-ring electron acceptors are developed through two-step synthesis from single aromatic units for constructing efficient OSCs. With the assistance of non-covalent interactions, these rotatable non-fused acceptors (in solution) allow transiting into planar and stackable conformation in condensed solid, promoting acceptors not only feasible solution-processability, but also excellent film characteristics. As results, decent power conversion efficiencies of 10.27% and 13.97% can be achieved in single and tandem OSCs consisting of simple solution-cast blends, in which the fully unfused acceptors exhibit exceptionally low synthetic complexity index. In addition, the unfused acceptor and its based OSCs exhibit promising stabilities under continuous illumination. Overall, this work reveals valuable insights on the structural design of simple and effective electron acceptors with great practical perspectives.Non-fullerene electron acceptors have pushed the efficiency of organic solar cells up to 15% but they all contain fused rings and are inconvenient to synthetic access. Here Yu et al. develop fully unfused acceptors featuring non-covalent intramolecular interactions, high efficiencies and high stability. |
| ArticleNumber | 2152 |
| Author | Chen, Fang-Xiao Shi, Minmin Yu, Zhi-Peng Li, Chang-Zhi Yin, Jing-Lin Lu, Xinhui Lau, Tsz-Ki Chen, Hongzheng Liu, Zhi-Xi Qin, Ran Kong, Xueqian |
| Author_xml | – sequence: 1 givenname: Zhi-Peng surname: Yu fullname: Yu, Zhi-Peng organization: State Key Laboratory of Silicon Materials, MOE Key Laboratory of Macromolecular Synthesis and Functionalization, Department of Polymer Science and Engineering, Zhejiang University – sequence: 2 givenname: Zhi-Xi surname: Liu fullname: Liu, Zhi-Xi organization: State Key Laboratory of Silicon Materials, MOE Key Laboratory of Macromolecular Synthesis and Functionalization, Department of Polymer Science and Engineering, Zhejiang University – sequence: 3 givenname: Fang-Xiao surname: Chen fullname: Chen, Fang-Xiao organization: State Key Laboratory of Silicon Materials, MOE Key Laboratory of Macromolecular Synthesis and Functionalization, Department of Polymer Science and Engineering, Zhejiang University – sequence: 4 givenname: Ran surname: Qin fullname: Qin, Ran organization: State Key Laboratory of Silicon Materials, MOE Key Laboratory of Macromolecular Synthesis and Functionalization, Department of Polymer Science and Engineering, Zhejiang University – sequence: 5 givenname: Tsz-Ki surname: Lau fullname: Lau, Tsz-Ki organization: Department of Physics, The Chinese University of Hong Kong – sequence: 6 givenname: Jing-Lin surname: Yin fullname: Yin, Jing-Lin organization: Department of Chemistry, Zhejiang University – sequence: 7 givenname: Xueqian orcidid: 0000-0002-1901-9073 surname: Kong fullname: Kong, Xueqian organization: Department of Chemistry, Zhejiang University – sequence: 8 givenname: Xinhui orcidid: 0000-0002-1908-3294 surname: Lu fullname: Lu, Xinhui organization: Department of Physics, The Chinese University of Hong Kong – sequence: 9 givenname: Minmin surname: Shi fullname: Shi, Minmin organization: State Key Laboratory of Silicon Materials, MOE Key Laboratory of Macromolecular Synthesis and Functionalization, Department of Polymer Science and Engineering, Zhejiang University – sequence: 10 givenname: Chang-Zhi surname: Li fullname: Li, Chang-Zhi email: czli@zju.edu.cn organization: State Key Laboratory of Silicon Materials, MOE Key Laboratory of Macromolecular Synthesis and Functionalization, Department of Polymer Science and Engineering, Zhejiang University – sequence: 11 givenname: Hongzheng surname: Chen fullname: Chen, Hongzheng organization: State Key Laboratory of Silicon Materials, MOE Key Laboratory of Macromolecular Synthesis and Functionalization, Department of Polymer Science and Engineering, Zhejiang University |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/31089140$$D View this record in MEDLINE/PubMed |
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| SubjectTerms | 140/131 140/146 140/58 147/3 639/301 639/301/299 639/301/299/946 Conformation Electrons Energy conversion efficiency Fullerenes Humanities and Social Sciences multidisciplinary Organic chemistry Organic semiconductors Photovoltaic cells Science Science (multidisciplinary) Solar cells Structural design Structural engineering |
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| Title | Simple non-fused electron acceptors for efficient and stable organic solar cells |
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