Mechanically strong MXene/Kevlar nanofiber composite membranes as high-performance nanofluidic osmotic power generators
Two-dimensional nanofluidic channels are emerging candidates for capturing osmotic energy from salinity gradients. However, present two-dimensional nanofluidic architectures are generally constructed by simple stacking of pristine nanosheets with insufficient charge densities, and exhibit low-effici...
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| Published in | Nature communications Vol. 10; no. 1; pp. 2920 - 9 |
|---|---|
| Main Authors | , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
London
Nature Publishing Group UK
02.07.2019
Nature Publishing Group Nature Portfolio |
| Subjects | |
| Online Access | Get full text |
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| Abstract | Two-dimensional nanofluidic channels are emerging candidates for capturing osmotic energy from salinity gradients. However, present two-dimensional nanofluidic architectures are generally constructed by simple stacking of pristine nanosheets with insufficient charge densities, and exhibit low-efficiency transport dynamics, consequently resulting in undesirable power densities (<1 W m
−2
). Here we demonstrate MXene/Kevlar nanofiber composite membranes as high-performance nanofluidic osmotic power generators. By mixing river water and sea water, the power density can achieve a value of approximately 4.1 W m
−2
, outperforming the state-of-art membranes to the best of our knowledge. Experiments and theoretical calculations reveal that the correlation between surface charge of MXene and space charge brought by nanofibers plays a key role in modulating ion diffusion and can synergistically contribute to such a considerable energy conversion performance. This work highlights the promise in the coupling of surface charge and space charge in nanoconfinement for energy conversion driven by chemical potential gradients.
Nanofluidic channels can capture osmotic energy from salinity gradients, but output power densities should be improved for practical applications. Here the authors report high-strength nanosheet/nanofiber composite membranes for harvesting osmotic energy from natural water with high output power. |
|---|---|
| AbstractList | Two-dimensional nanofluidic channels are emerging candidates for capturing osmotic energy from salinity gradients. However, present two-dimensional nanofluidic architectures are generally constructed by simple stacking of pristine nanosheets with insufficient charge densities, and exhibit low-efficiency transport dynamics, consequently resulting in undesirable power densities (<1 W m
−2
). Here we demonstrate MXene/Kevlar nanofiber composite membranes as high-performance nanofluidic osmotic power generators. By mixing river water and sea water, the power density can achieve a value of approximately 4.1 W m
−2
, outperforming the state-of-art membranes to the best of our knowledge. Experiments and theoretical calculations reveal that the correlation between surface charge of MXene and space charge brought by nanofibers plays a key role in modulating ion diffusion and can synergistically contribute to such a considerable energy conversion performance. This work highlights the promise in the coupling of surface charge and space charge in nanoconfinement for energy conversion driven by chemical potential gradients.
Nanofluidic channels can capture osmotic energy from salinity gradients, but output power densities should be improved for practical applications. Here the authors report high-strength nanosheet/nanofiber composite membranes for harvesting osmotic energy from natural water with high output power. Two-dimensional nanofluidic channels are emerging candidates for capturing osmotic energy from salinity gradients. However, present two-dimensional nanofluidic architectures are generally constructed by simple stacking of pristine nanosheets with insufficient charge densities, and exhibit low-efficiency transport dynamics, consequently resulting in undesirable power densities (<1 W m−2). Here we demonstrate MXene/Kevlar nanofiber composite membranes as high-performance nanofluidic osmotic power generators. By mixing river water and sea water, the power density can achieve a value of approximately 4.1 W m−2, outperforming the state-of-art membranes to the best of our knowledge. Experiments and theoretical calculations reveal that the correlation between surface charge of MXene and space charge brought by nanofibers plays a key role in modulating ion diffusion and can synergistically contribute to such a considerable energy conversion performance. This work highlights the promise in the coupling of surface charge and space charge in nanoconfinement for energy conversion driven by chemical potential gradients. Two-dimensional nanofluidic channels are emerging candidates for capturing osmotic energy from salinity gradients. However, present two-dimensional nanofluidic architectures are generally constructed by simple stacking of pristine nanosheets with insufficient charge densities, and exhibit low-efficiency transport dynamics, consequently resulting in undesirable power densities (<1 W m-2). Here we demonstrate MXene/Kevlar nanofiber composite membranes as high-performance nanofluidic osmotic power generators. By mixing river water and sea water, the power density can achieve a value of approximately 4.1 W m-2, outperforming the state-of-art membranes to the best of our knowledge. Experiments and theoretical calculations reveal that the correlation between surface charge of MXene and space charge brought by nanofibers plays a key role in modulating ion diffusion and can synergistically contribute to such a considerable energy conversion performance. This work highlights the promise in the coupling of surface charge and space charge in nanoconfinement for energy conversion driven by chemical potential gradients.Two-dimensional nanofluidic channels are emerging candidates for capturing osmotic energy from salinity gradients. However, present two-dimensional nanofluidic architectures are generally constructed by simple stacking of pristine nanosheets with insufficient charge densities, and exhibit low-efficiency transport dynamics, consequently resulting in undesirable power densities (<1 W m-2). Here we demonstrate MXene/Kevlar nanofiber composite membranes as high-performance nanofluidic osmotic power generators. By mixing river water and sea water, the power density can achieve a value of approximately 4.1 W m-2, outperforming the state-of-art membranes to the best of our knowledge. Experiments and theoretical calculations reveal that the correlation between surface charge of MXene and space charge brought by nanofibers plays a key role in modulating ion diffusion and can synergistically contribute to such a considerable energy conversion performance. This work highlights the promise in the coupling of surface charge and space charge in nanoconfinement for energy conversion driven by chemical potential gradients. Two-dimensional nanofluidic channels are emerging candidates for capturing osmotic energy from salinity gradients. However, present two-dimensional nanofluidic architectures are generally constructed by simple stacking of pristine nanosheets with insufficient charge densities, and exhibit low-efficiency transport dynamics, consequently resulting in undesirable power densities (<1 W m −2 ). Here we demonstrate MXene/Kevlar nanofiber composite membranes as high-performance nanofluidic osmotic power generators. By mixing river water and sea water, the power density can achieve a value of approximately 4.1 W m −2 , outperforming the state-of-art membranes to the best of our knowledge. Experiments and theoretical calculations reveal that the correlation between surface charge of MXene and space charge brought by nanofibers plays a key role in modulating ion diffusion and can synergistically contribute to such a considerable energy conversion performance. This work highlights the promise in the coupling of surface charge and space charge in nanoconfinement for energy conversion driven by chemical potential gradients. Nanofluidic channels can capture osmotic energy from salinity gradients, but output power densities should be improved for practical applications. Here the authors report high-strength nanosheet/nanofiber composite membranes for harvesting osmotic energy from natural water with high output power. Two-dimensional nanofluidic channels are emerging candidates for capturing osmotic energy from salinity gradients. However, present two-dimensional nanofluidic architectures are generally constructed by simple stacking of pristine nanosheets with insufficient charge densities, and exhibit low-efficiency transport dynamics, consequently resulting in undesirable power densities (<1 W m ). Here we demonstrate MXene/Kevlar nanofiber composite membranes as high-performance nanofluidic osmotic power generators. By mixing river water and sea water, the power density can achieve a value of approximately 4.1 W m , outperforming the state-of-art membranes to the best of our knowledge. Experiments and theoretical calculations reveal that the correlation between surface charge of MXene and space charge brought by nanofibers plays a key role in modulating ion diffusion and can synergistically contribute to such a considerable energy conversion performance. This work highlights the promise in the coupling of surface charge and space charge in nanoconfinement for energy conversion driven by chemical potential gradients. |
| ArticleNumber | 2920 |
| Author | Yang, Sheng Zhang, Panpan Chen, Guangbo Zhang, Jian Feng, Xinliang Zhang, Zhen |
| Author_xml | – sequence: 1 givenname: Zhen surname: Zhang fullname: Zhang, Zhen organization: Center for Advancing Electronics Dresden (Cfaed) and Department of Chemistry and Food Chemistry, Technische Universität Dresden – sequence: 2 givenname: Sheng surname: Yang fullname: Yang, Sheng organization: Center for Advancing Electronics Dresden (Cfaed) and Department of Chemistry and Food Chemistry, Technische Universität Dresden – sequence: 3 givenname: Panpan orcidid: 0000-0002-3967-6548 surname: Zhang fullname: Zhang, Panpan organization: Center for Advancing Electronics Dresden (Cfaed) and Department of Chemistry and Food Chemistry, Technische Universität Dresden – sequence: 4 givenname: Jian orcidid: 0000-0002-0912-1197 surname: Zhang fullname: Zhang, Jian organization: Center for Advancing Electronics Dresden (Cfaed) and Department of Chemistry and Food Chemistry, Technische Universität Dresden – sequence: 5 givenname: Guangbo surname: Chen fullname: Chen, Guangbo organization: Center for Advancing Electronics Dresden (Cfaed) and Department of Chemistry and Food Chemistry, Technische Universität Dresden – sequence: 6 givenname: Xinliang surname: Feng fullname: Feng, Xinliang email: xinliang.feng@tu-dresden.de organization: Center for Advancing Electronics Dresden (Cfaed) and Department of Chemistry and Food Chemistry, Technische Universität Dresden |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/31266937$$D View this record in MEDLINE/PubMed |
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| Snippet | Two-dimensional nanofluidic channels are emerging candidates for capturing osmotic energy from salinity gradients. However, present two-dimensional nanofluidic... Nanofluidic channels can capture osmotic energy from salinity gradients, but output power densities should be improved for practical applications. Here the... |
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| SubjectTerms | 639/4077/4072/4062 639/638/455/303 Aramid fiber reinforced plastics Charge density Chemical potential Contact angle Energy Energy charge Energy conversion Energy conversion efficiency Etching Fluidics Generators Graphene Humanities and Social Sciences Investigations Ion diffusion Kevlar (trademark) Membranes multidisciplinary MXenes Nanofibers Nanofluids Organic chemistry Potential gradient Rivers Salinity Science Science (multidisciplinary) Seawater Space charge Surface charge |
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| Title | Mechanically strong MXene/Kevlar nanofiber composite membranes as high-performance nanofluidic osmotic power generators |
| URI | https://link.springer.com/article/10.1038/s41467-019-10885-8 https://www.ncbi.nlm.nih.gov/pubmed/31266937 https://www.proquest.com/docview/2251064795 https://www.proquest.com/docview/2251690739 https://pubmed.ncbi.nlm.nih.gov/PMC6606750 https://doaj.org/article/b679ca4abe034bd097cafe94617b8329 |
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