Collective excitation of plasmon-coupled Au-nanochain boosts photocatalytic hydrogen evolution of semiconductor
Localized surface plasmon resonance (LSPR) offers a valuable opportunity to improve the efficiency of photocatalysts. However, plasmonic enhancement of photoconversion is still limited, as most of metal-semiconductor building blocks depend on LSPR contribution of isolated metal nanoparticles. In thi...
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| Published in | Nature communications Vol. 10; no. 1; pp. 4912 - 8 |
|---|---|
| Main Authors | , , , , , , |
| Format | Journal Article |
| Language | English |
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London
Nature Publishing Group UK
29.10.2019
Nature Publishing Group Nature Portfolio |
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| Abstract | Localized surface plasmon resonance (LSPR) offers a valuable opportunity to improve the efficiency of photocatalysts. However, plasmonic enhancement of photoconversion is still limited, as most of metal-semiconductor building blocks depend on LSPR contribution of isolated metal nanoparticles. In this contribution, the concept of collective excitation of embedded metal nanoparticles is demonstrated as an effective strategy to enhance the utilization of plasmonic energy. The contribution of Au-nanochain to the enhancement of photoconversion is 3.5 times increase in comparison with that of conventional isolated Au nanoparticles. Experimental characterization and theoretical simulation show that strongly coupled plasmonic nanostructure of Au-nanochain give rise to highly intensive electromagnetic field. The enhanced strength of electromagnetic field essentially boosts the formation rate of electron-hole pair in semiconductor, and ultimately improves photocatalytic hydrogen evolution activity of semiconductor photocatalysts. The concept of embedded coupled-metal nanostructure represents a promising strategy for the rational design of high-performance photocatalysts.
Plasmonic effect offers a valuable opportunity to improve the efficiency of semiconductor, photocatalysts. Here, the authors show that the collective excitation of plasmonic metal, nanoparticles is more favorable for enhancing the utilization of plasmonic energy by, semiconductors. |
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| AbstractList | Localized surface plasmon resonance (LSPR) offers a valuable opportunity to improve the efficiency of photocatalysts. However, plasmonic enhancement of photoconversion is still limited, as most of metal-semiconductor building blocks depend on LSPR contribution of isolated metal nanoparticles. In this contribution, the concept of collective excitation of embedded metal nanoparticles is demonstrated as an effective strategy to enhance the utilization of plasmonic energy. The contribution of Au-nanochain to the enhancement of photoconversion is 3.5 times increase in comparison with that of conventional isolated Au nanoparticles. Experimental characterization and theoretical simulation show that strongly coupled plasmonic nanostructure of Au-nanochain give rise to highly intensive electromagnetic field. The enhanced strength of electromagnetic field essentially boosts the formation rate of electron-hole pair in semiconductor, and ultimately improves photocatalytic hydrogen evolution activity of semiconductor photocatalysts. The concept of embedded coupled-metal nanostructure represents a promising strategy for the rational design of high-performance photocatalysts. Abstract Localized surface plasmon resonance (LSPR) offers a valuable opportunity to improve the efficiency of photocatalysts. However, plasmonic enhancement of photoconversion is still limited, as most of metal-semiconductor building blocks depend on LSPR contribution of isolated metal nanoparticles. In this contribution, the concept of collective excitation of embedded metal nanoparticles is demonstrated as an effective strategy to enhance the utilization of plasmonic energy. The contribution of Au-nanochain to the enhancement of photoconversion is 3.5 times increase in comparison with that of conventional isolated Au nanoparticles. Experimental characterization and theoretical simulation show that strongly coupled plasmonic nanostructure of Au-nanochain give rise to highly intensive electromagnetic field. The enhanced strength of electromagnetic field essentially boosts the formation rate of electron-hole pair in semiconductor, and ultimately improves photocatalytic hydrogen evolution activity of semiconductor photocatalysts. The concept of embedded coupled-metal nanostructure represents a promising strategy for the rational design of high-performance photocatalysts. Localized surface plasmon resonance (LSPR) offers a valuable opportunity to improve the efficiency of photocatalysts. However, plasmonic enhancement of photoconversion is still limited, as most of metal-semiconductor building blocks depend on LSPR contribution of isolated metal nanoparticles. In this contribution, the concept of collective excitation of embedded metal nanoparticles is demonstrated as an effective strategy to enhance the utilization of plasmonic energy. The contribution of Au-nanochain to the enhancement of photoconversion is 3.5 times increase in comparison with that of conventional isolated Au nanoparticles. Experimental characterization and theoretical simulation show that strongly coupled plasmonic nanostructure of Au-nanochain give rise to highly intensive electromagnetic field. The enhanced strength of electromagnetic field essentially boosts the formation rate of electron-hole pair in semiconductor, and ultimately improves photocatalytic hydrogen evolution activity of semiconductor photocatalysts. The concept of embedded coupled-metal nanostructure represents a promising strategy for the rational design of high-performance photocatalysts. Plasmonic effect offers a valuable opportunity to improve the efficiency of semiconductor, photocatalysts. Here, the authors show that the collective excitation of plasmonic metal, nanoparticles is more favorable for enhancing the utilization of plasmonic energy by, semiconductors. Plasmonic effect offers a valuable opportunity to improve the efficiency of semiconductor, photocatalysts. Here, the authors show that the collective excitation of plasmonic metal, nanoparticles is more favorable for enhancing the utilization of plasmonic energy by, semiconductors. |
| ArticleNumber | 4912 |
| Author | Liu, Gang Yu, Guiyang Zhang, Peng Qian, Jun Zhang, Bo Yan, Wenfu Zhang, Wenxiang |
| Author_xml | – sequence: 1 givenname: Guiyang surname: Yu fullname: Yu, Guiyang organization: State Key Laboratory of Inorganic Synthesis and Preparative Chemistry, College of Chemistry, Jilin University – sequence: 2 givenname: Jun surname: Qian fullname: Qian, Jun organization: School of Physics, Nankai University – sequence: 3 givenname: Peng orcidid: 0000-0003-3603-0175 surname: Zhang fullname: Zhang, Peng organization: Department of Chemistry, Dalhousie University – sequence: 4 givenname: Bo surname: Zhang fullname: Zhang, Bo organization: State Key Laboratory of Inorganic Synthesis and Preparative Chemistry, College of Chemistry, Jilin University – sequence: 5 givenname: Wenxiang surname: Zhang fullname: Zhang, Wenxiang organization: State Key Laboratory of Inorganic Synthesis and Preparative Chemistry, College of Chemistry, Jilin University – sequence: 6 givenname: Wenfu orcidid: 0000-0002-1000-6559 surname: Yan fullname: Yan, Wenfu organization: State Key Laboratory of Inorganic Synthesis and Preparative Chemistry, College of Chemistry, Jilin University – sequence: 7 givenname: Gang orcidid: 0000-0001-9800-0380 surname: Liu fullname: Liu, Gang email: lgang@jlu.edu.cn organization: State Key Laboratory of Inorganic Synthesis and Preparative Chemistry, College of Chemistry, Jilin University |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/31664023$$D View this record in MEDLINE/PubMed |
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| Snippet | Localized surface plasmon resonance (LSPR) offers a valuable opportunity to improve the efficiency of photocatalysts. However, plasmonic enhancement of... Abstract Localized surface plasmon resonance (LSPR) offers a valuable opportunity to improve the efficiency of photocatalysts. However, plasmonic enhancement... Plasmonic effect offers a valuable opportunity to improve the efficiency of semiconductor, photocatalysts. Here, the authors show that the collective... |
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| SubjectTerms | 119/118 140/133 147/143 639/301/299/890 639/4077/909/4101/4102 639/638/440 639/925/357/354 Electromagnetic fields Electromagnetism Excitation Gold Holes (electron deficiencies) Humanities and Social Sciences Hydrogen evolution Metals multidisciplinary Nanoparticles Nanostructure Photocatalysis Photocatalysts Science Science (multidisciplinary) Surface plasmon resonance |
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| Title | Collective excitation of plasmon-coupled Au-nanochain boosts photocatalytic hydrogen evolution of semiconductor |
| URI | https://link.springer.com/article/10.1038/s41467-019-12853-8 https://www.ncbi.nlm.nih.gov/pubmed/31664023 https://www.proquest.com/docview/2310418945 https://search.proquest.com/docview/2310675527 https://pubmed.ncbi.nlm.nih.gov/PMC6820756 https://doaj.org/article/50a0f75064744683b433784ceeea0db9 |
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