Tuneable near white-emissive two-dimensional covalent organic frameworks
Most two-dimensional (2D) covalent organic frameworks (COFs) are non-fluorescent in the solid state even when they are constructed from emissive building blocks. The fluorescence quenching is usually attributed to non-irradiative rotation-related or π–π stacking-caused thermal energy dissipation pro...
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| Published in | Nature communications Vol. 9; no. 1; pp. 2335 - 9 |
|---|---|
| Main Authors | , , , , , , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
London
Nature Publishing Group UK
13.06.2018
Nature Publishing Group Nature Portfolio |
| Subjects | |
| Online Access | Get full text |
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| Abstract | Most two-dimensional (2D) covalent organic frameworks (COFs) are non-fluorescent in the solid state even when they are constructed from emissive building blocks. The fluorescence quenching is usually attributed to non-irradiative rotation-related or π–π stacking-caused thermal energy dissipation process. Currently there is a lack of guiding principle on how to design fluorescent, solid-state material made of COF. Herein, we demonstrate that the eclipsed stacking structure of 2D COFs can be used to turn on, and tune, the solid-state photoluminescence from non-emissive building blocks by the restriction of intramolecular bond rotation via intralayer and interlayer hydrogen bonds among highly organized layers in the eclipse-stacked COFs. Our COFs serve as a platform whereby the size of the conjugated linkers and side-chain functionalities can be varied, rendering the emission colour-tuneable from blue to yellow and even white. This work provides a guide to design new solid-state emitters using COFs.
Encoding functionalities in covalent organic frameworks (COFs) is important for widening their application field but the development of fluorescent COFs is hampered by a lack of guiding design principles. Here the authors demonstrate tuning and switching of the photoluminescence in 2D COFs made of non-emissive building blocks. |
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| AbstractList | Most two-dimensional (2D) covalent organic frameworks (COFs) are non-fluorescent in the solid state even when they are constructed from emissive building blocks. The fluorescence quenching is usually attributed to non-irradiative rotation-related or π–π stacking-caused thermal energy dissipation process. Currently there is a lack of guiding principle on how to design fluorescent, solid-state material made of COF. Herein, we demonstrate that the eclipsed stacking structure of 2D COFs can be used to turn on, and tune, the solid-state photoluminescence from non-emissive building blocks by the restriction of intramolecular bond rotation via intralayer and interlayer hydrogen bonds among highly organized layers in the eclipse-stacked COFs. Our COFs serve as a platform whereby the size of the conjugated linkers and side-chain functionalities can be varied, rendering the emission colour-tuneable from blue to yellow and even white. This work provides a guide to design new solid-state emitters using COFs. Most two-dimensional (2D) covalent organic frameworks (COFs) are non-fluorescent in the solid state even when they are constructed from emissive building blocks. The fluorescence quenching is usually attributed to non-irradiative rotation-related or π–π stacking-caused thermal energy dissipation process. Currently there is a lack of guiding principle on how to design fluorescent, solid-state material made of COF. Herein, we demonstrate that the eclipsed stacking structure of 2D COFs can be used to turn on, and tune, the solid-state photoluminescence from non-emissive building blocks by the restriction of intramolecular bond rotation via intralayer and interlayer hydrogen bonds among highly organized layers in the eclipse-stacked COFs. Our COFs serve as a platform whereby the size of the conjugated linkers and side-chain functionalities can be varied, rendering the emission colour-tuneable from blue to yellow and even white. This work provides a guide to design new solid-state emitters using COFs. Encoding functionalities in covalent organic frameworks (COFs) is important for widening their application field but the development of fluorescent COFs is hampered by a lack of guiding design principles. Here the authors demonstrate tuning and switching of the photoluminescence in 2D COFs made of non-emissive building blocks. Encoding functionalities in covalent organic frameworks (COFs) is important for widening their application field but the development of fluorescent COFs is hampered by a lack of guiding design principles. Here the authors demonstrate tuning and switching of the photoluminescence in 2D COFs made of non-emissive building blocks. Most two-dimensional (2D) covalent organic frameworks (COFs) are non-fluorescent in the solid state even when they are constructed from emissive building blocks. The fluorescence quenching is usually attributed to non-irradiative rotation-related or π-π stacking-caused thermal energy dissipation process. Currently there is a lack of guiding principle on how to design fluorescent, solid-state material made of COF. Herein, we demonstrate that the eclipsed stacking structure of 2D COFs can be used to turn on, and tune, the solid-state photoluminescence from non-emissive building blocks by the restriction of intramolecular bond rotation via intralayer and interlayer hydrogen bonds among highly organized layers in the eclipse-stacked COFs. Our COFs serve as a platform whereby the size of the conjugated linkers and side-chain functionalities can be varied, rendering the emission colour-tuneable from blue to yellow and even white. This work provides a guide to design new solid-state emitters using COFs.Most two-dimensional (2D) covalent organic frameworks (COFs) are non-fluorescent in the solid state even when they are constructed from emissive building blocks. The fluorescence quenching is usually attributed to non-irradiative rotation-related or π-π stacking-caused thermal energy dissipation process. Currently there is a lack of guiding principle on how to design fluorescent, solid-state material made of COF. Herein, we demonstrate that the eclipsed stacking structure of 2D COFs can be used to turn on, and tune, the solid-state photoluminescence from non-emissive building blocks by the restriction of intramolecular bond rotation via intralayer and interlayer hydrogen bonds among highly organized layers in the eclipse-stacked COFs. Our COFs serve as a platform whereby the size of the conjugated linkers and side-chain functionalities can be varied, rendering the emission colour-tuneable from blue to yellow and even white. This work provides a guide to design new solid-state emitters using COFs. |
| ArticleNumber | 2335 |
| Author | Chen, Zhi-Hui Wu, Jishan Xu, Qing-Hua Lu, Yixin Wang, Juefan Chen, Yifeng Li, Xing Tang, Wei Xu, Hai-Sen Leng, Kai Gao, Qiang Loh, Kian Ping Quek, Su Ying Ning, Guo-Hong |
| Author_xml | – sequence: 1 givenname: Xing surname: Li fullname: Li, Xing organization: Department of Chemistry, National University of Singapore, 3 Science Drive 3, Centre for Advanced 2D Materials, National University of Singapore, 6 Science Drive 2, NUS Graduate School for Integrative Sciences and Engineering, National University of Singapore, Centre for Life Sciences, #05-01, 28 Medical Drive – sequence: 2 givenname: Qiang surname: Gao fullname: Gao, Qiang organization: Department of Chemistry, National University of Singapore, 3 Science Drive 3 – sequence: 3 givenname: Juefan orcidid: 0000-0003-3199-7651 surname: Wang fullname: Wang, Juefan organization: Centre for Advanced 2D Materials, National University of Singapore, 6 Science Drive 2, Department of Physics, National University of Singapore, 2 Science Drive 3 – sequence: 4 givenname: Yifeng surname: Chen fullname: Chen, Yifeng organization: Centre for Advanced 2D Materials, National University of Singapore, 6 Science Drive 2, Department of Physics, National University of Singapore, 2 Science Drive 3 – sequence: 5 givenname: Zhi-Hui surname: Chen fullname: Chen, Zhi-Hui organization: Department of Chemistry, National University of Singapore, 3 Science Drive 3 – sequence: 6 givenname: Hai-Sen surname: Xu fullname: Xu, Hai-Sen organization: Department of Chemistry, National University of Singapore, 3 Science Drive 3 – sequence: 7 givenname: Wei surname: Tang fullname: Tang, Wei organization: Institute of Materials Research and Engineering, ASTAR, 2 Fusionopolis Way, Innovis – sequence: 8 givenname: Kai surname: Leng fullname: Leng, Kai organization: Department of Chemistry, National University of Singapore, 3 Science Drive 3, Centre for Advanced 2D Materials, National University of Singapore, 6 Science Drive 2 – sequence: 9 givenname: Guo-Hong orcidid: 0000-0002-5640-9062 surname: Ning fullname: Ning, Guo-Hong organization: Department of Chemistry, National University of Singapore, 3 Science Drive 3 – sequence: 10 givenname: Jishan orcidid: 0000-0002-8231-0437 surname: Wu fullname: Wu, Jishan organization: Department of Chemistry, National University of Singapore, 3 Science Drive 3 – sequence: 11 givenname: Qing-Hua orcidid: 0000-0002-4153-0767 surname: Xu fullname: Xu, Qing-Hua organization: Department of Chemistry, National University of Singapore, 3 Science Drive 3 – sequence: 12 givenname: Su Ying surname: Quek fullname: Quek, Su Ying organization: Centre for Advanced 2D Materials, National University of Singapore, 6 Science Drive 2, Department of Physics, National University of Singapore, 2 Science Drive 3 – sequence: 13 givenname: Yixin surname: Lu fullname: Lu, Yixin organization: Department of Chemistry, National University of Singapore, 3 Science Drive 3 – sequence: 14 givenname: Kian Ping surname: Loh fullname: Loh, Kian Ping email: chmlohkp@nus.edu.sg organization: Department of Chemistry, National University of Singapore, 3 Science Drive 3, Centre for Advanced 2D Materials, National University of Singapore, 6 Science Drive 2 |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/29899332$$D View this record in MEDLINE/PubMed |
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| ContentType | Journal Article |
| Copyright | The Author(s) 2018 2018. This work is published under http://creativecommons.org/licenses/by/4.0/ (the “License”). Notwithstanding the ProQuest Terms and Conditions, you may use this content in accordance with the terms of the License. |
| Copyright_xml | – notice: The Author(s) 2018 – notice: 2018. This work is published under http://creativecommons.org/licenses/by/4.0/ (the “License”). Notwithstanding the ProQuest Terms and Conditions, you may use this content in accordance with the terms of the License. |
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| DOI | 10.1038/s41467-018-04769-6 |
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| Snippet | Most two-dimensional (2D) covalent organic frameworks (COFs) are non-fluorescent in the solid state even when they are constructed from emissive building... Encoding functionalities in covalent organic frameworks (COFs) is important for widening their application field but the development of fluorescent COFs is... |
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| Title | Tuneable near white-emissive two-dimensional covalent organic frameworks |
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